Measurements of summer radon and its progeny concentrations along with environmental gamma dose rates in Taiwan

The concentrations of 222Rn (radon) and its progeny with surrounding environmental gamma-dose rates were measured simultaneously inside and outside of buildings at 10 locations around Taipei and Hualien in Taiwan. For summer radon in Taiwan, indoor concentrations were estimated to be about 20 Bq m(-3) with about 90 nSv h- of environmental gamma, and outdoors, about 10 Bq m(-3) with about 70 nSv h(-1). The equilibrium factors were calculated to be 0.2-0.3 indoors and 0.3-0.4 outdoors. Indoor radon concentration had a weak positive correlation with gamma-dose rate. Since there is a possibility that high radon concentrations exist indoors during the cool season in Taiwan because of extremely low ventilation rates in the dwellings, a winter survey in January through February will be needed for future estimation of the annual effective dose.     

Radon-222 in Brazil: an outline of indoor and outdoor measurements

This study discusses the methodology for measuring and assessing the radon concentration in indoor and outdoor environments. A research study was developed to investigate the long-term behavior of the diurnal and seasonal fluctuations of radon (222)Rn EEC (Equilibrium-Equivalent Concentration) and the influence of temperature and other climatic aspects on this behavior. The study was performed by means of both integrated and instantaneous measurements of radon and its short-lived daughter products for a period of 1 year in an indoor environment in Rio de Janeiro city, Brazil (reference environment), with continuous measurement, using a radon monitor with an alpha spectrometry detector.For a single day, a variability of about 50% could be observed in the (222)Rn EEC values measured on a hourly basis, with a maximum occurring early in the morning and a minimum in the afternoon. For the long-term period, seasonality is responsible for a two order of magnitude variability, with a maximum of 50 Bq.m(-3) in winter (dry season) and a minimum of 0.5 Bq.m(-3) in the summer months (wet season), outdoors. A negative correlation with temperature was observed. The conclusions of this experiment led to a survey of radon gas concentration in dwellings in Rio de Janeiro city, Brazil, in urban area with nearly 7 million inhabitants, through integrated sampling methods, using a Solid State Nuclear Track Detectors Technique (SSNTD). The study was conducted in different geomorphological locations in town. The radon gas concentration in Rio de Janeiro dwellings ranged from 5 Bq.m(-3) to 200 Bq.m(-3). A good correlation between indoor radon gas concentration and location of dwellings was observed. The seashore areas presented the lowest levels of indoor radon concentration, whereas the highest levels were found close to the mountains.     

Seasonal variations of 222Rn concentrations in the air of a tunnel located in Nagano city

The seasonal variation of 222Rn concentrations in the air of tunnels constructed during World War II at Nagano City has been investigated. The determination of 222Rn concentrations in tunnel air was performed using a solid-state nuclear track detector technique. The monthly radon concentrations changed smoothly, decreasing towards winter and increasing towards summer, and it was found that the concentrations strongly correlate with the temperature difference between the inside and the outside of the tunnel. In the innermost areas of the tunnel, the maximum concentration was observed in July, its value being about 6500 Bq m (-3). The concentrations of radon in the tunnel air decrease exponentially towards the openings of the tunnel, which indicates that the radon concentration in the tunnel is basically governed by diffusion and mixing of radon gas with air. These observations lead to the conclusion that the seasonal variation of the radon concentration in the tunnel air is mainly caused by a convection current due to a stack effect induced by the temperature difference between the tunnel air and the outside air.     

Seasonal variations of Rn concentrations in the air of a tunnel located in Nagano city

The seasonal variation of 222Rn concentrations in the air of tunnels constructed during World War II at Nagano City has been investigated. The determination of 222Rn concentrations in tunnel air was performed using a solid-state nuclear track detector technique. The monthly radon concentrations changed smoothly, decreasing towards winter and increasing towards summer, and it was found that the concentrations strongly correlate with the temperature difference between the inside and the outside of the tunnel. In the innermost areas of the tunnel, the maximum concentration was observed in July, its value being about 6500 Bq m (-3). The concentrations of radon in the tunnel air decrease exponentially towards the openings of the tunnel, which indicates that the radon concentration in the tunnel is basically governed by diffusion and mixing of radon gas with air. These observations lead to the conclusion that the seasonal variation of the radon concentration in the tunnel air is mainly caused by a convection current due to a stack effect induced by the temperature difference between the tunnel air and the outside air.     

Seasonal variations of aerosol residence time in the lower atmospheric boundary layer

During a one year period, from Jan. 2002 up to Dec. 2002, approximately 130 air samples were analyzed to determine the atmospheric air activity concentrations of short- and long-lived (222Rn) decay products 214Pb and 210Pb. The samples were taken by using a single-filter technique and gamma-spectrometry was applied to determine the activity concentrations. A seasonal fluctuation in the concentration of 214Pb and 210Pb in surface air was observed. The activity concentrations of both radionuclides were observed to be relatively higher during the winter/autumn season than in spring/summer season. The mean activity concentration of 214Pb and 210Pb within the whole year was found to be 1.4+/-0.27 Bq m(-3) and 1.2+/-0.15 mBq m(-3), respectively. Different 210Pb:214Pb activity ratios during the year varied between 1.78 x 10(-4) and 1.6 x 10(-3) with a mean value of 8.9 x 10(-4) +/- 7.6 x 10(-5). From the ratio between the activity concentrations of the radon decay products 214Pb and 210Pb a mean residence time (MRT) of aerosol particles in the atmosphere of about 10.5+/-0.91 d could be estimated. The seasonal variation pattern shows relatively higher values of MRT in spring/summer season than in winter/autumn season. The MRT data together with relative humidity (RH), air temperature (T) and wind speed (WS), were used for a comprehensive regression analysis of its seasonal variation in the atmospheric air.     

Low-infiltration housing in Rochester, New York: A study of air-exchange rates and indoor air quality

A sample of 58 occupied homes in Rochester, NY, most of which incorporated special builder-designed weatherization components, were studied to assess (1) the effectiveness of construction techniques designed to reduce air leakage; (2) the indoor air quality and air-exchange rates in selected airtight houses, and (3) the impact on indoor air quality of mechanical ventilation systems employing air-to-air heat exchangers. The “specific leakage area” was measured in each house using the fan pressurization technique. Houses built with polyethylene vapor barriers and joint-sealing were as a group 50% tighter than a similar group of houses without such components. Mechanical ventilation systems with air-to-air heat exchangers were installed in nine relatively airtight houses, some of which had gas stoves and/or tobacco smoking occupants. Air-exchange rates and indoor concentrations of radon (Rn), formaldehyde (HCHO), nitrogen dioxide (NO₂), and humidity were measured in each house for 1-week periods with and without mechanical ventilation. More detailed measurements, including concentrations of carbon monoxide and inhalable particulates, were made in two of these houses by a mobile laboratory. In all nine houses, air-exchange rates were relatively low (0.2–0.5 ach) without mechanical ventilation, and yet indoor concentrations of Rn, HCHO, and NO₂ were below existing guidelines. Mechanical ventilation systems were effective in further reducing indoor contaminant concentrations. We conclude that when contaminant source strengths are low, acceptable indoor air quality can be compatible with low air-exchange rates.     

A survey of radon level in underground buildings in China

From 2003-2004, using solid state nuclear detectors, a survey of the air radon level in 234 underground buildings in 23 cities of China was carried out during spring as well as summer and winter. The annual radon concentrations in these underground buildings range from 14.9 to 2482 Bq m(-3), with an overall mean value of 247 Bqm(-3). When radon concentrations are averaged according to cities, Fuzhou and Baotou have the relatively higher radon levels, which are 714 and 705 Bqm(-3), respectively. Guangzhou and Shanghai have the relatively lower radon levels with 71.1 and 72.6 Bqm(-3). The annual effective dose by exposure to radon received by people working in these cities is concluded to be 1.6 mSv. The geological formation, coating level, decorating materials and ventilation situation all affect the radon concentration in underground buildings. The radon level in underground buildings has the lowest value in winter and the highest value in summer.     

Variations of airborne and waterborne Rn-222 in houses in Maine

Concentrations of airborne radon ranging from 0.05 to 135 pCi/L were found in houses in Maine. Tracketch cups were placed in five positions for 100 houses to determine integrated average radon concentrations over the period October 1980–May 1981. To investigate the association between elevated radon concentrations in well water and the indoor airborne radon concentrations, the radon in the water supplies of these houses was measured by liquid scintillation. Monitors of airborne radon, recording in intervals of 10 min for periods of 5–7 days, were used for dynamic studies in 18 houses, determining the component of airborne radon associated with major water uses, such as showers, laundry, and dishwashing, which liberate radon in bursts. House residents kept logs noting the time of major water uses. For some of the houses, ventilation rates ranging from 0.3 to 2 air changes per hour were determined by analysis of the dynamic data. The component of airborne radon associated with water sources was found to vary inversely with ventilation rate and directly with waterborne radon concentration, with 0.8 ± 0.2 pCi Rn/L air per nCi Rn/L water at a ventilation rate of 1.0 air change per hour. The data are pertinent to a study which has revealed significant correlations between county averages, from the National Cancer Institute, or age-adjusted cancer mortality rates in Maine and average values of radon concentrations in water for the counties.     

Investigations on indoor radon in Austria, Part 1: Seasonality of indoor radon concentration

In general, indoor radon concentration is subject to seasonal variability. The reasons are to be found (1) in meteorological influence on the transport properties of soil, e.g. through temperature, frozen soil layers and soil water saturation; and (2) in living habits, e.g. the tendency to open windows in summer and keep them closed in winter, which in general leads to higher accumulation of geogenic Rn in closed rooms in winter. If one wants to standardize indoor Rn measurements originally performed at different times of the year, e.g. in order to make them comparable, some correction transform as a function of measurement time which accounts for these effects must be estimated. In this paper, the seasonality of indoor Rn concentration measured in Austria is investigated as a function of other factors that influence indoor Rn. Indoor radon concentration is clearly shown to have seasonal variability, with higher Rn levels in winter. However, it is complicated to quantify the effect because, as a consequence of the history of an Rn survey, the measurement season maybe correlated to geological regions, which may introduce a bias in the estimate of the seasonality amplitude.     

A nationwide survey of outdoor radon concentration in Japan

Nationwide outdoor radon (222Rn) concentrations in Japan were measured to survey the environmental outdoor 222Rn level and to estimate the effective dose to the general public from 222Rn and its progeny. The 222Rn concentration was measured with a passive-type radon monitor. The 222Rn monitors were installed at about 700 points throughout Japan from 1997 to 1999. The annual mean 222Rn concentration in Japan was estimated from four quarters measurements of 47 prefectures in Japan. Nationwide outdoor mean 222Rn concentration was 6.1 Bq m(-3). This was about 40% of the indoor 222Rn concentration in Japan. The 222Rn concentration in Japan ranged from 3.3 Bq m(-3) in the Okinawa region to 9.8 Bq m(-3) in the Chugoku region, reflecting geological characteristics. Seasonal variation of outdoor 222Rn concentration was also found to be lowest in July to September, and highest in October to December. From the results of this 222Rn survey and previous indoor 222Rn survey program, the effective dose to the general public from 222Rn and its progeny was estimated to be 0.45 mSv y(-1).     

Seasonal variations of natural ventilation and radon-222 exhalation in a slightly rising dead-end tunnel

The concentration activity of radon-222 has been monitored, with some interruptions, from 1997 to 2005 in the end section of a slightly rising, dead-end, 38-m long tunnel located in the Phulchoki hill, near Kathmandu, Nepal. While a high concentration varying from 6 x 10(3) Bq m(-3) to 10 x 10(3) Bq m(-3) is observed from May to September (rainy summer season), the concentration remains at a low level of about 200 Bq m(-3) from October to March (dry winter season). This reduction of radon concentration is associated with natural ventilation of the tunnel, which, contrary to expectations for a rising tunnel, takes place mainly from October to March when the outside air temperature drops below the average tunnel temperature. This interpretation is supported by temperature measurements in the atmosphere of the tunnel, a few meters away from the entrance. The temporal variations of the diurnal amplitude of this temperature indeed follow the ventilation rate deduced from the radon measurements. In the absence of significant ventilation (summer season), the radon exhalation flux at the rock surface into the tunnel atmosphere can be inferred; it exhibits a yearly variation with additional transient reductions associated with heavy rainfall, likely to be due to water infiltration. No effect of atmospheric pressure variations on the radon concentration is observed in this tunnel. This experiment illustrates how small differences in the location and geometry of a tunnel can lead to vastly different behaviours of the radon concentration versus time. This observation has consequences for the estimation of the dose rate and the practicability of radon monitoring for tectonic purposes in underground environments.     

Indoor radon (222Rn) concentration measurements in Cyprus using high-sensitivity portable detectors

Using high-sensitivity radon ((222)Rn) portable detectors (passive electronic devices of the type RADIM3), the airborne (222)Rn concentration in the interior of various Cypriot buildings and dwellings was measured. For each preselected building and dwelling, a calibrated detector was put into a closed room, and the (222)Rn concentration was registered in sampling intervals of 2 to 4 h for a total counting time of typically 48 h. (222)Rn activity concentrations were found to be in the range of 6.2 to 102.8 Bq m(-3), with an overall arithmetic mean value of (19.3+/-14.7) Bq m(-3). This value is by a factor of two below the world average (population-weighted) value of 39 Bq m(-3). The total annual effective dose equivalent to the Cypriot population was calculated to be between 0.16 and 2.6 mSv with an overall arithmetic mean value of (0.49+/-0.37) mSv.     

Spatial and time variations of radon-222 concentration in the atmosphere of a dead-end horizontal tunnel

The concentration of radon-222 has been monitored since 1995 in the atmosphere of a 2 m transverse dimension, 128 m long, dead-end horizontal tunnel located in the French Alps, at an altitude of 1600 m. Most of the time, the radon concentration is stable, with an average value ranging from 200 Bq m(-3) near the entrance to about 1000 Bq m(-3) in the most confined section, with an equilibrium factor between radon and its short-lived decay products varying from 0.61 to 0.78. However, radon bursts are repeatedly observed, with amplitudes reaching up to 36 x 10(3) Bq m(-3) and durations varying from one to several weeks, with similar spatial variations along the tunnel as the background concentration. These spatial variations are qualitatively interpreted in terms of natural ventilation. Comparing the radon background concentration with the measured radon exhalation flux at the wall yields an estimate of 8+/-2 x 10(-6) s(-1) (0.03+/-0.007 h(-1)) for the ventilation rate. The hypothesis that the bursts could be due to transient changes in ventilation can be ruled out. Thus, the bursts are the results of transient increased radon exhalation at the walls, that could be due to meteorological effects or possibly combined hydrological and mechanical forcing associated with the water level variations of the nearby Roselend reservoir lake. Such studies are of interest for radiation protection in poorly ventilated underground settings, and, ultimately, for a better understanding of radon exhalation associated with tectonic or volcanic processes.     

Analysis of temperature influences on the amplitude-frequency characteristics of Rn gas concentration

The ventilation mechanism of Rn gas in underground environments is considered. Ventilation plays an important role in influencing the variability (harmonics) of Rn gas in the porous space below the earth's surface. We propose a new physical-environmental model of relating Rn gas concentrations to air temperature variations at the earth's surface. Applicability of this model was tested after searching for Rn gas indicators of geodynamic processes in two underground tunnels in central and southern Israel. The theoretical estimation of Rn gas concentrations shows a good agreement with the observed values. We demonstrate the possibility of Rn gas anomalies being caused by atmospheric temperature variations and the necessity to take these effects into account when investigating geodynamic processes.     

Monitoring and modelling of indoor radon concentrations in a multi-storey building at Mumbai,India

Radon (Rn(222)) levels in an indoor atmosphere of a multi-storey building at Mumbai have been measured for one year covering all the four seasons. Monitoring was carried out using the time-integrated passive detector technique, using Kodak-115 type Solid State Nuclear Track Detector (SSNTD) films of 2.5x2.5 cm size. Measured indoor radon levels showed a decreasing trend with height with concentration ranging from 41 Bq m(-3) at ground floor level to 15 Bq m(-3) at 19th floor level. Using the dose conversion factors, the inhalation dose due to breathing of radon gas is estimated to be 1.03 mSv y(-1) at the ground floor to 0.38 mSv y(-1) at the 19th floor level. Measured indoor radon concentrations on each floor were compared with the computed values using a mathematical model. The agreement between measured values and calculated values of indoor concentrations at different floors was very good within the limitations of various field parameter values.     

Estimating the amount and distribution of radon flux density from the soil surface in China

Based on an idealized model, both the annual and the seasonal radon ((222)Rn) flux densities from the soil surface at 1099 sites in China were estimated by linking a database of soil (226)Ra content and a global ecosystems database. Digital maps of the (222)Rn flux density in China were constructed in a spatial resolution of 25 km x 25 km by interpolation among the estimated data. An area-weighted annual average (222)Rn flux density from the soil surface across China was estimated to be 29.7+/-9.4 mBq m(-2)s(-1). Both regional and seasonal variations in the (222)Rn flux densities are significant in China. Annual average flux densities in the southeastern and northwestern China are generally higher than those in other regions of China, because of high soil (226)Ra content in the southeastern area and high soil aridity in the northwestern one. The seasonal average flux density is generally higher in summer/spring than winter, since relatively higher soil temperature and lower soil water saturation in summer/spring than other seasons are common in China.     

A survey of indoor workplace radon concentration in Japan

Radon ((222)Rn) concentration was measured at indoor workplaces in Japan to estimate effective dose to the public from (222)Rn and its progeny. Measurements were made from 2000 to 2003 at 705 sites in four categories of office, factory, school and hospital. Passive type Rn monitors equipped with two sheets of polycarbonate thin films for measuring radon concentrations were installed at observation sites and replaced every 3 months to observe seasonal variations in (222)Rn concentrations. The range of annual mean (222)Rn concentrations for all sites was 1.4-182 Bq m(-3), with the arithmetic mean and standard deviation were 20.8 and 19.5 Bq m(-3). Annual mean (222)Rn concentration observed at office, factory, school and hospital were 22.6, 10.1, 28.4 and 19.8 Bq m(-3), respectively. Seasonal variations in (222)Rn concentrations at offices, schools and hospitals were similar to those found in dwellings, and variations in factories were similar to those found in outdoor environments. (222)Rn concentration observed in every quarter period was found to decrease as follows: school>office>hospital>factory. The average effective dose to the public due to (222)Rn was estimated to be 0.41 mSv y(-1) weighted by the working population. Considering the (222)Rn exposure in indoor workplaces, effective dose to the general public is estimated to be in the range from approximately 0.42 to 0.52 mSv y(-1).     

Contribution of (222)Rn-bearing water to the occupational exposure in thermal baths

The present study investigates the short- and long-term effects of radon ((222)Rn) released from water on the progeny exposure in a thermal spa. For the purposes of this work, the Polichnitos spa was used as a case study. The bathroom was supplied with water containing 110-210 kBq m(-3) of (222)Rn. The (222)Rn concentration in air and the short-lived (222)Rn progenies in attached and unattached form were monitored into the bathroom and the surrounding premises. The equilibrium factor (F-factor) and the unattached fraction were estimated. The results of this study show that water flow during bath filling is by far the dominant mechanism by which (222)Rn is released in the air of the bathroom. The progeny exposure was correlated linearly with the (222)Rn concentration in the entering water. The annual effective dose received by a worker was found to be below the lower limit value of 3 mSv recommended by ICRP 65. The dose limit was exceeded only for water containing more than 300 kBq m(-3).     

Spatiotemporal variation of radon and carbon dioxide concentrations in an underground quarry: coupled processes of natural ventilation, barometric pumping and internal mixing

Radon-222 and carbon dioxide concentrations have been measured during several years at several points in the atmosphere of an underground limestone quarry located at a depth of 18 m in Vincennes, near Paris, France. Both concentrations showed a seasonal cycle. Radon concentration varied from 1200 to 2000 Bq m⁻³ in summer to about 800-1400 Bq m⁻³ in winter, indicating winter ventilation rates varying from 0.6 to 2.5 × 10⁻⁶ s⁻¹. Carbon dioxide concentration varied from 0.9 to 1.0% in summer, to about 0.1-0.3% in winter. Radon concentration can be corrected for natural ventilation using temperature measurements. The obtained model also accounts for the measured seasonal variation of carbon dioxide. After correction, radon concentrations still exhibit significant temporal variation, mostly associated with the variation of atmospheric pressure, with coupling coefficients varying from −7 to −26 Bq m⁻³ hPa⁻¹. This variation can be accounted for using a barometric pumping model, coupled with natural ventilation in winter, and including internal mixing as well. After correction, radon concentrations exhibit residual temporal variation, poorly correlated between different points, with standard deviations varying from 3 to 6%. This study shows that temporal variation of radon concentrations in underground cavities can be understood to a satisfactory level of detail using non-linear and time-dependent modelling. It is important to understand the temporal variation of radon concentrations and the limitations in their modelling to monitor the properties of natural or artificial underground settings, and to be able to assess the existence of new processes, for example associated with the preparatory phases of volcanic eruptions or earthquakes.     

Long period study of outdoor radon concentration in Milan and correlation between its temporal variations and dispersion properties of atmosphere

The results of a survey of outdoor radon concentrations in Milan are reported. Measurements were performed hourly over a continuous four year period from January 1997 to December 2000. Radon concentration was obtained by two means: both direct measurement of radon; and measurement of its decay products. The average daily pattern of radon concentration featured a minimum in the late afternoon and a maximum in the early hours of the morning. A seasonal pattern with higher concentrations in winter than in summer (from around 15 Bq m(-3) in winter to around 5 Bq m(-3) in summer) was also observed. Similar average annual values of around 10 Bq m(-3) were obtained. The annual effective outdoor radon dose was found to be 0.12 mSv. The variation from minimum in the afternoon to maximum the following morning was found to be a good indicator of the height of the nocturnal mixing layer. The variation between maximum and minimum levels on the same day is an index of the maximum height of the mixing layer. Furthermore, our long term measurements of radon have permitted us to examine the dispersion characteristics of the atmosphere over Milan, and to establish the frequency of conditions unfavourable to the dispersion of atmospheric pollutants.