浙江省环保重点城市CO2排放的控制模式

通过分析城市ＳＯ２地面浓度来源，运用高、中、低架源对地面污染物浓度贡献的理论及高斯烟羽模式推出ＳＯ２空气质量管理模式，确定了城市ＳＯ２地面环境质量的控制目标。     

边界层顶垂直速度对大气污染物地面浓度的影响

本文把地形、地转涡度及埃克曼抽吸作用共同引起的垂直运动通过大气污染物的平流扩散方程,引入到大气扩散模式中来.并通过实例计算了地面轴线浓度及其最大地面浓度距离后发现:在有些情况下,这些要素引起的垂直运动对大气污染物的地面浓度影响是重要的.     

浙江省环保重点城市SO 2 排放的控制模式

通过分析城市SO2 地面浓度来源 ,运用高、中、低架源对地面污染物浓度贡献的理论及高斯烟羽模式推出SO2空气质量管理模式 ,确定了城市SO2 地面环境质量的控制目标。     

大气污染物排放调查监测研究进展

系统总结了当前大气污染物排放调查监测的主要方法及其在全球、区域、局地等不同尺度的典型应用，分析了地面监测、模型模拟与遥感反演3种方法受排放源多样、成分复杂、时空变异显著等因素影响，在尺度效应、成分解析等方面存在的问题。从优化监测方法、改进监测模式、融合监测技术等角度，提出了构建现代化大气污染物排放调查监测网络、开展污染物在不同排放阶段的变化解析研究及在不同圈层间的迁移全过程研究等建议。     

基于M apInfo的大气污染物复合多源模式研究及应用

研究了在MapInfp环境下的大气污染物复合多源模式，利用MapBasic编制了不同风向条件下的污染源坐标转换程序，同时利用Surfer软件绘制了污染物浓度等值线，并在MapInfo中与基础底图叠加。通过对某工业区SO2长期平均浓度的预测，证明复合多源模式在环境影响评价中具有很好的应用价值。     

丹东市二氧化硫叠加模式的研制及应用

采用《制定地方大气污染物排放标准的技术方法》(GB/T 3840-1991)中的高斯模式作为大气污染物地面浓度基本公式,计算丹东市区内任一点位上的点源排放SO2在下风向网格交叉点上的叠加浓度.采用点到直线的距离公式计算垂直于平均风向的水平横向距离和下风向距离,以丹东市采暖锅炉排放SO,为例计算多点源网格落地浓度.     

长株潭区域一次重度污染过程气象成因

利用PM_2.5质量浓度、地面气象要素、NCEP、ERSST＿V3、GBL等资料，研究了2021年12月7—11日长株潭地区一次重度空气污染过程的特征及成因。结果表明，高空平直环流、无明显槽脊影响，地面弱冷空气活跃是本次重度空气污染过程的主要环流形势特征；地面均压场、小风和升温增湿是此次重度空气污染过程的主要气象要素特征。污染物浓度变化与主导风向和污染通道密切相关，本地风速对混合层的高度、污染物水平扩散影响较大，600～700 hPa逆温层有利于污染物在主导风作用下近距离传输及在低层交换积累。我国中东部污染物积聚是长株潭区域重要的污染来源，长株潭地区存在区域性同步污染现象。低层流入长株潭区域气流轨迹差异及地理条件是长株潭污染物空间分布差异的重要因素。     

关于废水中污染物浓度日均值的思考

在环境污染防治工作从污染物浓度控制逐步向排污总量控制转变的过渡阶段中，污染物浓度日均值仍然发挥着十分重要的作用，文中阐述了日均值的监测时段、监测频率及计算方法等技术要求，并结合排污总量监测、提出了一些建议。     

一个监测和估算非均匀面源大气污染物排放速率的方法

目前对于无组织面源污染物排放量的估算 主要采用以下几种方法:①物料衡算法;②经验 估算法;③地面浓度反推法。     

对建立大气环境总量控制法规体系的思考

文中指出了《大气污染物综合排放标准》存在的不完善性，提出建立大气污染物总量控制制度，使大气污染物的控制由浓度控制转向总量与浓度结合的控制体系；建立大气污染物总量控制法规体系，规范排污行为．并阐述了大气污染物总量控制指标的技术路线。     

近地面NO_2浓度卫星遥感估算问题

对卫星遥感监测大气NO_2的差分算法涉及的科学问题进行了综述,包括去除大气散射和地表反射噪声影响、大气拉曼散射引起的Ring效应校正、不同大气成分分离和观测垂直归一化等问题。国际上通过剔除平流层NO_2获得对流层柱浓度产品,文章绕开平流层NO_2获取问题,提出了结合大气化学模式模拟的垂直廓线直接估算近地面NO_2浓度技术方法,以更好地满足环境空气质量的观测需求,阐述了几个影响NO_2反演精度的相关问题。     

A Generalized Analytical Model for Crosswind-Integrated Concentrations with Ground-Level Deposition in the Atmospheric Boundary Layer

A generalized mathematical model describing the crosswind-integrated concentrations is presented for dispersion of pollutants emitted from a continuous source in the atmospheric boundary layer with deposition to the ground surface. The model is based on a solution of the resulting two-dimensional steady state advection-diffusion equation with deposition to the ground surface. It considers the horizontal wind speed as a generalized function of vertical height above the ground surface and eddy diffusivity as a function of both downwind distance from the source and vertical height. Various special cases of the model are deduced. A sensitivity analysis of the model prediction of the ground-level crosswind-integrated concentrations with deposition velocity is performed. Various issues and limitations associated with this work are discussed. The model is evaluated with the observations of a depositing tracer obtained from Hanford dual diffusion experiment in stable conditions. The statistical measures show that the present model, by considering deposition, is performing well with the observations. The model is giving an over-predicting trend with the observations and predicts 100 % cases within a factor of two. On the other hand, the consideration of a non-depositing condition for a depositing tracer yields the severe over-prediction and thus, it introduces the significant errors in the model prediction. The selection of the lower boundary condition for a depositing tracer at the height of deposition surface gives better prediction than those at a height of surface roughness length.     

Source Release-Rate Estimation of Atmospheric Pollution from a Non-Steady Point Source at a Known Location

The goal is to build up an inverse model capable of finding the release history of atmospheric pollution by using measured gas concentration data at just one location on the ground and identify the factors which affects the accuracy of the model predictions. The problem involves a non-steady point source of pollution at a known location in the atmosphere. This problem of finding the release rate is an ill-posed inverse problem and its solution is extremely sensitive to errors in the measurement data. Special regularisation methods, which stabilise the process of the solution, must be used to solve the problem. The method described in this paper is based on linear least-squares regression and Tikhonov regularisation, coupled with the solution of an advection-diffusion equation for a non-steady point source. The accuracy of the method is examined by imposing normally-distributed relative noise into the concentration data generated by the forward model as well as some real experimental data.     

Study on the effect of porous fence on air quality and traffic noise level around a double-decked road structure

Fence for traffic noise control sometimes causes adverse effect on air pollution. Thus in this study, performance of porous fence as a tool for control of both air pollution and noise pollution was evaluated. A two-dimensional numerical model for flow and pollutant concentration and an analytical model for traffic noise were utilized in the analysis of a double-decked road structure with fences only at ground (Case 1) and at both ground and upper deck (Case 2). Porous fences were assumed only at the ground level since the solid fences at the upper deck usually leads to desirable result on air pollution. Effects of the variable porosity on air quality and noise level near road were evaluated. Obtained results showed: (1) flow pattern in leeward of fence was drastically changed at 40–50% porosity in Case 1 and 50% in Case 2. The porosity larger than 40% excluded presence of a circulation behind the fence. (2) Effect of porous fence on air pollution was different in Cases 1 and 2. In Case 1, the porous fence generally resulted in the reduction of air pollution at the ground level; on the other hand, in Case 2, it rather led to increase of the concentration. (3) Traffic noise level was also largely changed by the porosity of the fence; an example of simultaneous evaluation of the effects of porous fence on both air and noise pollution in Case 1 showed that the fence of 60% porosity leads to reduction of air pollution by 20% compared with solid fence case, and reduction of noise pollution by 4–6% in dB compared with no fence case, at l m high and 10 m from the road.     

Model Assessment of Air-Pollution in Prague

Results of relatively simple gaussian dispersion model are presented. This model, developed in the beginning of this decade, is suitable mainly for determination of spatial distributions of annual mean concentrations of such kinds of air-pollution as sulphur dioxide (SO₂), mixture of nitrogen oxides (NO_x) or suspended particulate matter (SPM) from all types of emission sources located within the city - point sources, line sources and area sources. Model has been used in years 1994, 1996 and 1998 to assess the air-pollution distributions of the above mentioned kinds in the Prague area and the development of the air quality state. It contributed to the decision making process when possible impact of some changes in traffic system or in system of domestic heating, for example, has been investigated. In this contribution, behaviour of sulphur dioxide (SO₂) and mixture of nitrogen oxides (NO_x) ground concentration distributions are analyzed with respect to changing emission situation in Prague in recent years. Results show that SO₂ ground concentration level decreases mainly due to changes in local heating methods and type of fuel used. Different trend can be seen in NO_x ground concentrations thanks to rapid increase in the traffic density.     

Fluorine distribution in aquatic environment and its health effect in the Western Region of the Songnen Plain, Northeast China

Endemic fluorosis was investigated and studied in the west region of the Songnen plain, Northeast China in 2001–2002. The results showed that the fluorine distribution in aquatic environment was that the fluorine concentrations in the lake water and unconfined ground water were higher than that in the river water and confined ground water. The lake water (Alkali lake) is connected with unconfined ground water. In unconfined ground water, from the east and southeast areas to the west and the northwest areas of the plain, fluorine concentration fluctuated with high and low alternatively. The fluorine in the water comes from the weathering of rocks and minerals in the mountains and hills around the Songnen Plain. The main influence factors of the fluorine distribution in aquatic environment are discussed. Unconfined ground water containing high fluorine is used as drinking water. In this region, the fluorine concentration in drinking water is evidently correlated to the morbidity of dental and skeletal fluorosis. High fluorine concentration in drinking water has endangered human health.     

点源扩散大气预测软件

建设项目的点源扩散大气预测软件,包括了<环境影响评价技术导则-大气环境>第三级评价有风时,静风和小风扩散模式;最大地面浓度Cm及其距排气筒的距离Xm模式;烟气抬升公式以及等值线点位值的计算功能.该软件运算快速、简便、准确.     

An assessment of fluoride in the coastal aquifer of the Bara tract in Bharuch district, Gujarat (India)

The fluoride (F) concentration in the coastal aquifers of Bara tract in Bharuch district, Gujarat was determined by potentiometric method using an ion-selective electrode. The fluoride concentration in these aquifers varies between 0.060 to 3.51 mg/L. It was also found that F has a positive correlation with pH and HCO(3)(-) whereas negatively correlated with Ca(2+), indicating that high fluoride in ground water is associated with low calcium content. This suggests that the higher pH of water promotes the leaching of fluoride and thus affects the concentration of fluoride in the ground water. It was also found that there exists no relationship between F, EC, and ground water table from surface in the ground water.     

某石化工业园区大气中VOCs垂直分布的无人机监测研究

利用无人机对某石化工业园区地面至100 m大气中的VOCs进行监测，通过不同高度数据对比，总结该石化工业园区挥发性有机物的垂直分布特征，并分析其化学反应活性。监测结果表明，VOCs体积分数和总臭氧生成潜势随高度增加均呈下降趋势，地面和15~30 m高度的VOCs浓度及臭氧生成潜势基本一致。主要VOCs物种浓度垂直分布特征可分为均匀分布、随高度增加浓度不断降低、随高度增加浓度先升后降3种。含氧有机物和烷烃在大气中体积分数较大，主要特征挥发性有机物为丙酮、乙醛、乙烷、乙醇等；臭氧生成潜势贡献较大的组分为含氧有机物、烯烃和炔烃，关键活性物质为甲醛、乙醛、丁烯醛、正丁醛等。含氧有机物的体积分数和臭氧生成潜势贡献在地面至100 m高度都明显高于其他组分，应作为VOCs浓度和化学活性控制的重点。     

Physical Modeling of Emissions from Naturally Ventilated Underground Parking Garages

The dispersion of pollutants from naturally ventilated underground parking garages has been studied in a boundary layer wind tunnel. Two idealized model setups have been analysed, one was simulating pollutant dispersion around an isolated rectangular building and one was representing dispersion in a finite array of idealized building blocks. Flow and dispersion close to modelled ground level emission sources was measured. The results illustrate the complexity of the flow around buildings and provide insight in pollutant transport from ground level sources located directly on building surfaces. As a result, areas critical with respect to high pollutant concentrations could be visualized. Particularly, the results show high concentration gradients on the surface of the buildings equipped with modelled emission sources. Inside the boundary layers on the building walls, a significant amount of pollutants is transported to upwind locations on the surface of the building. The paper documents the potential of physical modelling to be used for the simulation and measurement of dispersion close to emission sources and within complex building arrangements.