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1.
Indoor radon distribution of subway stations in a Korean major city   总被引:1,自引:0,他引:1  
The overall survey on indoor radon concentration was conducted at all subway stations in a major city, Daejeon in the central part of Korea. It was quarterly performed from September 2007 to August 2008. The annual arithmetic mean of indoor radon concentration of all the stations was 34.1 ± 14.7 Bq m−3, and the range of values was from 9.4 to 98.2 Bq m−3. The radon concentrations in groundwater (average 31.0 ± 0.8 Bq m−3) were not significantly high in most stations, but the concentration (177.9 ± 2.3 Bq L−1) of one station was over the level of 148 Bq L−1 in drinking water proposed by U.S. EPA. Based on indoor survey results, the approximate average of the annual effective dose by radon inhalation to the employees and passengers were 0.24 mSv y−1, and 0.02 mSv y−1, respectively. Although the effective dose based on the UNSCEAR report was potentially estimated, for more accurate assessment, the additional survey on the influence by indoor radon will be necessary.  相似文献   

2.
Galicia (NW Spain) is a radon-prone area in the Iberian Peninsula. Measurements were carried out at a rural dwelling, with an annual average of radon concentration over 4000 Bq m−3 and a maximum of 9000 Bq m−3, found during a radon screening campaign held in the Autonomous Community of Galicia. We performed a detailed study to identify the main contamination source and the behaviour of the radon concentration, in which a linear dependence with temperature was verified, once corrected for relative humidity. We used different passive methods (charcoal canisters and two types of etched track detectors) as well as a radon concentration monitor that provided continuous measurement. Subsequent to this characterization, and in order to reduce the high radon concentration, a remedial action was developed using different passive and forced ventilation methods. A modified subslab depressurization technique was found to be the most effective remedy, providing a radon concentration reduction of around 96%. This method also has the advantages of being inexpensive and reliable over time.  相似文献   

3.
An estimation of the indoor background radiation dose distribution was carried out in dwellings of eleven villages located within and around the uranium mineralization area of Kylleng-Pyndensohiong, Mawthabah in West Khasi Hills District of Meghalaya, India. The ambient indoor gamma radiation level was monitored using Thermo Luminescence Dosimeters (TLDs) while the indoor radon and thoron concentration was measured using twin-cup dosimeters employing Solid State Nuclear Track Detectors (SSNTDs). Results obtained from the study reveals that the local inhabitants of villages located close to the mining site receive higher doses than those inhabitants of villages located at a much farther distance from the mining site. The average total annual effective dose was found to be varying from 1.2 mSv y−1 in the village of Langpa to 3.4 mSv y−1 in the village of Nongbah Jynrin. The data obtained will serve as a reference in documenting changes to environmental radioactivity if mining is to be carried out in the future.  相似文献   

4.
Least squares (LS), Theil’s (TS) and weighted total least squares (WTLS) regression analysis methods are used to develop empirical relationships between radium in the ground, radon in soil and radon in dwellings to assist in the post-closure assessment of indoor radon related to near-surface radioactive waste disposal at the Low Level Waste Repository in England. The data sets used are (i) estimated 226Ra in the <2 mm fraction of topsoils (eRa226) derived from equivalent uranium (eU) from airborne gamma spectrometry data, (ii) eRa226 derived from measurements of uranium in soil geochemical samples, (iii) soil gas radon and (iv) indoor radon data. For models comparing indoor radon and (i) eRa226 derived from airborne eU data and (ii) soil gas radon data, some of the geological groupings have significant slopes. For these groupings there is reasonable agreement in slope and intercept between the three regression analysis methods (LS, TS and WTLS). Relationships between radon in dwellings and radium in the ground or radon in soil differ depending on the characteristics of the underlying geological units, with more permeable units having steeper slopes and higher indoor radon concentrations for a given radium or soil gas radon concentration in the ground. The regression models comparing indoor radon with soil gas radon have intercepts close to 5 Bq m−3 whilst the intercepts for those comparing indoor radon with eRa226 from airborne eU vary from about 20 Bq m−3 for a moderately permeable geological unit to about 40 Bq m−3 for highly permeable limestone, implying unrealistically high contributions to indoor radon from sources other than the ground. An intercept value of 5 Bq m−3 is assumed as an appropriate mean value for the UK for sources of indoor radon other than radon from the ground, based on examination of UK data. Comparison with published data used to derive an average indoor radon: soil 226Ra ratio shows that whereas the published data are generally clustered with no obvious correlation, the data from this study have substantially different relationships depending largely on the permeability of the underlying geology. Models for the relatively impermeable geological units plot parallel to the average indoor radon: soil 226Ra model but with lower indoor radon: soil 226Ra ratios, whilst the models for the permeable geological units plot parallel to the average indoor radon: soil 226Ra model but with higher than average indoor radon: soil 226Ra ratios.  相似文献   

5.
In order to evaluate the influence of faulting on the variability of geogenic radon at detailed scale (1:2000), data on gamma ray fluxes, U and Th concentrations in rocks, radon in soil-gas and radon in groundwater were collected in three target areas on the Oliveira do Hospital region (Central Portugal). This region stands on the Iberian Uranium Province, and is dominantly composed of Hercynian granites and metasedimentary rocks of pre-Ordovician age, crosscut by faults with dominant strike N35°E, N55°E and N75°E. Radiometric anomalies are frequent, associated with faults of the referred systems and metasedimentary enclaves; the analytical data confirms that these anomalies are produced by local high uranium contents in rocks and fault-filling materials (n = 34, range 13-724 ppm), while other radiogenic elements are relatively constant (e.g. Th 4-30 ppm). Radon concentration in soil can be extremely high, up to 12,850 kBq m−3 (n = 215), with a large proportion of results above 100 kBq m−3. Unsurprisingly, groundwater also shows high radon concentrations, with observed values in the range 150-4850 Bq.L−1 (n = 17). From the results it is concluded that metasedimentary enclaves, as well as faults, can accumulate uranium from circulating fluids, and as a consequence, strongly locally enhance geogenic radon potential. Due to this fact, for the purpose of land use planning in such uranium-enriched regions, very detailed geological mapping is needed to precisely recognize radon high risk areas. A correlation between radon concentration in soil or in groundwater and gamma ray fluxes was established pointing to the possible use of these fluxes as a first step in assessing geogenic radon potential, at least to geological setting similar to the study area.  相似文献   

6.
Radon exhalation from building materials for decorative use   总被引:2,自引:0,他引:2  
Long-term exposure to radon increases the risk of developing lung cancer. There is considerable public concern about radon exhalation from building materials and the contribution to indoor radon levels. To address this concern, radon exhalation rates were determined for 53 different samples of drywall, tile and granite available on the Canadian market for interior home decoration. The radon exhalation rates ranged from non-detectable to 312 Bq m−2 d−1. Slate tiles and granite slabs had relatively higher radon exhalation rates than other decorative materials, such as ceramic or porcelain tiles. The average radon exhalation rates were 30 Bq m−2 d−1 for slate tiles and 42 Bq m−2 d−1 for granite slabs of various types and origins. Analysis showed that even if an entire floor was covered with a material having a radon exhalation rate of 300 Bq m−2 d−1, it would contribute only 18 Bq m−3 to a tightly sealed house with an air exchange rate of 0.3 per hour. Generally speaking, building materials used in home decoration make no significant contribution to indoor radon for a house with adequate air exchange.  相似文献   

7.
Radon and gamma radiation level measurements were carried out inside the La Carolina mine, one of the oldest gold mining camps of southern South America, which is open for touristic visits nowadays. CR-39 track-etch detectors and thermoluminescent dosimeters of natural CaF2 and LiF TLD-100 were exposed at 14 points along the mine tunnels in order to estimate the mean 222Rn concentration and the ambient dose equivalent during the summer season (November 2008 to February 2009). The values for the 222Rn concentration at each monitoring site ranged from 1.8 ± 0.1 kBq m−3 to 6.0 ± 0.5 kBq m−3, with a mean value of 4.8 kBq m−3, indicating that these measurements exceed in about three times the upper action level recommended by ICRP for workplaces. The correlations between radon and gamma radiation levels inside the mine were also investigated. Effective doses due to 222Rn and gamma rays inside the mine were determined, resulting in negligible values to tourists. Considering the effective dose to the mine tourist guides, values exceeding 20 mSv of internal contribution to the effective doses can be reached, depending on the number of working hours inside the mine.  相似文献   

8.
It is shown in this work that parameters of the Jacobi model, which describes behavior of short-lived radon progeny, are not independent. The relationship between deposition rate of attached radon progeny and attachment rate of their unattached fraction was determined in this paper. It was found that deposition rate increases when the attachment rate is smaller; this effect is more pronounced for larger friction velocity. The deposition rate of attached radon progeny is presented here as a function of friction velocity, ventilation and attachment rate. Deposition rate of attached fraction was estimated in the range 0.012-0.46 h−1, when attachment rate varies from 10 h−1 to 100 h−1.  相似文献   

9.
The paper presents the results of year-long measurements of radon (222Rn) concentration inside 129 buildings in Poland in relation to the geological conditions of their foundation. The authors took into account the division of the country into tectonic units, as well as the lithology of the rocks forming the bedrock of these buildings. As expected, the highest value of mean annual 222Rn concentration (845 Bq/m3) was recorded in a building situated in the area of the Sudetes, while the highest geometric mean (characteristic of the expected log-normal data distribution) was calculated based on measurements from buildings located within the East-European craton, in the area of Mazury-Podlasie monocline, where it reached 231 Bq/m3. Such results reflect geological conditions - the occurrence of crystalline rocks (especially U- and Ra-enriched granites and orthogneisses) on the surface in the Sudetes, and of young post-glacial sediments containing fragments of Scandinavian crystalline rocks, also enriched with U and Ra, in the area of Mazury-Podlasie monocline. However, the least expected result of the investigations was finding out that, contrary to the hitherto widespread belief, none of the major tectonic units of Poland can be excluded from the list of those containing buildings with mean annual 222Rn concentration exceeding 200 Bq/m3. The mean annual concentration of radon for all the buildings were much higher than the mean concentration value (49.1 Bq/m3) of indoor radon in Poland quoted so far. These results cast a completely new light on the necessity to perform measurements of radon concentration in residential buildings in Poland, no more with reference to small areas with outcrops of crystalline rocks (especially the Sudetes, being the Polish fragment of the European Variscan belt), but for all the major tectonic units within Poland.  相似文献   

10.
Radon and gamma dose rate measurements were performed in 512 schools in 8 of the 13 regions of Greece. The distribution of radon concentration was well described by a lognormal distribution. Most (86%) of the radon concentrations were between 60 and 250 Bq m−3 with a most probable value of 135 Bq m−3. The arithmetic and geometric means of the radon concentration are 149 Bq m−3 and 126 Bq m−3 respectively. The maximum measured radon gas concentration was 958 Bq m−3. As expected, no correlation between radon gas concentration and indoor gamma dose rate was observed. However, if only mean values for each region are considered, a linear correlation between radon gas concentration and gamma dose rate is apparent. Despite the fact that the results of radon concentration in schools cannot be applied directly for the estimation of radon concentration in homes, the results of the present survey indicate that it is desirable to perform an extended survey of indoor radon in homes for at least one region in Northern Greece.  相似文献   

11.
This paper shows the results of a survey carried out at some refractory manufacturing plants. During the first part of the survey, the concentration of natural radioactivity in raw materials and end-products, coming from four plants, was assessed. Several raw materials and, as a consequence, some end-products as well have shown activity concentrations exceeding a few hundreds of Bq kg−1 of 238U and 232Th. In some important raw materials, such as bauxite and corundums, a remarkable radioactive disequilibrium was observed; this is probably due to the high temperature processes undergone by these materials. The second part of the survey focussed on the measurements of ambient equivalent dose rates, airborne dust concentrations and radon indoor. On the basis of results obtained, the effective dose for the standard worker was estimated. Two different types of refractory plants were investigated. Effective doses for both plants were lower than 1 mSv y−1.  相似文献   

12.
Removal of uranium [U(VI)] from aqueous solutions with humic acid-immobilized zirconium-pillared clay (HA-Zr-PILC) was investigated using a batch adsorption technique. The adsorbent was characterized using XRD, FTIR, SEM, TG/DTG, surface area analyzer and potentiometric titration. The effects of pH, contact time, initial concentration, adsorbent dose, and adsorption isotherm on the removal process were evaluated. A maximum removal of 97.6 ± 2.1 and 94.7 ± 3.3% was observed for an initial concentration of 50 and 100 mg L−1, respectively at pH 6.0 and an adsorbent dose of 2.0 g L−1. Equilibrium was achieved in approximately 180 min. The mechanism for the removal of U(VI) ions by HA-Zr-PILC was based on an ion exchange reaction. The experimental kinetic and isotherm data were analyzed using a second-order kinetic equation and Langmuir isotherm model, respectively. The monolayer adsorption capacity for U(VI) removal was found to be 132.68 ± 5.04 mg g−1. An increase of temperature of the medium caused an increase in metal adsorption. Complete removal (≅100%) of U(VI) from 1.0 L of a simulated nuclear industry effluent sample containing 10.0 mg U(VI) ions was possible with 1.5 g of HA-Zr-PILC. The adsorbent was suitable for repeated use (over 4 cycles) without any noticeable loss of capacity.  相似文献   

13.
The Syabru-Bensi hydrothermal zone, Langtang region (Nepal), is characterized by high radon-222 and CO2 discharge. Seasonal variations of gas fluxes were studied on a reference transect in a newly discovered gas discharge zone. Radon-222 and CO2 fluxes were measured with the accumulation chamber technique, coupled with the scintillation flask method for radon. In the reference transect, fluxes reach exceptional mean values, as high as 8700 ± 1500 g m−2 d−1 for CO2 and 3400 ± 100 × 10−3 Bq m−2 s−1 for radon. Gases fluxes were measured in September 2007 during the monsoon and during the dry winter season, in December 2007 to January 2008 and in December 2008 to January 2009. Contrary to expectations, radon and its carrier gas fluxes were similar during both seasons. The integrated flux along this transect was approximately the same for radon, with a small increase of 11 ± 4% during the wet season, whereas it was reduced by 38 ± 5% during the monsoon for CO2. In order to account for the persistence of the high gas emissions during monsoon, watering experiments have been performed at selected radon measurement points. After watering, radon flux decreased within 5 min by a factor of 2–7 depending on the point. Subsequently, it returned to its original value, firstly, by an initial partial recovery within 3–4 h, followed by a slow relaxation, lasting around 10 h and possibly superimposed by diurnal variations. Monsoon, in this part of the Himalayas, proceeds generally by brutal rainfall events separated by two- or three-day lapses. Thus, the recovery ability shown in the watering experiments accounts for the observed long-term persistence of gas discharge. This persistence is an important asset for long-term monitoring, for example to study possible temporal variations associated with stress accumulation and release.  相似文献   

14.
Natural background gamma radiation and radioactivity concentrations were investigated from 2003 to 2005 in Kinta District, Perak, Malaysia. Sample locations were distant from any ‘amang’ processing plants. The external gamma dose rates ranged from 39 to 1039 nGy h−1. The mean external gamma dose rate was 222 ± 191 nGy h−1. Small areas of relatively enhanced activity were located having external gamma dose rates of up to 1039 ± 104 nGy h−1. The activity concentrations of 238U, 232Th and 40K were analyzed by using a high-resolution co-axial HPGe detector system. The activity concentration ranges were 12–426 Bq kg−1 for 238U, 19–1377 Bq kg−1 for 232Th and <19–2204 Bq kg−1 for 40 K. Based on the radioactivity levels determined, the gamma-absorbed dose rates in air at 1 m above the ground were calculated. The calculated dose rates and measured dose rates had a good correlation coefficient, R of 0.94. To evaluate the radiological hazard of the natural radioactivity, the radium equivalent activity, the gamma-absorbed dose rate and the mean population weighted dose rate were calculated. An isodose map for the Kinta District was also produced.  相似文献   

15.
Significantly high radiation level and radionuclide concentration along Quilon beach area of coastal Kerala have been reported by several investigators. Detailed gamma radiation level survey was carried out using a portable scintillometer. Detailed studies on radionuclides concentration in different environmental matrices of high background areas were undertaken in the coastal areas of Karunagapalli, Kayankulam, Chavara, Neendakara and Kollam to study the distribution and enrichment of the radionuclides in the region. The absorbed gamma dose rates in air in high background area are in the range 43-17,400 nGyh−1. Gamma radiation level is found to be maximum at a distance of 20 m from the sea waterline in all beaches. The soil samples collected from different locations were analysed for primordial radionuclides by gamma spectrometry. The activity of primordial radionuclides was determined for the different size fractions of soil to study the enrichment pattern. The highest activity of 232Th and 226Ra was found to be enriched in 125-63 μ size fraction. The preferential accumulation of 40K was found in <63 μ fraction. The minimum 232Th activity was 30.2 Bq kg−1, found in 1000-500 μ particle size fraction at Kollam and maximum activity of 3250.4 Bq kg−1 was observed in grains of size 125-63 μ at Neendakara. The lowest 226Ra activity observed was 33.9 Bq kg−1 at Neendakara in grains of size 1000-500 μ and the highest activity observed was 482.6 Bq kg−1 in grains of size 125-63 μ in Neendakara. The highest 40K activity found was 1923 Bq kg−1 in grains of size <63 μ for a sample collected from Neendakara. A good correlation was observed between computed dose and measured dose in air. The correlation between 232Th and 226Ra was also moderately high. The results of these investigations are presented and discussed in this paper.  相似文献   

16.
One of the essential parameters influencing of the dose conversion factor is the ratio of unattached short-lived radon progeny. This may differ from the value identified for indoor conditions when considering special workplaces such as mines. Inevitably, application of the dose conversion factors used in surface workplaces considerably reduces the reliability of dose estimation in the case of mines.This paper surveyed the concentration of radon and its short-lived radon progeny and identified the unattached fraction of short-lived radon progeny. As well equilibrium factor during the month of August was calculated simultaneously at two extraction faces in a manganese ore mine.During working hours the average radon concentrations were 220 Bq m−3 and 530 Bq m−3 at Faces 1 and 2; the average short-lived progeny concentration was 90 Bq m−3 and 190 Bq m−3, the average equilibrium factors were 0.46 and 0.36, and the average unattached fractions were 0.21 and 0.17, respectively. The calculated dose conversion factor was between 9 and 27 mSv WLM−1, but higher values could also be possible.  相似文献   

17.
The role of puddle sediments as a final depot of 137Cs horizontal migration within the urban landscape is studied using the example of Ekaterinburg city, Russia. Radioactive contamination in the city appeared due to fallout after atmospheric testing of nuclear weapons and nuclear accidents. Contamination density of 137Cs in the region was assessed from archive data to be about 5.1 kBq/m2, of which the maximum activity concentration (<30 Bq/kg) is associated with the upper 15 cm soil layer. Results of the survey reported here indicate a mean 137Cs activity concentration in puddle sediments of 80 Bq/kg, with a maximum value of 540 Bq/kg. It is estimated that horizontal migration has led to about a fourfold concentration of 137Cs in puddle sediments.  相似文献   

18.
Natural radioactive materials under certain conditions can reach hazardous radiological levels. So, it becomes necessary to study the natural radioactivity levels in soil to assess the dose for the population in order to know the health risks and to have a baseline for future changes in the environmental radioactivity due to human activities. The natural radionuclide (226Ra, 232Th, and 40K) contents in soil were determined for 26 locations around the Upper Siwaliks of Kala Amb, Nahan and Morni Hills, Northern India, using high-resolution gamma-ray spectrometric analysis. It was observed that the concentration of natural radionuclides viz., 226Ra, 232Th and 40K, in the soil varies from 28.3 ± 0.5 to 81.0 ± 1.7 Bq kg−1, 61.2 ± 1.3 to 140.3 ± 2.6 Bq kg−1 and 363.4 ± 4.9 to 1002.2 ± 11.2 Bq kg−1 respectively. The total absorbed dose rate calculated from activity concentration of 226Ra, 232Th and 40K ranged from 71.1 to 162.0 nGy h−1. The radium equivalent (Req) and the external hazard index (Hex), which resulted from the natural radionuclides in soil, were also calculated and found to vary from 149.4 to 351.8 Bq kg−1and from 0.40 to 0.95 respectively. These values in Upper Siwaliks area were compared with that from the adjoining areas of Punjab. The radium equivalent activities in all the soil samples were lower than the limit (370 Bq kg−1) set in the Organization for Economic Cooperation and Development (OECD) report and the dose equivalent was within the safe limit of 1 mSv y−1.  相似文献   

19.
The paper presents a systematic study on suitability of various gamma lines for monitoring of 238U activity in soil samples around a uranium mineralized zone of Kylleng Pyndengsohiong Mawthabah (Domiasiat), Meghalaya in India. The area lies in a plateau region which recieves the highest average annual rainfall (12,000 mm) in the world. The geochemical behaviour of the uranium and its daughter products at such wet climatic conditions imposes restrictions to assess 238U through gamma lines of radon decay products. Soil samples were collected from nine locations around the uranium mineralization zone for analysis. The ratio of the concentration of uranium obtained from gamma energies of radium daughter products to the 63.29 keV of 234Th was found to vary from 1.01 to 2.07, which indicates a pronounced disequilibrium between uranium and radium daughters. The results obtained from various gamma energies were validated from the data generated by Instrumental Neutron Activation Analysis (INAA) technique. The 238U activities from the two analytical methods show a well fitted regression line with correlation coefficient 0.99 which validates the reliability of 63.29 keV energy for estimation of uranium in such conditions.  相似文献   

20.
High indoor radon concentrations in Jordan result in internal exposures of the residents due to the inhalation of radon and its short-lived progeny. It is therefore important to quantify the annual effective dose and further the radiation risk to the radon exposure. This study describes the methodology and the biokinetic and dosimetric models used for calculation of the inhalation doses exposed to radon progeny. The regional depositions of aerosol particles in the human respiratory tract were firstly calculated. For the attached progeny, the activity median aerodynamic diameters of 50 nm, 230 nm and 2500 nm were chosen to represent the nucleation, accumulation and coarse modes of the aerosol particles, respectively. For the unattached progeny, the activity median thermodynamic diameter of 1 nm was chosen to represent the free progeny nuclide in the room air. The biokinetic models developed by the International Commission on Radiological Protection (ICRP) were used to calculate the nuclear transformations of radon progeny in the human body, and then the dosimetric model was applied to estimate the organ equivalent doses and the effective doses with the specific effective energies derived from the mathematical anthropomorphic phantoms. The dose conversion coefficient estimated in this study was 15 mSv WLM−1 which was in the range of the values of 6-20 mSv WLM−1 reported by other investigators. Implementing the average indoor radon concentration in Jordan, the annual effective doses were calculated to be 4.1 mSv y−1 and 0.08 mSv y−1 due to the inhalation of radon progeny and radon gas, respectively. The total annual effective dose estimated for Jordanian population was 4.2 mSv y−1. This high annual effective dose calculated by the dosimetric approach using ICRP biokinetic and dosimetric models resulted in an increase of a factor of two in comparison to the value by epidemiological study. This phenomenon was presented by the ICRP in its new published statement on radon.  相似文献   

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