Effect of leachate recirculation on the migration of copper and zinc in municipal solid waste and municipal solid waste incineration bottom ash co-disposed landfill

Municipal solid waste incinerator (MSWI) bottom ash was allowed to be disposed of with municipal solid waste (MSW) in landfill sites in the recently enacted standard of China. In this study, three sets of simulated landfill reactors, namely, conventional MSW landfill (CL), conventional MSWI bottom ash and MSW co-disposed landfill (CCL), and leachate recirculated MSWI bottom ash and MSW co-disposed landfill (RCL), were operated to investigate the environmental impact of the co-disposal. The effect of leachate recirculation on the migration of Cu and Zn in the co-disposed landfill was also presented. The results showed that the co-disposal of MSWI bottom ash with MSW would not enhance the leaching of Cu and Zn from landfill. However, the co-disposal increased the Cu and Zn contents of the refuse in the bottom layer of the landfill from 56.7 to 65.3 mg/kg and from 210 to 236 mg/kg, respectively. The recirculation of the leachate could further increase the Cu and Zn contents of the refuse in the bottom layer of the landfill to 72.9 and 441 mg/kg, respectively. Besides these observations, the results also showed that the co-disposed landfill with leachate recirculation could facilitate the stabilization of the landfill.     

Passive drainage and biofiltration of landfill gas: Australian field trial

In Australia a significant number of landfill waste disposal sites do not incorporate measures for the collection and treatment of landfill gas. This includes many old/former landfill sites, rural landfill sites, non-putrescible solid waste and inert waste landfill sites, where landfill gas generation is low and it is not commercially viable to extract and beneficially utilize the landfill gas. Previous research has demonstrated that biofiltration has the potential to degrade methane in landfill gas, however, the microbial processes can be affected by many local conditions and factors including moisture content, temperature, nutrient supply, including the availability of oxygen and methane, and the movement of gas (oxygen and methane) to/from the micro-organisms. A field scale trial is being undertaken at a landfill site in Sydney, Australia, to investigate passive drainage and biofiltration of landfill gas as a means of managing landfill gas emissions at low to moderate gas generation landfill sites. The design and construction of the trial is described and the experimental results will provide in-depth knowledge on the application of passive gas drainage and landfill gas biofiltration under Sydney (Australian) conditions, including the performance of recycled materials for the management of landfill gas emissions.     

Modelling of environmental impacts of solid waste landfilling within the life-cycle analysis program EASEWASTE

A new computer-based life-cycle assessment model (EASEWASTE) has been developed to evaluate resource and environmental consequences of solid waste management systems. This paper describes the landfilling sub-model used in the life-cycle assessment program EASEWASTE, and examines some of the implications of this sub-model. All quantities and concentrations of leachate and landfill gas can be modified by the user in order to bring them in agreement with the actual landfill that is assessed by the model. All emissions, except the generation of landfill gas, are process specific. The landfill gas generation is calculated on the basis of organic matter in the landfilled waste. A landfill assessment example is provided. For this example, the normalised environmental effects of landfill gas on global warming and photochemical smog are much greater than the environmental effects for landfill leachate or for landfill construction. A sensitivity analysis for this example indicates that the overall environmental impact is sensitive to the gas collection efficiency and the use of the gas, but not to the amount of leachate generated, or the amount of soil or liner material used in construction. The landfill model can be used for evaluating different technologies with different liners, gas and leachate collection efficiencies, and to compare the environmental consequences of landfilling with alternative waste treatment options such as incineration or anaerobic digestion.     

Assessing the true cost of landfills

The most common means for disposing of municipal solid waste is burial in a sanitary landfill. However, many landfill owners significantly underestimate the total cost of landfill disposal by considering only land and operating costs, ignoring external physical and social costs associated with landfills. This paper proposes an approach to estimating (in monetary terms) the external costs arising from the development and operation of a landfill. All cost information is based on typical U.S. landfill cost structures. The approach is illustrated by applying it to a case study of a proposed landfill in Durham, North Carolina (U.S.A.). This case study demonstrates that the method can be applied easily and yields reasonable results.     

Movement of unlined landfill under preloading surcharge

As organic solid waste is decomposed in a landfill and mass is lost due to gas and leachate formation, the landfill settles. Settlement of a landfill interferes with the rehabilitation and subsequent use of the landfill site after closure. This study examined the soil/solid waste movement at the Al-Qurain landfill in Kuwait after 15 years of closure as plans are underway for redevelopment of the landfill site that occupies about a km(2) with an average depth of 8-15m. Field experiments were conducted for 6 mo to measure soil/solid waste movement and water behavior within the landfill using two settlement plates with a level survey access, Casagrande-type piezometers, pneumatic piezometers, and magnetic probe extensometers. Previous results obtained indicated that biological decomposition of refuse continued after closure of the landfill site. The subsurface water rise enhanced the biological activities, which resulted in the production of increasing quantities of landfill gas. The refuse fill materials recorded a high movement rate under the imposed preloading as a result of an increase in the stress state. Up to 55% of the total movement was observed during the first 2 weeks of fill placement and increased to 80% within the first month of the 6-mo preloading test. Pneumatic piezometers showed an increase in water head, which is attributed to the developed pressure of gases escaping during the preloading period.     

Impact of MSW landfill on the environmental contamination of phthalate esters

This study aims to investigate the impact of MSW landfill on the contamination of phthalate esters (PAEs) in nearby environment. Landfill leachate, surface water, groundwater and soil profile samples were collected from a MSW landfill area in Wuhan, China. Contents of 16 PAEs were detected for each sample using gas chromatography method. Results showed that landfill had an obvious effect on the contamination of PAEs in groundwater, whereas showed no tremendous effect on the PAEs contamination in surface water and topsoil. Seven possible transportation processes of PAEs in landfill area were put forward. However, the especially important processes are the invasion of PAEs into aquifer through weathered crevice, horizontal transportation in aquifer and upward infiltration with groundwater. It is suggested that the whole landfill area should be engineered with seepage-proof membrane and clay so as to prevent landfill leachate from flowing out of the filling area. On the other hand, no weathering crevice is permitted in the landfill area as it will affect groundwater seriously.     

利用生活垃圾填埋场上建设飞灰固化物填埋场适宜性探讨

针对利用原有生活垃圾填埋场改扩建飞灰固化物填埋场,从勘查设计和建设角度,通过与常规生活垃圾填埋的安全和环保各相关因素对比,分析扩建前后填埋场稳定性、防渗及导排系统等勘察设计要点,研讨扩建工程新老填埋堆体基础层、防渗及导排系统等安全环保关键技术及扩建的适宜性,为扩建的可行性研究提出较为系统的技术论证思路。     

Implementation of the semi-aerobic landfill system (Fukuoka method) in developing countries: a Malaysia cost analysis

Most of the existing solid waste landfill sites in developing countries are practicing either open dumping or controlled dumping. Proper sanitary landfill concepts are not fully implemented due to technological and financial constraints. Implementation of a fully engineered sanitary landfill is necessary and a more economically feasible landfill design is crucial, particularly for developing countries. This study was carried out by focusing on the economics from the development of a new landfill site within a natural clay area with no cost of synthetic liner up to 10 years after its closure by using the Fukuoka method semi-aerobic landfill system. The findings of the study show that for the development of a 15-ha landfill site in Malaysia with an estimated volume of 2,000,000 m(3), the capital investment required was about US 1,312,895 dollars, or about US 0.84 dollars/tonne of waste. Assuming that the lifespan of the landfill is 20 years, the total cost of operation was about US 11,132,536 dollars or US 7.15 dollars/tonne of waste. The closure cost of the landfill was estimated to be US 1,385,526 dollars or US 0.89 dollars/tonne of waste. Therefore, the total cost required to dispose of a tonne of waste at the semi-aerobic landfill was estimated to be US 8.89 dollars. By considering an average tipping fee of about US 7.89 dollars/tonne of waste in Malaysia in the first year, and an annual increase of 3% to about US 13.84 dollars in year-20, the overall system recorded a positive revenue of US 1,734,749 dollars. This is important information for the effort of privatisation of landfill sites in Malaysia, as well as in other developing countries, in order to secure efficient and effective landfill development and management.     

Assessment of benefits and risks of landfill materials for agriculture in Eritrea

In Eritrea, farmers have applied landfill materials as fertiliser to their fields for several decades. A sampling scheme in the landfill site of Asmara and selected farmers' fields was carried out to investigate the benefits and risks of using landfill materials for agriculture. Soil samples were collected from farmers' fields (7 samples) and from the Asmara landfill site (12 samples). The samples were analysed for major plant nutrients, heavy metals (Cd, Cr, Cu, Pb, Ni, Hg and Zn), and some physical properties. Nearly 65% (by weight) of the total landfill material mined from the landfill site constituted waste fractions of various substances. The remaining 35% was composed of soil-like materials, which are apparently used to fertilize agricultural soils. The average organic matter, total nitrogen, and available phosphorus contents of soils with landfill material measured 2.4%, 0.13%, and 45 mg kg(-1), respectively. However, soils without landfill material consisted of 1.1 % organic matter, 0.04% total N, and <40 mg kg(-1) of available P. Except for Hg, all the other heavy metals in the landfill site showed values above the permissible limits. In particular, the average concentrations of Cu (913 mg kg(-1)) and Pb (598 mg kg(-1)) in the landfill site were nine-fold and four-fold greater than the allowable limits, respectively. It is, therefore, suggested that composting fresh organic wastes should be considered and tested as an alternative material for fertilising agricultural soils and to maintain the quality of the environment.     

In situ nitrogen removal from leachate by bioreactor landfill with limited aeration

The feasibility of simultaneous nitrification and denitrification in a bioreactor landfill with limited aeration was assessed. Three column reactors, simulating bioreactor landfill operations under anaerobic condition (as reference), intermittent forced aeration and enhanced natural aeration were hence established, where aerated columns passed through two phases, i.e., fresh landfill and well-decomposed landfill. The experimental results show that limited aeration decreased nitrogen loadings of leachate distinctly in the fresh landfill. In the well-decomposed landfill, the NH(4)(+)-N of the input leachate could be nitrified completely in the aerated landfill columns. The nitrifying loadings of the column cross section reached 7.9 g N/m(2)d and 16.9 g N/m(2)d in the simulated landfill columns of intermittent forced aeration and enhanced natural aeration, respectively. The denitrification was influenced by oxygen distribution in the landfill column. Intermittent existence of oxygen in the landfill with the intermittent forced aeration was favorable to denitrify the NO(2)(-)-N and NO(3)(-)-N, indicated by the high denitrification efficiency (>99%) under the condition of BOD(5)/TN of more than 5.4 in leachate; locally persistent existence of oxygen in the landfill with enhanced natural aeration could limit the denitrification, indicated by relatively low denitrification efficiency of about 75% even when the BOD(5)/TN in leachate had an average of 7.1.     

The potential for aeration of MSW landfills to accelerate completion

Landfilling is a popular waste disposal method, but, as it is practised currently, it is fundamentally unsustainable. The low short-term financial costs belie the potential long-term environmental costs, and traditional landfill sites require long-term management in order to mitigate any possible environmental damage. Old landfill sites might require aftercare for decades or even centuries, and in some cases remediation may be necessary. Biological stabilisation of a landfill is the key issue; completion criteria provide a yardstick by which the success of any new technology may be measured. In order for a site to achieve completion it must pose no risk to human health or the environment, meaning that attenuation of any emissions from the site must occur within the local environment without causing harm. Remediation of old landfill sites by aerating the waste has been undertaken in Germany, the United States, Italy and The Netherlands, with considerable success. At a pilot scale, aeration has also been used in newly emplaced waste to accelerate stabilisation. This paper reviews the use of aerobic landfill worldwide, and assesses the ways in which the use of aerobic landfill techniques can decrease the risks associated with current landfill practices, making landfill a more sustainable waste disposal option. It focuses on assessing ways to utilise aeration to enhance stabilisation. The results demonstrated that aeration of old landfill sites may be an efficient and cost-effective method of remediation and allow the date of completion to be brought forward by decades. Similarly, aeration of newly emplaced waste can be effective in enhancing degradation, assisting with completion and reducing environmental risks. However, further research is required to establish what procedure for adding air to a landfill would be most suitable for the UK and to investigate new risks that may arise, such as the possible emission of non-methane organic compounds.     

Passive drainage and biofiltration of landfill gas: results of Australian field trial

A field scale trial was undertaken at a landfill site in Sydney, Australia (2004-2008), to investigate passive drainage and biofiltration of landfill gas as a means of managing landfill gas emissions from low to moderate gas generation landfill sites. The objective of the trial was to evaluate the effectiveness of a passive landfill gas drainage and biofiltration system at treating landfill gas under field conditions, and to identify and evaluate the factors that affect the behaviour and performance of the system.The trial results showed that passively aerated biofilters operating in a temperate climate can effectively oxidise methane in landfill gas, and demonstrated that maximum methane oxidation efficiencies greater than 90% and average oxidation efficiencies greater than 50% were achieved over the 4 years of operation. The trial results also showed that landfill gas loading was the primary factor that determined the behaviour and performance of the passively aerated biofilters. The landfill gas loading rate was found to control the diffusion of atmospheric oxygen into the biofilter media, limiting the microbial methane oxidation process. The temperature and moisture conditions within the biofilter were found to be affected by local climatic conditions and were also found to affect the behaviour and performance of the biofilter, but to a lesser degree than the landfill gas loading.     

Consequences of raising the height of a landfill in a water-deficient climate

A large-scale field experiment has been carried out at the Coastal Park landfill which serves the City of Cape Town, South Africa. The landfill is unlined, and the City Council was under pressure from the central Government to cap and close the existing landfill and to establish an extension to the landfill with a lining to prevent the escape of leachate into the ground water. Measuring cells, installed to measure the rate of leachate flow from the landfill had shown that over a period of 9 years, from 1987 to 1995, leachate flow had averaged only 2% of rainfall. It therefore appeared possible, by increasing the moisture absorption capacity of the landfill, i.e., by increasing its height, to stop the leachate flow completely. If this could be achieved, there would be no need for a lining, and the raising would considerably extend the life of the landfill.The paper describes the experiment and its results, including the effects of the raising on leachate flow, settlement, leachate quality and the potential for polluting ground water, and the landfill’s water balance.     

Tree establishment and growth at Pitsea landfill site,Essex, U.K.

Investigations at an 11-year-old landfill site have shown that soil moisture was positively, and soil oxygen was negatively correlated with temperature and concentration of soil methane generated by decomposition of the underlying landfill materials. A thin (0.2 m) cover of soil-forming material over the landfill showed acute oxygen deficiency and high temperatures. The high moisture content of this cover was probably caused by upward movement of water from within the landfill across a temperature gradient. Nearly all the trees of five species on the thinnest (0.2 m) cover died, but survival and growth was markedly improved on 1.5 m additional clay cover over the landfill. This material prevented landfill gas contamination, and also contained sufficient plant-available soil moisture to negate the large soil moisture deficits the area experiences in most summers. The evidence presented shows that landfill sites are dynamic in the distribution of landfill temperature and gas emissions and the planning of tree planting schemes should take this into account.     

Landfill reduction experience in The Netherlands

Modern waste legislation aims at resource efficiency and landfill reduction. This paper analyses more than 20 years of landfill reduction in the Netherlands. The combination of landfill regulations, landfill tax and landfill bans resulted in the desired landfill reduction, but also had negative effects. A fierce competition developed over the remaining waste to be landfilled. In 2013 the Dutch landfill industry generated €40 million of annual revenue, had €58 million annual costs and therefore incurred an annual loss of €18 million. It is not an attractive option to prematurely end business. There is a risk that Dutch landfill operators will not be able to fulfil the financial obligations for closure and aftercare. Contrary to the polluter pays principle the burden may end up with society. EU regulations prohibiting export of waste for disposal are in place. Strong differentials in landfill tax rate between nations have nevertheless resulted in transboundary shipment of waste and in non-compliance with the self-sufficiency and proximity principles. During the transformation from a disposal society to a recycling society, it is important to carefully plan required capacity and to guide the reorganisation of the landfill sector. At some point, it is no longer profitable to provide landfill services. It may be necessary for public organisations or the state to take responsibility for the continued operation of a ‘safety net’ in waste management. Regulations have created a financial incentive to pass on the burden of monitoring and controlling the impact of waste to future generations. To prevent this, it is necessary to revise regulations on aftercare and create incentives to actively stabilise landfills.     

Trends in the use of Fenton,electro-Fenton and photo-Fenton for the treatment of landfill leachate

Advanced oxidation processes (AOPs) such as Fenton, electro-Fenton and photo-Fenton have been applied effectively to remove refractory organics from landfill leachate. The Fenton reaction is based on the addition of hydrogen peroxide to the wastewater or leachate in the presence of ferrous salt as a catalyst. The use of this technique has proved to be one of the best compromises for landfill leachate treatment because of its environmental and economical advantages. Fenton process has been used successfully to mineralize wide range of organic constituents present in landfill leachate particularly those recalcitrant to biological degradation. The present study reviews the use of Fenton and related processes in terms of their increased application to landfill leachate. The effects of various operating parameters and their optimum ranges for maximum COD and color removal are reviewed with the conclusion that the Fenton and related processes are effective and competitive with other technologies for degradation of both raw and pre-treated landfill leachate.     

Landfill leachate affects metabolic responses of Zea mays L. seedlings

With an increasing focus on phyto-remediation options for landfill leachate, it is important to understand the responses of plant systems to landfill leachate stress. It is especially important to study the tolerant mechanisms of plant systems. We investigated several physiological changes of Zea mays L. (maize) in response to landfill leachate. Specifically, we investigated growth, chlorophyll content, lipid peroxidation, protein oxidation and activities of antioxidant enzymes. The results indicate that landfill leachate affected the growth and chlorophyll level of maize seedlings. Furthermore, landfill leachate elevated the levels of lipid peroxidation and protein oxidation in leaf tissues in a time-dependent manner, accompanied by the changes in antioxidant status. The physiological responses varied as a function of leachate concentration, and the growth inhibition, chlorophyll content inhibition and oxidative stress occurred after the exposure of higher concentrations of leachate. Higher concentrations of landfill leachate contained higher levels of pollutants. Our results indicate that landfill leachate affected the metabolic responses of plant systems. The risk of pollution occurred mainly in samples of higher concentration. Therefore, the critical aspect of phyto-remediation for landfill leachate is controlling its concentration. In doing so, plant systems may be able to tolerate the environmental stress of landfill leachate.     

Findings from long-term monitoring studies at MSW landfill facilities with leachate recirculation

This paper presents findings from long-term monitoring studies performed at full-scale municipal solid waste landfill facilities with leachate recirculation. Data from two facilities at a landfill site in Delaware, USA were evaluated as part of this study: (1) Area A/B landfill cells; and (2) two test cells (one with leachate recirculation and one control cell). Data from Area A/B were compared with proposed waste stability criteria for leachate quality, landfill gas production, and landfill settlement. Data from the test cells were directly compared with each other. Overall, the trends at Area A/B pointed to the positive effects (i.e., more rapid waste degradation) that may be realized through increasing moisture availability in a landfill relative to the reported behavior of more traditionally operated (i.e., drier) landfills. Some significant behavioral differences between the two test cells were evident, including dissimilarities in total landfill gas production quantity and the extent of waste degradation observed in recovered time capsules. Differences in leachate quality were not as dramatic as anticipated, probably because the efficiency of the leachate recirculation system at distributing leachate throughout the waste body in the recirculation cell was low.     

Quantification of landfill emissions to air: a case study of the Ano Liosia landfill site in the greater Athens area.

Fugitive pollutant emissions from municipal solid waste landfills have the potential to cause annoyance and health impacts in the surrounding residential areas. The overall objective of this research was to perform an assessment of fugitive pollutant emissions and a dispersion analysis downwind of a specific landfill site. The study was performed at the closed Ano Liosia landfill site which is located in the greater Athens area. The human exposure from priority to health-risk pollutants emitted from landfill, such as vinyl chloride and benzene, was estimated by the landfill gas emission LandGEM 2.01 software combined with the atmospheric long-term dispersion model ISC3-LT. The emission and meteorological conditions under which the models were applied referred to the worst-case scenario. This scenario was used for the evaluation of the maximum human exposure assessed beyond the Ano Liosia landfill towards the residential areas. The above scenario provides the minimum downwind distance of the health-risk zone which is calculated to be equal to 1.5 km from the landfill. Within this distance the assessed air pollutant concentration for several air pollutants was significantly above the World Health Organization reference lifetime exposure health criteria. Finally, the applied methodology was used in the Ano Liosia landfill, where atmospheric concentrations of pollutants measured in the field were compared with model predictions.     

Landfill aeration in the framework of a reclamation project in Northern Italy

In situ aeration by means of the Airflow technology was proposed for landfill conditioning before landfill mining in the framework of a reclamation project in Northern Italy. A 1-year aeration project was carried out on part of the landfill with the objective of evaluating the effectiveness of the Airflow technology for landfill aerobization, the evolution of waste biological stability during aeration and the effects on leachate and biogas quality and emissions.The main outcomes of the 1-year aeration project are presented in the paper.The beneficial effect of the aeration on waste biological stability was clear (63% reduction of the respiration index); however, the effectiveness of aeration on the lower part of the landfill is questionable, due to the limited potential for air migration into the leachate saturated layers.During the 1-year in situ aeration project approx. 275 MgC were discharged from the landfill body with the extracted gas, corresponding to 4.6 gC/kgDM. However, due to the presence of anaerobic niches in the aerated landfill, approx. 46% of this amount was extracted as CH₄, which is higher than reported in other aeration projects. The O₂ conversion quota was lower than reported in other similar projects, mainly due to the higher air flow rates applied.The results obtained enabled valuable recommendations to be made for the subsequent application of the Airflow technology to the whole landfill.