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1.
Composting is a method for preparing organic fertilizers that represents a suitable management option for the recycling of two-phase olive mill waste (TPOMW) in agriculture. Four different composts were prepared by mixing TPOMW with different agro-industrial by-products (olive pruning, sheep manure and horse manure), which were used either as bulking agents or as N sources. The mature composts were added during six consecutive years to a typical “Picual” olive tree grove in the Jaén province (Spain). The effects of compost addition on soil characteristics, crop yield and nutritional status and also the quality of the olive oil were evaluated at the end of the experiment and compared to a control treated only with mineral fertilization. The most important effects on soil characteristics included a significant increase in the availability of N, P, K and an increase of soil organic matter content. The application of TPOMW compost produced a significant increase in olive oil content in the fruit. The compost amended plots had a 15% higher olive oil content than those treatment with inorganic fertilization. These organics amendments maintained the composition and quality of the olive oil.  相似文献   

2.
The co-composting of solid residue from olive oil production process, exhausted olive cake (EOC), with poultry manure (PM) watered with olive mill wastewater (OMW) was considered as an efficient method for the treatment of olive oil extraction effluent having high organic content including phenolic polluting compounds. The process was carried out by using three aerated windrows of variable compositions. OMW was used continuously during the bio-oxidative period, which lasted three months, to replace water for windrow moistening. The main process parameters (temperature, pH, humidity and C/N) were monitored over four months to ascertain the maturity of the compost. The composting process lasted four months during which 26 moistenings of the mixtures were performed with OMW or water to keep moisture within the ideal range of 45-60% (w/w). At the maturity stage, the C/N ratios were less than 16, pH of the resulting products were slightly alkaline (pH=8) and electrical conductivity was relatively high in the OMW mixtures (5.46-5.48 Sm(-1)) when compared with water application. Nitrates increased (0.16-0.42%) and phenol contents were reduced by more than 49%. Mature composts were then used as an amendment for potato production in a field where no inhibitory effect was observed. Potato productivity increased 10-23% as a result of compost application. No noticeable negative impact of OMW on the soil system was observed. Phenolic compound concentrations in the stabilised composts were comparable in the three studied mixtures (different sites) and averaged 0.24%. Considering previous results and this three year study, it has been observed that the benefit of these composts demonstrated the potential sustainable agronomic production of potato while using locally available recycled organic materials.  相似文献   

3.
The influence of bulking agents on organic matter (OM) stability and nitrogen (N) availability in sewage sludge composts was investigated. The same sludge was composted on an industrial plant with different mixtures of bulking agents. The composting process included an active phase and a curing phase, both lasting 6 weeks, separated by the screening of composts. The OM evolution was characterised by carbon (C) and N mass balances in biochemical fractions. The OM stability and N potential availability of final composts were measured during soil incubations. During composting, the C and N losses reached more than 62% of the initial C and more than 45% of the initial N, respectively, due to C mineralisation or N volatilisation and screening. The bulking materials mostly influenced OM evolution during the active phase. They contributed to the mitigation of N losses during the active phase where N immobilisation through active microbial activity was favoured by bulking agents increasing the C:N ratio of the initial mixtures. However, the influence of bulking agents on OM evolution was removed by the screening; this induced the homogenisation of compost characteristics and led to the production of sludge composts with similar organic matter characteristics, C degradability and N availability.  相似文献   

4.
One of the main disadvantages in the composting of two-phase olive mill wastes (TPOMW) is the long time required for its transformation (up to 40 weeks). The aim of this work was to evaluate the relationship between the degradation of the lignocellulosic fraction of TPOMW and the organic matter (OM) mineralisation rate in four composting piles prepared with different bulking agents and N-sources used to enhance OM degradation. The kinetics of degradation of the lignocellulosic fraction was compared to conventional maturation and stability indices to evaluate its impact on the duration of the composting process. The composition of bulking agents mainly affected the water-soluble fraction which influenced the OM degradation rate (linear or exponential OM degradation pattern) at early stages of the composting process but it neither modified the duration of the process (between 34 and 36 weeks) nor the total OM degradation underwent by the piles. The high initial mineral N availability was a key factor to significantly enhanced microbial activity. The mixture with urea as N-source registered the most efficient degradation of hemicellulose, cellulose and lignin, reducing the thermophilic phase and the total duration of TPOMW composting.  相似文献   

5.
This paper describes experiments that demonstrate the effects and potential for remediation of a former steelworks site in Wales polluted with polycyclic aromatic hydrocarbons (PAHs) and volatile organic compounds (VOCs). Under field conditions, PAH-contaminated soil was composted in-vessel, with or without organic feedstocks, receiving forced aeration for 80 days followed by 4 months maturation. Treatments compared PAH removal in contaminated soil to contaminated soil mixed with three different organic waste mixes after composting and after composts were spread to land. After composting, PAH concentrations declined in all treatments, by up to 38%. Sixteen months after the composts were landspread and vegetation was established, only those containing contaminated soil with organic additions exhibited further PAH removal, by up to 29%. Composting resulted in a decline in the relative concentration of small PAHs, whereas the landspreading-vegetation phase saw a decline in the relative concentration of medium PAHs in two of the three composts exhibiting PAH removal. Under controlled glasshouse conditions, vegetated soil columns of differing depths were exposed to VOCs from beneath. VOC vapour affected both shoot and root growth and soil microbial activity; effects varied with distance from the VOC source. This work demonstrated that on-site remediation of aged PAH-contaminated land can be successfully initiated by in-vessel co-composting followed by land spreading and vegetation, within a practical timeframe.  相似文献   

6.
Olive mill wastes represent an important environmental problem in Mediterranean areas where they are generated in huge quantities in short periods of time. Their high phenol, lipid and organic acid concentrations turn them into phytotoxic materials, but these wastes also contain valuable resources such as a large proportion of organic matter and a wide range of nutrients that could be recycled. In this article, recent research studies for the valorisation of olive mill wastes performed by several authors were reviewed: second oil extraction, combustion, gasification, anaerobic digestion, composting and solid fermentation are some of the methods proposed. Special attention was paid to the new solid waste generated during the extraction of olive oil by the two-phase system. The peculiar physicochemical properties of the new solid waste, called two-phase olive mill waste, caused specific management problems in the olive mills that have led to the adaptation and transformation of the traditional valorisation strategies. The selection of the most suitable or appropriate valorisation strategy will depend on the social, agricultural or industrial environment of the olive mill. Although some methods are strongly consolidated in this sector, other options, more respectful with the environment, should also be considered.  相似文献   

7.
The TAO model of Transformation of Added Organic materials (AOM) calibrated on AOMs and substrates of temperate areas was used to assess the transformations in soil of carbon and nitrogen forms of AOMs: raw materials, selected mixtures and composts from Ouagadougou urban wastes. AOMs were studied in terms of chemical and biochemical contents and for their C and N mineralization during incubations in a typical Ferric Lixisol of the sub-urban agriculture of Ouagadougou. The TAO model was used to predict the transformations of C (very labile, resistant and stable organic C) and N (very labile, resistant and stable organic N, produced and immobilized inorganic N) forms driven by AOM biochemical data. Without any change in calibration formulae, TAO predicted accurately the C transformations and inorganic N production of most of the tested AOMs, with a tendency to slightly overestimate C mineralization of previously well-composted materials and re-mineralization of immobilized N. Complementary adjustments using more complete data from laboratory experiments are suggested, but the model agrees with other data collected in the field and appears as a promising tool to optimise the management of urban wastes in the tropical area as well as for agro industrial organic fertilizers of the temperate zone. This application suggests ways to improve the management of urban wastes aiming to optimize agricultural yields, system sustainability and C sequestration in soil.  相似文献   

8.
The effect of land application of biosolids on an agricultural soil was studied in a 2-month incubation experiment. The soil microbial biomass and the availability of heavy metals in the soil was monitored after the application of four different composting mixtures of sewage sludge and cotton waste, at different stages of composting. Land application caused an increase of both size and activity of soil microbial biomass that was related to the stabilization degree of the composting mixture. Sewage sludge stabilization through composting reduced the perturbance of the soil microbial biomass. At the end of the experiment, the size and the activity of the soil microbial biomass following the addition of untreated sewage sludge were twice those developed with mature compost. For the mature compost, the soil microbial biomass recovered its original equilibrium status (defined as the specific respiration activity, qCO2) after 18 days of incubation, whereas the soil amended with less stabilized materials did not recover equilibrium even after the two-month incubation period. The stabilization degree of the added materials did not affect the availability of Zn, Ni, Pb, Cu, Cr and Cd in the soil in the low heavy metal content of the sewage sludge studied. Stabilization of organic wastes before soil application is advisable for the lower perturbation of soil equilibria status and the more efficient C mineralization.  相似文献   

9.
Three sewage sludge composts were obtained from mixtures of an aerobic sludge (AS) and three organic wastes differing widely in chemical composition: an extremely biodegradable waste (municipal solid waste, MSW), a plant residue (grape debris) and a residue with a carbon fraction not easily mineralizable (peat residue). The following mixtures were made, the proportions referring to their total organic carbon content: AS-MSW 1/1, AS-GRAPE 3/1 and AS-PEAT 1/1. These mixtures were composted over 3 months in the open air with periodical turning, and were left to mature afterwards for 4 months. Uncomposted mixtures and composted mixtures, before and after maturation, were incubated for 38 days, under laboratory conditions, with a calcareous soil and the CO2 emission of the samples periodically measured.Uncomposted mixtures emitted much greater quantities of carbon than those composted, whether before or after maturation period. Both at the beginning and at the end of composting, differences were observed between the total amount of carbon emitted by the mixture containing peat waste and the others. However, the quantities of carbon emitted from the three mixtures tended to even out in mature composts, reaching a maximum of 600 mg carbon per 100 g total organic carbon. This shows that, although the mineralization of carbon depends on the nature of the organic waste mixed with the sewage sludge, it tends to even out when the mixtures have undergone composting.  相似文献   

10.
Changes in the chemical and chemical-structural composition of the organic matter of two different sewage sludges (aerobic and anaerobic) mixed with sawdust (1:1 and 1:3, v/v) during composting were determined by monitoring chemical and microbiological parameters as well as by pyrolysis-gas chromatography. Composting was carried out in periodically turned outdoor piles, which were sampled for analysis 1, 30, 60 and 90 days after the beginning of the composting process. Both volatile organic matter and the water soluble C fraction decreased during composting, indicating that the more labile C fractions are mineralized during the process. Microbial activity as measured by microbial respiration (CO(2) evolved from compost samples during incubation) also decreased with composting, reflecting the more stable character of the resulting compost. No major differences were observed between the four composts studied as regards their chemical-structural characteristics. The acetonitrile, acetic acid and phenol pyrolytic fragment tended to increase with composting. Although the final composts were more aromatic in nature than the starting materials, a low degree of humification was observed in all four composts studied, as determined by their high proportion of polysaccharides and alkyl compounds. For this reason, the relationship between pyrolytic fragments, such as benzene/toluene or benzene+toluene/pyrrol+phenols, which are used as indices of humification for soil organic matter, are not of use for such poorly evolved sludge composts; instead, ratios that involve carbohydrate derivatives and aromatic compounds, such as furfural+acetic/benzene+toluene or acetic/toluene, are more sensitive indices for reflecting the transformations of these materials during composting. Both the chemical and microbiological parameters and pyrolytic analysis provided valuable information concerning the nature of the compost's organic matter and its changes during the composting process.  相似文献   

11.
Several urban wastes of different nature and level of organic matter stability (municipal solid wastes, sewage sludges and composts) have been characterized analysing fertility and phytotoxicity parameters. Sewage sludges showed the highest N and P values of all the wastes. The total K content of the wastes was low but almost all was available to plants. Mature composts had the lowest organic carbon and humic substances values as a consequence of organic matter mineralization during the composting process. The soluble C at pH 2/precipitated C ratio decreased as the stability of the organic matter increased. In spite of the heterogeneity of the wastes analysed, the organic matter/total organic C ratio was largely constant with a mean value of 2.05. In no case did the heavy metal levels exceed the maximum allowed by the EU disposition for sewage sludges use in agriculture. The highest levels of phytotoxic substances occurred in the fresh wastes. The germination rates and root length were highest with mature composts. Germination index and root length were negatively correlated with water soluble carbon (WSC) and WSC/N ratio. The principal component analysis showed that extractable C, soluble C at pH 2 and water soluble C were the C fractions which most contributed to the total variability.  相似文献   

12.
A study was conducted to investigate physico-chemical properties, fertilizing potential and heavy metal polluting potentials of municipal solid waste composts produced in 29 cities of the country. Results indicated that except a very few samples, all other samples have normal pH and EC. Organic matter as well as major nutrients N and P contents in MSW composts are generally low as compared to the composts prepared from rural wastes. Heavy metal contents in composts from bigger cities (>1 million population) were higher by about 86% for Zn, 155% for Cu, 194% for Cd, 105% for Pb, 43% for Ni and 132% for Cr as compared to those from smaller cities (<1 million population). Composts prepared from source separated biogenos wastes contained, on average, higher organic matter (by 57%), total N (by 77%) and total P (by 78%), but lower concentrations of heavy metals Zn (by 63%), Cu (by 78%), Cd (by 64%), Pb (by 84%), Ni (by 50%), and Cr (by 63%) as compared to those prepared from mixed wastes. Partial segregation at the site of composting did not improve quality of compost significantly in terms of fertilizing parameters and heavy metal contents. Majority of MSW composts did not conform to the quality control guideline of ‘The Fertilizer (Control) Order 1985’ in respect of total organic C, total P, total K as well as heavy metals Cu, Pb and Cr. In order to enable the relevant stakeholders to judge overall quality, a scheme has been proposed for the categorization of composts into different marketable classes (A, B, C, and D) and restricted use classes (RU-1, RU-2, and RU-3) on the basis their fertilizing potential and as well as potential for contaminating soil and food chain. Under the scheme, ‘Fertilizing index’ was calculated from the values of total organic C, N, P, K, C/N ratio and stability parameter, and ‘Clean index’ was calculated from the contents of heavy metals, taking the relative importance of each of the parameters into consideration. As per the scheme, majority of the compost samples did not belong to any classes and hence, have been found unsuitable for any kind of use. As per the regulatory limits of different countries, very few compost samples (prepared from source separated biogenos wastes) were found in marketable classes (A, B, C and D) and some samples (11–14) were found suitable only for some restricted use.  相似文献   

13.
Organic wastes can be recycled as a source of plant nutrients, enhancing crop production by improving soil quality. However, the study of the dynamic of soil nutrient, especially the N dynamic, after soil application of any organic material is vital for assessing a correct and effective use of the material, minimizing the losses of nitrate in leachates and avoiding the negative environmental effects that it may cause in groundwater. To estimate the effect of three organic materials, a municipal solid waste compost (MWC), a non-composted paper mill sludge (PS), and an agroforest compost (AC) on the N dynamic of a sandy soil two experiments were carried out: an incubation experiment and a column experiment. The incubation experiment was conducted to estimate the N mineralization rate of the different soil-amendment mixtures. The soil was mixed with the organic amendments at a rate equivalent to 50,000 kg ha(-1) and incubated during 40 weeks at constant moisture content (70% of its water-holding capacity) and temperature (28 degrees C) under aerobic conditions. Organic amendment-soil samples showed an immobilization of N during the first weeks, which was more noticeable and longer in the case of PS-treated soil compared to the other two amendments due to its high C/N ratio. After this immobilization stage, a positive mineralization was observed for all treatment, especially in MWC treated soil. Contemporaneously a 1-year column (19 cm diameter and 60 cm height) experiment was carried out to estimate the nitrate losses from the soil amended with the same organic materials. Amendments were mixed with the top soil (0-15 cm) at a rate equivalent to 50,000 kg ha(-1). The columns were periodically irrigated simulating rainfall in the area of study, receiving in total 415 mm of water, and the water draining was collected during the experimental period and analysed for NO3-N. At the end of the experimental period NO3-N content in soil columns at three depths (0-20, 20-35 and 35-50 cm) was determined. The nitrate concentration in drainage water confirmed the results obtained in the incubation experiment: nitrate leaching was higher in soil treated with MWC due to its higher N-mineralization rate. Nevertheless, the nitrate losses represented a low amount compared with the total nitrogen added to soil. No clear signs of water-draining contamination were observed during the first year after the application of AC and PS; however, the nitrate leaching in soil treated with MWC slightly exceeded the limit allowed for the Drinking Water Directive 98/83/CE.  相似文献   

14.
In Ireland, conversion of biodegradable farm wastes such as pig manure spent mushroom compost and poultry litter wastes to pelletised fertilisers is a desirable option for farmers. In this paper, results obtained from the composting of pig waste solids (20% w/w) blended with other locally available biodegradable wastes comprising poultry litter (26% w/w), spent mushroom compost (26% w/w), cocoa husks (18% w/w) and moistened shredded paper (10% w/w) are presented. The resulting 6-mo old 'mature' composts had a nutrient content of 2.3% total N, 1.6% P and 3.1% K, too 'low' for direct use as an agricultural fertiliser. Formulations incorporating dried blood or feather meal amendments enriched the organic N-content, reduced the moisture in mature compost mixtures and aided the granulation process. Inclusion of mineral supplements viz., sulphate of ammonia, rock phosphate and sulphate of potash, yielded slow release fertilisers with nutrient N:P:K ratios of 10:3:6 and 3:5:10 that were suited for amenity grasslands such as golf courses for spring or summer application and autumn dressing, respectively. Rigorous microbiological tests carried out throughout the composting, processing and pelletising phases indicated that the formulated organo-mineral fertilisers were free of vegetative bacterial pathogens.  相似文献   

15.
Compost application to turfgrass soils may increase dissolved organic C (DOC) levels which affects nutrient dynamics in soil. The objectives of this study were to investigate the influence of compost source and application rate on soil organic C (SOC), DOC, NO(3), and available P during 29 months after a one-time application to St. Augustinegrass [Stenotaphrum secundatum (Walt.) Kuntze] turf. Compost sources had variable composition, yet resulted in few differences in SOC, DOC, and NO(3) after applied to soil. Available NO(3) rapidly decreased after compost application and was unaffected by compost source and application rate. Available P increased after compost application and exhibited cyclical seasonal patterns related to DOC. Compost application decreased soil pH relative to unamended soil, but pH increased during the course of the study due to irrigation with sodic water. Increasing the compost application rate increased SOC by 3 months, and levels remained fairly stable to 29 months. In contrast, DOC continued to increase from 3 to 29 months after application, suggesting that compost mineralization and growth of St. Augustinegrass contributed to seasonal dynamics. Dissolved organic C was 75%, 78%, and 101% greater 29 months after application of 0, 80, and 160 Mg compostha(-1), respectively, than before application. Impacts of composts on soil properties indicated that most significant effects occurred within a few months of application. Seasonal variability of SOC, DOC, and available P was likely related to St. Augustinegrass growth stages as well as precipitation, as declines occurred after precipitation events.  相似文献   

16.
An attempt was made to recycle waste biomass and mineral powder (waste mica) as an alternative source of potassium (K) through composting technology. Two different waste biomass, isabgol straw and palmarosa distillation waste along with two levels of waste mica (2 and 4% as K) were used for preparation of enriched composts. A notable decrease of C:N ratio was observed at the end of the composting (150 days) as an indicator of compost maturity. The mature composts were evaluated for K-supplying capacity through laboratory leaching and soil incubation study. Significantly higher water-soluble K released initially followed by a sharp decrease up to 21 days of leaching thereafter gradually decreased up to 35 days of leaching. Water-soluble K was released from K-enriched (mica charged) compost significantly higher than the ordinary compost throughout the leaching period. Soil incubation study also revealed that application of K-enriched compost greatly improved the available K (water soluble and exchangeable) pools in K-deficient soil which indicated that a considerable amount of K releases during composting. Therefore, K-enriched compost could be an effective alternative of costly commercial K fertilizer and eco-friendly approach to utilize low-cost waste mineral powder and plant residue.  相似文献   

17.
In order to study the suitability of composting olive mill wastewater (OMW-L) by repeated applications, OMW-L was added to one mixture of lawn trimmings and olive husks as bulking agents. The composting process of this mixture was compared with another pile having 35% of olive mill wastewater sludge (OMW-S) obtained from evaporation ponds and a third, as a control, without olive mill wastewater. The repeated applications of OMW-L resulted in a sharp decrease in respiration measurements after the first 20 days of composting and showed a re-increase after 40 days following the substituting of OMW-L by water. The OMW-L addition increased the rate of water-soluble phenols in the compost and caused the appearance of a phenol fraction of high molecular-mass (510 kDa) at the end of composting. OMW-L addition also caused a clear decrease in both thermophilic bacteria and thermophilic eumycete counts. A longer persistence of phytotoxicity was observed in comparison with the other piles. However, the OMW-S produced a compost with a high degree of maturity.  相似文献   

18.
The effects of adding biosolids to a green waste feedstock (100% green waste, 25% v/v biosolids or 50% biosolids) on the properties of composted products were investigated. Following initial composting, 20% soil or 20% fly ash/river sand mix was added to the composts as would be carried out commercially to produce manufactured soil. Temperatures during composting reached 50 °C, or above, for 23 days when biosolids were included as a composting feedstock but temperatures barely reached 40 °C when green waste alone was composted. Addition of biosolids to the feedstock increased total N, EC, extractable NH4, NO3 and P but lowered pH, macroporosity, water holding capacity, microbial biomass C and basal respiration in composts. Additions of soil or ash/sand to the composts greatly increased the available water holding capacity of the materials. Principal component analysis (PCA) of PCR-DGGE 16S rDNA amplicons separated bacterial communities according to addition of soil to the compost. For fungal ITS-RNA amplicons, PCA separated communities based on the addition of biosolids. Bacterial species richness and Shannon’s diversity index were greatest for composts where soil had been added but for fungal communities these parameters were greatest in the treatments where 50% biosolids had been included. These results were interpreted in relation to soil having an inoculation effect and biosolids having an acidifying effect thereby favouring a fungal community.  相似文献   

19.
Influence of aeration rate on nitrogen dynamics during composting   总被引:6,自引:0,他引:6  
The paper aimed to study the influence of aeration rate on nitrogen dynamics during composting of wastewater sludge with wood chips. Wastewater sludge was sampled at a pig slaughterhouse 24h before each composting experiment, and mixtures were made at the same mass ratio. Six composting experiments were performed in a lab reactor (300 L) under forced aeration. Aeration flow was constant throughout the experiment and aeration rates applied ranged between 1.69 and 16.63 L/h/kg DM of mixture. Material temperature and oxygen consumption were monitored continuously. Nitrogen losses in leachates as organic and total ammoniacal nitrogen, nitrite and nitrate, and losses in exhaust gases as ammonia were measured daily. Concentrations of total carbon and nitrogen i.e., organic nitrogen, total ammoniacal nitrogen, and nitrite and nitrate were measured in the initial substrates and in the composted materials. The results showed that organic nitrogen, which was released as NH4+/NH3 by ammonification, was closely correlated to the ratio of carbon removed from the material to TC/N(org) of the initial substrates. The increase of aeration was responsible for the increase in ammonia emissions and for the decrease in nitrogen losses through leaching. At high aeration rates, losses of nitrogen in leachates and as ammonia in exhaust gases accounted for 90-99% of the nitrogen removed from the material. At low aeration rates, those accounted for 47-85% of the nitrogen removed from the material. The highest concentrations of total ammoniacal nitrogen in composts occurred at the lowest aeration rate. Due to the correlation of ammonification with biodegradation and to the measurements of losses in leachates and in exhaust gases, the pool NH4+/NH3 in the composting material was calculated as a function of time. The nitrification rate was found to be proportional to the mean content of NH4+/NH3 in the material, i.e., initial NH4+/NH3 plus NH4+/NH3 released by ammonification minus losses in leachates and in exhaust gases. The aeration rate was shown to be a main parameter affecting nitrogen dynamics during composting since it controlled the ammonification, the ammonia emission and the nitrification processes.  相似文献   

20.
To evaluate the effect of vermiculite addition on composting food wastes from Korean households, food wastes were composted in three small bins to which different additives were added. The following three bins were employed: in Case I, only recycled compost was composted; in Case II, food wastes with recycled compost; and in Case III, food wastes with recycled compost and vermiculite. In the experiment performed for 30 days, it was confirmed that the supplementary addition of vermiculite to the composting mixture did not significantly improve the weight loss rate and the decomposition rate of food wastes. Due to dilution through the use of inorganic vermiculite, the vermiculite addition reduced the organic matter concentration of the composting mixtures. Vermiculite addition did not raise the pH value. Weight losses of roughly 70% were observed based on calculating moisture loss as well as dry food waste loss and not considering additives, while dry food waste loss was 29.4% and 35.8% with and without the addition of vermiculite, respectively. For these experiments, the major portion of the weight loss was the loss of water. The results indicate a need to differentiate between weight loss percentages and decomposition percentages, and a need to indicate if either of these percentages includes or excludes the mass of additives.  相似文献   

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