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1.
Fifteen species of wild mushrooms and underlying soil samples collected in a virgin landscape of Augustowska Forest in northeastern Poland in 1997-98 were analyzed for total mercury to evaluate the status of contamination and usefulness of higher mushrooms as possible bioindicators of mercury pollution. Among the 15 species analyzed, Pinewood King Bolete, Scaly Tooth and King Bolete showed relatively high bioconcentration factors (BCF: dry-weight normalized concentrations of mercury in mushrooms relative to concentrations in soil) for mercury, which varied between 69 and 110. These three species were also characterized by great concentrations of total mercury in caps (between 2,000 +/- 800 and 2,300 +/- 1,100 ng g-1 dry wt) and stalks (between 850 +/- 390 and 1,000 +/- 500 ng g-1 dry wt.). Species such as Red-hot Milk Cap, Poison Pax and Common Chantherelle had mercury BCFs of less than 1, while Gipsy Bolete, Orange Birch Bolete, Brown Scaber Stalk, Variegated Bolete, Sandy Knight-cap and Yellow-cracking Bolete were weak or moderate mercury accumulators with BCFs between 1 and 40. Concentrations of mercury in mushrooms were greater than the tolerance limits suggested for mercury in plant foods.  相似文献   

2.
A systemic study on the natural radionuclides such as (210)Po and (210)Pb in the environmental matrices and biota of Ennore Creek has been undertaken to establish a baseline data on the radiation profile of Ennore Creek environment. The environmental samples such as water, sediment, and biota (seaweeds, molluscs, crustaceans, and fishes) have been subjected to analyses. It has been observed that the concentration of (210)Po and (210)Pb in the water samples of Ennore Creek as 2.7 and 1.63 m Bq L(-1), respectively. The activity concentration of (210)Po and (210)Pb in the sediment sample was 17.9 and 28.9 Bq kg(-1), respectively. The bivalve mollusk Perna viridis have been identified to accumulate higher concentrations of (210)Po and (210)Pb suggesting that they could serve as bioindicator of radionuclides in the Ennore Creek environment. The committed effective dose for human beings was found at 81.13-216.8 and 2.1-297.2 μSv year(-1) for (210)Po and (210)Pb, respectively.  相似文献   

3.
This study was aimed at assessing the levels of 210Pb and 210Po concentrations as well as gross alpha and beta activities in environmental monitors from the Catalan stretch of the Ebro River (Spain), potentially influenced by the presence of sediments with high concentrations of 238U and its decay chain daughters in the Flix reservoir. The chronic daily intake of 210Pb and 210Po through ingestion and inhalation of soils was evaluated, and the derived non-carcinogenic and carcinogenic risks were characterized. The low concentration of radioisotopes in soils resulted in a negligible annual effective dose. The levels of 210Pb and 210Po were determined in various groups of highly consumed food (fish and seafood, vegetables, fruits, and rice), and their dietary intake was calculated. The annual effective dose for the adult people from food intake was estimated in 3.3 × 10???2 mSv, mostly due to 210Po. Overall, the current radioactivity levels in the Catalan stretch of the Ebro River should not mean any additional health risk for the population living nearby. However, an integral assessment of the risks derived from exposure to other pollutants (e.g., metals and organochlorine compounds) jointly with radionuclides could be of great interest.  相似文献   

4.
Micro element and heavy metal contents of mushrooms were determined by Inductively Coupled Plasma Atomic Emission Spectrometry (ICP-AES). It was seen an increase in the heavy metal contents (except Cu and Zn) of the mushrooms until the second dose. A decrease was seen in heavy metal intake of the mushroom in the application of the third dose. The highest accumulation occurred from the upper soils treated with the second dose. Amounts of Cd, Cr, Cu, Pb and Zn, which were accumulated in the mushroom after the application of this dose, were detected as 5.7, 23.1, 75.7, 62.8 and 99.3 ppm, respectively.  相似文献   

5.
The amount of the trace elements As, Ba, Cd, Cr, Cu, Hg, Li, Mn, Ni, Pb, Rb, Se, Sr, and Zn was measured in top soils and edible mushrooms, Boletus edulis, Macrolepiota procera, collected at five distinct green microhabitats inside the Lucca province, North-Central Italy (years 2008–2009). Results showed a top soil element content within the Italian statutory limits. Concerning the amount of mushroom elements, we observed significant species-differences obtaining higher levels of Ni, Rb, and Se in B. edulis or As, Pb, Cu in M. procera. Bioaccumulation factors (BCFs: element in mushroom/element in soil) resulted species-dependent and element-selective: in particular, B. edulis preferentially accumulated Se (BCFs varying from 14 to 153), while M. procera mainly concentrated Cu (BCFs varying from 5 to 15). As well, both species displayed between-site BCF differences. By a multivariate principal component approach, cluster analysis (CA), we could resolve two main clusters of soil element composition, corresponding to the most ecologically divergent sites. Besides, CA showed no cluster relating to element contents of B. edulis at the different collection sites, while a separation in groups was found for M. procera composition with respect to harvesting locations, suggesting uptake systems, in this saprotrophic species, sensitive to microhabitat. Regarding consumer safety, Cd, Hg, Pb levels resulted sometime relevant in present samples, never reaching values from current literature on mushrooms collected in urban-polluted areas. Our findings encourage a deeper assessment of the molecular mechanisms of metal intake by edible mushrooms, encompassing genetic biochemical and geo-ecological variables, with particular awareness to element bioavailability in soils and fungi.  相似文献   

6.
In view of considerable natural background radioactivity reported from southwest coast of India, the current study documents bioaccumulation of 210Po in two dominant coastal sand dune perennial mat-forming wild legumes, Canavalia cathartica and C. maritima. Root, stem, leaf, mature beans, dry seeds and rhizosphere sand were analyzed for 210Po concentration. 210Po activity decreased in the order of leaves > roots > seeds > stems > beans. The highest 210Po activity was recorded in rhizosphere sand samples (5.78-5.88 Bq kg(-1)) followed by the leaf samples (3.27-3.07 Bq kg(-1)), while it was lowest in mature beans (0.13-0.20 Bq kg(-1)). 210Po activities or tissue moisture between plant species were not significantly different (p > 0.05; t-test). But 210Po activity vs. moisture differed significantly in all tissues (p = 0.0001), vegetative tissues (root, stem and leaf) (p = 0.0016), seeds (p = 0.0393) and proteins in seeds (p = 2.355 x 10(-6)) indicating the importance of moisture and protein in 210Po accumulation. Although 210Po has affinity for proteins, it did not concentrate too much in seed proteins of Canavalia. Concentration of 210Po in mature beans is at safe levels as fisher folk only consume tender pods occasionally. 210Po activity in Canavalia is compared with other plant materials. As the landraces of C. cathartica and C. maritima are distributed throughout pantropical coastal areas, the current study emphasizes on considering them as bioindicators to monitor 210Po in coastal sand dune biomes and in turn the health of coastal population.  相似文献   

7.
The aim of the work was to determine the 210Po content in phytobenthos species (seaweeds and angiosperms) from Puck Bay (southern Baltic). Alpha spectrometry was used to measure and calculate the activities and concentrations of polonium 210Po in the phytobenthos. The activity of 210Po in Puck Bay waters was determined to estimate the bioconcentration factors (BCF) of these plants. The 210Po concentration in water was estimated at 0.25 mBq dm(-3). The lowest polonium concentration in the phytobenthos was found in Cladophora rupestris (0.12 Bq kg(-1) wet wt.), the highest in Chara crinita (1.12 Bq kg(-1) wet wt.). Polonium is accumulated in these phytobenthos species; the bioconcentration factors (BCF) ranged from 450 to 4400.  相似文献   

8.
The study was performed using a silicon surface barrier alpha spectrometer at Bhabha Atomic Research Centre, Mumbai, India. Through the study, the observed 210Po activity in water sample from different locations in the Domiasiat area ranges from 0.04 to 0.69 Bq/l. The daily and annual intake of 210Po through water was also estimated and the mean value of 0.72 and 263.61 Bq, respectively, were observed. It is observed that the effective doses through water were higher than the World Health Organization recommended dose of 0.05 mSv/year. The total annual effective doses through terrestrial ingestion for all the locations was studied and the mean annual effective dose was observed to be 0.315 mSv, which, when compared to the worldwide and the Indian values, was observed to be slightly higher. The mean activity in soil is found to be 124.8 ±5.7 Bq/kg and in meat the activity is 0.43 ±0.05 Bq/kg. In fishes, an activity of 0.48 ±0.07 Bq/kg in Garra lamta, 0.29 ±0.02 Bq/kg in Neolissocheilus hexaganolepis, and 3.3 ±0.1 Bq/kg in Macrobrachium sp. is observed. Activity concentration in plant samples was analyzed and the activity ranges from 0.020 ±0.002 to 9.69 ±0.35 Bq/kg. Committed effective dose by the adult population of the Domiasiat area through intake of 210Po through these food items was also determined and compared with the Indian average value and the worldwide average value.  相似文献   

9.
Activities of 210Po and 210Pb in various tissues of four species of decapod crabs and two species of cephalopod mollusks (cuttlefishes) of Kudankulam coast were studied. A non-uniform distribution of these radionuclides was observed between the organs. Of all the tissues, 210Po and 210Pb were found accumulated more in the hepatopancreas and intestine of crabs and in the digestive gland, shell gland, and intestine of cephalopods. Among crabs, Charybdis lucifera registered a little higher 210Po and 210Pb activities. The cephalopod species Loligo duvauceli displayed higher 210Po and 210Pb in some organs when compared to Sepia pharaonis. The muscle of all the species registered lower activity. In cephalopods, the activity ratio of 210Po/210Pb fell within the range of 1?C2 for most of the organs, and in crab tissues, it varied from 1.7 to 31.4. The biological concentration factor for organs of cephalopods ranged from 1.2 ×103 to 4.3 ×105 for 210Po and 4.8 ×102 to 8.4 ×104 for 210Pb and for organs of crabs it varied between 2.0 ×104 and 1.9 ×106 for 210Po and 9.2 ×102 and 2.4 ×104 for 210Pb. The study revealed that the organs associated with digestion and metabolism displayed a higher activity concentration than the other tissues. A significant variation in the accumulation of 210Po and 210Pb was noted between species (P?<?0.05). The activity levels recorded are in agreement with values recorded in related organisms in other parts of the world. The data generated will act as a reference database for these organisms of this coast in which a nuclear power station is under construction.  相似文献   

10.
Activities of 21?Po and 21?Pb in whole-body and in various tissues of brachyuran crabs collected along the Kudankulam coast were studied. A non-uniform distribution of these radionuclides was observed between the various tissues. Of all the tissues, 21?Po and 21?Pb were found to accumulate more in the hepatopancreas and intestine. Among the crabs studied, Charybdis lucifera registered higher 21?Po and 21?Pb activity. Muscle tissue in all the species registered lower activity. The 21?Po/21?Pb activity ratio was found to be greater than unity. The biological concentration factor for organs varied between ~ 10? and 10? for 21?Po and ~102 and 10? for 21?Pb. A significant variation in the accumulation of 21?Po and 21?Pb was noted between species and between seasons (p < 0.05). The mean whole-body internal dose ranged from 1.42 to 6.86 μGy h?1 for 21?Po and from 3.0 × 10?3 to 8.0 × 10?3 μGy h?1 for 21?Pb. The external dose for 21?Po and 21?Pb was 2.41 × 10?? to 5.76 × 10?? μGy h?1 and 4.14 × 10?? to 8.26 × 10?? μGy h?1, respectively. The activity levels recorded are in agreement with values recorded in related organisms in other parts of the world. The total committed effective dose due to the intake of both radionuclides ranged from 80.3 to 871.7 μSv y?1. The median dose calculated due to 21?Po and 21?Pb in certain crabs in Kudankulam is less and would not pose any significant radiological impact on health or a cancer risk to the public, and the seafood is considered safe for human consumption.  相似文献   

11.
The persistence of an island of remnant vegetation within a tailings retention system provided an opportunity to conduct a pilot study to develop hypothesis concerning the impacts of acid spray and radiation on arid zone flora and fauna. Ecological changes were investigated by comparing species abundance and condition on both the study island and remote control areas. Hopbush (Dodonaea viscosa), geckos and a common ant species, Iridomyrmex rufoniger sp. B were abundant in control regions but absent from the study region, whereas densities of colonising plant species, Helea beetles and scorpions were unusually high at the impacted site. These disparities are probably attributable to acid spray at the impacted site and hence are potentially useful bioindicators of these impacts. Dragon and skink populations were apparently unaffected by the polluted ecosystem, although Ctenophorus nuchalis proved to be a significant bioaccumulator of radionuclides. Bioaccumulation of the radionuclides, 238U, 230Th, 210Pb and particularly 210Po were significantly greater than that reported elsewhere in the literature. Further radionuclide monitoring of herbivorous dragon species, possibly concentrating upon 210Po levels, was the suggested outcome of this pilot study.  相似文献   

12.
In the present study the spatial and the vertical distributions of 210Pb were investigated in the soils around a uranifereous coal fired power plant (CPP) in Yatagan Basin, in Western Turkey. The variation of 226Ra activity along the soil profiles was studied to assess the unsupported 210Pb distribution in the same samples. 226Ra was measured by gamma spectroscopy and 210Pb activities were determined from 210Po activities using radiochemical deposition and alpha spectroscopy. The total 210Pb activity concentrations in bulk core samples varied in the range of 38-250 Bq kg(-1) in the study sites and of 22-78 Bq kg(-1) in reference site. In the sectioned cores sampled from the study areas the ranges for activity concentrations of 226Ra, total 210Pb and unsupported 210Pb are 24-77; 39-344 and 4-313 Bq kg(-1), respectively. Corresponding ranges for reference site are 37-39; 39-122 and 1-83 Bq kg(-1).  相似文献   

13.
Bottom sediments reflect in general the relative contamination of a sea area. Therefore, a great deal of monitoring work has been dedicated to the analysis of bottom sediments. Izmir Bay is a very important pollution centre in Turkish Aegean coast region due to a densely populated community, industrial complex and maritime transportation, and there are many streams flowing into the bay that pass through a number of industrial and agricultural areas. It had received the majority of domestic and industrial wastewaters until the wastewater treatment plant was constructed. It is well known that sediments play an important role as reservoirs of a fraction of the pollution in aquatic systems. Therefore, sediment samples were collected monthly from three stations which are located in the inner part of the bay during the period January to December 2003. Temporal variations and seasonal changes on their 210Po and 210Pb contents were examined, and the activity concentrations of 210Po and 210Pb were found to vary from 43±6 to 132±12 and 27±5 to 91±9 Bq kg???1 dry wt, respectively. The highest values of those natural radionuclides were measured at Kar??yaka Station because of the current systems of the bay. Seasonally, the 210Pb levels were found to increase during the winter time for all the stations.  相似文献   

14.
本文对国外3种名烟、国内畅销47种烟及新疆7种烟进行研究。结果表明:香烟中~(210)Po和~(210)Pb平衡系数为0.801;烟雾中~(210)Po和~(210)Pb比值为1.15,表明烟雾中~(210)Po量比~(210)Pb多;主流烟雾中~(210)Po占整支烟~(210)Po量的12.93%,而~(210)Pb占8.17%;烟咀阻留~(210)Po效率为(52.0±10.7)%,阻留~(210)Pb效率为(58.3±7.2)%;估算了每日吸一盒烟的人,20年肺和支气管剂量当量,约1.38 ×10~(-2)S_v。  相似文献   

15.
Ingestion of radionuclides and heavy metals through drinking water and food intake represents one of the important pathways for long-term health considerations. Milk and milk products are main constituents of the daily diet. Radionuclides and heavy metals can be apprehended in the ecosystem of the East Singhbhum region which is known for its viable grades of uranium, copper and other minerals. For the risk assessment studies, samples of milk were collected from twelve villages around Bagjata mining area and analysed for U(nat), 226Ra, 230Th, 210Po, Fe, Mn, Zn, Pb, Cu and Ni. Analysis of the results of the study reveals that the geometric mean of U(nat), 226Ra, 230Th and 210Po was 0.021, 0.24, 0.23 and 1.08 Bq l???1, respectively. The ingestion dose was calculated to be 12.34 ??SvY???1 which is reflecting the natural background dose via the route of ingestion, and much below the 1 mSv limit set in the new ICRP recommendations. The excess lifetime cancer risk was estimated to be 1.72 × 10???4 which is within the acceptable excess individual lifetime cancer risk value of 1 × 10???4. The geometric mean of Fe, Mn, Zn, Cu and Ni was 4.91, 0.29, 4.77, 0.56 and 0.48 mgl???1, respectively; whereas the daily intake was computed to be 0.44, 0.03, 0.43, 0.05 and 0.04 mg/day, respectively. Pb was not detected in any of the samples. The hazard quotient revealed that the intake of the heavy metals through the ingestion of milk does not pose any apparent threat to the local people as none of the HQ of the heavy metals exceeds the limit of 1.  相似文献   

16.
The concentrations of (238)U, (234)U, (226)Ra, (210)Po and (210)Pb have been determined in surface waters collected along the course of the Shu River, lying on the border between Kazakhstan and Kyrgyzstan. In the study area, the river runs through some of the largest uranium deposits worldwide, which were actively exploited during the nuclear weapons and nuclear energy programmes of the former Soviet Union. The data show an increasing trend in uranium concentrations downstream the river from the city of Tokmak to the city of Shu, with good correlation between total uranium concentrations and total dissolved solids. Data on uranium isotopes disequilibrium show the presence of technogenic uranium inputs into the Shu River downstream from the city of Karasu, evidenced by a decrease in the measured (234)U/(238)U isotopic ratio from 1.63 in uncontaminated sites to 1.29 in sites affected by past mining activities.  相似文献   

17.
The Screening Level Concentration (SLC) approach was used to derive Lowest Effect Level (LEL) and Severe Effect Level (SEL) concentrations for nine metals (As, Cr, Cu, Pb, Mo, Ni, Se, U and V) and three radionuclides (226Ra, 210Pb, and 210Po) released to the aquatic environment during the mining and milling of uranium ore. This method was chosen because it allowed for the best use of the considerable historical and current data collected for diverse purposes in the uranium mining and milling regions of Canada (20,606 data points used in the analysis). Except for Cr, all the LELs derived in this study using the weighted method and published sediment quality guidelines (SQGs) were highly reliable (> 85%) in predicting sites unimpacted by uranium mining/milling defined as sites where reductions in the abundance and species richness of benthic invertebrate communities were < 20%. The derived SEL values and corresponding published SQGs (with the exception of Ni) were not reliable predictors (≤60%) of severe impacts on benthic invertebrate communities when severe impacts are defined as a reduction in abundance and species richness ≥40%. Most of the severely impacted sites had sediment contaminant concentrations well below the SEL values. It is concluded that LELs derived using the weighted method can reliably be used in ecological risk assessments as concentrations below which adverse effects on benthic invertebrate communities are not expected. In contrast, it is recommended that SELs not be used in assessments of uranium mining/milling activities as concentrations above which adverse effects are anticipated.  相似文献   

18.
In Egypt, nineteen water springs with temperatures exceeding 35 degrees C, which can be considered thermal waters, were reported. The radiological aspects of thermal water in three northern regions of Egypt (Gulf of Suez, Cairo, and Bahariya Oasis) were investigated. The activity concentrations of natural radionuclides of 226Ra, 40K, total uranium and 210Pb (210Po) in water samples were determined using gamma spectrometry, laser fluorimetry and alpha spectrometry after chemical separation, respectively. The highest concentrations are detected in two locations, namely Sudr and Hammam Faroun springs, which are the hottest waters in Egypt (89 and 72 degrees C respectively). It seems that the presence of 226Ra is correlated to the water mineralization and the depth and the temperature of the reservoir's base. Also, these results seem evidence of uranium accumulation at depth in the mother bedrock and/or uranium immobilization due to uranium reduction to the immobile 4+-oxidation state in the reservoir base. The average activity concentrations of 40K are dependent on the water's origin, i.e. meteoric water mixed with sea water (Gulf of Suez springs) and meteoric water (Bahariya Oasis wells). There is no prescribed dose limit for short term and temporary exposure to thermal water. Workers at the thermal springs should be regularly monitored because of their continuous exposure to enhanced radiation levels over a long period of time. The hydrochemical characteristics, environmental isotopes aspects and water origin are briefly discussed based on published data.  相似文献   

19.
The first detectable activities of radioiodine (131)I, and radiocaesium (134)Cs and (137)Cs in the air over Central Poland were measured in dust samples collected by the ASS-500 station in the period of 21(st) to 24(th) of March, 2011. However, the highest activity of both fission products, (131)I and (137)Cs: 8.3 mBq m(-3) and 0.75 mBq m(-3), respectively, were obtained in the samples collected on 30(th) March, i.e.~18 days after the beginning of the fission products' discharge from the damaged units of the Fukushima Daiichi Nuclear Power Plant. The simultaneously determined corrected aerosol residence time for the same samples by (210)Pb/(210)Bi and (210)Pb/(210)Po methods was equal to 10 days. Additionally, on the basis of the activity ratio of two other natural cosmogenic radionuclides, (7)Be and (22)Na in these aerosol samples, it was possible to estimate the aerosol residence time at ~150 days for the solid particles coming from the stratospheric fallout. These data, as well as the differences in the activity size distribution of (7)Be and (131)I in the air particulate matter, show, in contrast to the Chernobyl discharge, a negligible input of stratospheric transport of Fukushima-released fission products.  相似文献   

20.
Opencast mining of uranium may lead to natural erosion of ore material due to overland flow of water accumulated from rainfall. The overland flow may ultimately reach the nearby surface water body. This process may lead to the release of 238U and its daughter products into the surface water body. A model is developed to assess the radiological impact of the erosion in terms of dose through drinking water pathway due to 238U and its progeny in the surface water body. The in-growth of progeny is taken into account using Bateman equations. The study brings out the importance of incorporating decay chain transport in the radiological impact assessment studies. It is also observed that 210Po, 210Pb, 226Ra, and 230Th together contribute to about 95.5 % of the total dose. The model is then extended to incorporate the uncertainty associated with the dose due to consumption of the reservoir water by employing Wilk’s Method. Such a model can be very useful in establishing regulations related to dose through drinking water pathway around an opencast mine. Wilk’s method is computationally less expensive as compared to the exact methods like Monte Carlo method. Wilk’s method is used to calculate a value greater than α percentile value for the dose to the public due to 238U and its progeny in the reservoir through drinking water pathway with confidence level β (α/β value). When applied to a hypothetical case using some literature data on surface water bodies, it is found that with increase in the value of α or β, the α/β value in general, shows an increasing trend as expected. Depending upon the nature of the problem under study, one can calculate an α/β value i.e. 95/95 value, 99/95 value etc., and that value can be helpful in establishing the regulatory limiting value. Also, the α/β value can be used to check whether dose due to a particular radioactive release is within the specified limits.  相似文献   

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