Evaluation of fast atmospheric dispersion models in a regular street network

Environmental Fluid Mechanics - The need to balance computational speed and simulation accuracy is a key challenge in designing atmospheric dispersion models that can be used in scenarios where...     

A new view of dispersion in well-mixed estuaries

A two-dimensional simulation of Delaware estuary hydrodynamics has been constructed. This simulation has been achieved through a rational estimate of the character of natural turbulence. Non-homogeneous velocities, on the cross-section, are employed in two-dimensional, laterally homogeneous species mass balances. In turn, concentration profiles are interpreted in the form of classical, one-dimensional dispersion coefficients. Variation of dispersion as a function of both freshwater inflow and longitudinal distance was generated. Variation of dispersion in time within a tidal cycle was found to be insignificant while no significant variation from one tidal cycle to the next has been detected.The modeling process involves the solution of tractable equations by implicit numerical methods and is capable of being excited by a wide range of input conditions.A study of the sensitivity of dispersion due to vertical mass diffusion revealed that longitudinal mixing characteristics are inversely proportional to vertical eddy diffusivity and analysis of the numerical results showed the dispersion coefficient is essentially insensitive to variation of longitudinal mass diffusivity. This leads to the conclusion that turbulent diffusivity of mass in the longitudinal direction may be taken as constant for most purposes in the study of a two-dimensional species mass balance model.A field program was carried out near the Delaware Memorial Bridge to collect velocity profiles. Substantial portions of the scheme have been verified (i.e. one- and two-dimensional tidal dynamic models) through the use of these data.     

Large-eddy simulation of turbulent flow and dispersion over a complex urban street canyon

Turbulent flow and dispersion characteristics over a complex urban street canyon are investigated by large-eddy simulation using a modified version of the Fire Dynamics Simulator. Two kinds of subgrid scale (SGS) models, the constant coefficient Smagorinsky model and the Vreman model, are assessed. Turbulent statistics, particularly turbulent stresses and wake patterns, are compared between the two SGS models for three different wind directions. We found that while the role of the SGS model is small on average, the local or instantaneous contribution to total stress near the surface or edge of the buildings is not negligible. By yielding a smaller eddy viscosity near solid surfaces, the Vreman model appears to be more appropriate for the simulation of a flow in a complex urban street canyon. Depending on wind direction, wind fields, turbulence statistics, and dispersion patterns show very different characteristics. Particularly, tall buildings near the street canyon predominantly generate turbulence, leading to homogenization of the mean flow inside the street canyon. Furthermore, the release position of pollutants sensitively determines subsequent dispersion characteristics.     

Large eddy simulation of plume dispersion behind an aircraft in the take-off phase

The aim of this paper is to provide an investigation, using large eddy simulation, into plume dispersion behind an aircraft in co-flowing take-off conditions. Validation studies of the computational model were presented by Aloysius and Wrobel (Environ Model Softw 24:929–937, 2009) and a study of the flow and dispersion properties of a double-engine aircraft jet was presented by Aloysius et al. (EEC/SEE/2007/001, EUROCONTROL Experimental Centre, ), in which only the engine was modelled. In this paper, the complete geometry of a Boeing 737 is modelled and investigated. The current work represents a contribution towards a better understanding of the source dynamics behind an airplane jet engine during the take-off and landing phases. The information provided from these simulations will be useful for future improvements of existing dispersion models.     

Lagrangian models of dispersion in marine environment

Turbulent dispersion can be studied successfully by using Lagrangian particle models. In general, the prediction of correct concentration fields is a complex issue when the turbulent field is inhomogeneous and non-stationary. Two classes of Lagrangian dispersion models have been considered in this work, which are based on the Wiener process and the so called “well-mixed” criterion. In order to test the performances of these models and shed light on the underlying physical processes and modeling assumptions, four different numerical models have been compared and tested by means of their long time behavior by considering several study cases concerning idealized marine environment. Furthermore, the coupling of the community model Princeton Ocean Model (POM) with the Lagrangian model LASEMOD (LAgrangian SEa MODel) is used to investigate the temporal and spatial evolution of a passive pollutant released in the vicinity of the coast in the Tyrrhenian Sea basin. The simulation shows with reasonable accuracy the time evolution of both the hydrodynamic and the concentration fields and provides a useful insight into the evaluation of the environmental impact of pollutant releases along the coast.     

Simple elimination models: Theoretical estimates of the effect of variations in elimination rates

This paper analyses the effect of variations in the elimination rates of four elimination models. Three types of variations are studied: (1) a periodic change between two elimination rates; (2) changes between two elimination rates at random times; and (3), an elimination rate varying smoothly in time, generated by having the elimination rate vary exponentially with temperature and a sinusoidally varying temperature. The elimination process is described by four different models: (1) a single compartment; (2) two compartments in parallel; (3) two compartments in series; and (4) the Goldstein-Elwood model. It is shown that for all 12 cases, the solutions can be given the same form as with constant elimination rates through reinterpretation of the parameters. As a special case, the use of elimination methods to estimate respiration is discussed and a possible source of error is pointed out.     

Comparison of atmospheric modelling systems simulating the flow,turbulence and dispersion at the microscale within obstacles

Three different modelling techniques to simulate the pollutant dispersion in the atmosphere at the microscale and in presence of obstacles are evaluated and compared. The Eulerian and Lagrangian approaches are discussed, using RAMS6.0 and MicroSpray models respectively. Both prognostic and diagnostic modelling systems are considered for the meteorology as input to the Lagrangian model, their differences and performances are investigated. An experiment from the Mock Urban Setting Test field campaign observed dataset, measured within an idealized urban roughness, is used as reference for the comparison. A case in neutral conditions was chosen among the available ones. The predicted mean flow, turbulence and concentration fields are analysed on the basis of the observed data. The performances of the different modelling approaches are compared and their specific characteristics are addressed. Given the same flow and turbulence input fields, the quality of the Lagrangian particle model is found to be overall comparable to the full-Eulerian approach. The diagnostic approach for the meteorology shows a worse agreement with observations than the prognostic approach but still providing, in a much shorter simulation time, fields that are suitable and reliable for driving the dispersion model.     

Modelling of turbulent dispersion for numerical simulation of wind-driven rain on bridges

Wind-driven rain (WDR) is responsible for many potential negative effects on bridges, such as structural cracking, aggregate erosion, steel corrosion and storm water management problems and so on. Hence, accurate evaluations of the WDR effects on bridges are essential to provide solutions for preventing material degradation and improving durability capability of bridges. However, in most previous WDR numerical studies, the turbulent dispersion of raindrops was neglected. In this paper, the turbulent dispersion is integrated into Eulerian multiphase model to investigate the WDR effects on a bridge with rectangular cross-section. Especially, the influences of the turbulent dispersion are discussed in detail by comparing the WDR simulation results for the cases with and without consideration of the turbulent dispersion in terms of WDR flow fields, volume fraction, specific catch ratio, catch ratio, rain loads and aerostatic force coefficients. The results indicate that the turbulent dispersion for a certain range of raindrop size is needed to be taken into account for obtaining accurate WDR simulation results for bridges.     

重气连续泄漏扩散的盐水模拟实验

根据相似理论,分析了用盐水模拟方法研究意外泄漏的重气在大气中扩散过程的可行性,通过假设重气为不可压缩气体以及在均匀温度场中扩散等条件,推导出模拟实验的准则数.采用缩比模型的盐水模拟实验,对重气在大气中的扩散速度及浓度变化进行了分析,证实了重气扩散过程中的重力沉降、密度分层以及近源区分叉等现象.实验表明,在满足主导准则数相等的条件下,盐水在清水中的扩散可以较好地再现重气在大气中的扩散特征.     

不同结构形状的街道峡谷内污染物扩散

针对不同的城市街道峡谷结构形状,通过求解二维不可压缩N-S方程和K-ε湍流模型方程及污染物对流扩散方程,数值模拟了街道峡谷内的流场及机动车排放污染物浓度场,从而说明了街道峡谷的结构是影响街道峡谷内污染气体扩散的主要因素之一。     

Three-Dimensional Modelling of Concentration Fluctuations in Complicated Geometry

The strong fluctuating component in the measured concentration time series of a dispersing gaseous pollutant in the atmospheric boundary layer, and the hazard level associated to short-term concentration levels, demonstrate the necessity of calculating the magnitude of turbulent fluctuations of concentration using computational simulation models. Moreover the computation of concentration fluctuations in cases of dispersion in realistic situations, such as built-up areas or street canyons, is of special practical interest for hazard assessment purposes. In this paper, the formulation and evaluation of a model for concentration fluctuations, based on a transport equation, are presented. The model is applicable in cases of complex geometry. It is included in the framework of a computational code, developed for simulating the dispersion of buoyant pollutants over complex geometries. The experimental data used for the model evaluation concerned the dispersion of a passive gas in a street canyon between 4 identical rectangular buildings performed in a wind tunnel. The experimental concentration fluctuations data have been derived from measured high frequency concentrations. The concentration fluctuations model is evaluated by comparing the model's predictions with the observations in the form of scatter plots, quantile-quantile plots, contour plots and statistical indices as the fractional bias, the geometrical mean variance and the factor-of-two percentage. From the above comparisons it is concluded that the overall model performance in the present complex geometry case is satisfactory. The discrepancies between model predictions and observations are attributed to inaccuracies in prescribing the actual wind tunnel boundary conditions to the computational code.     

Verification of the plume rise/dispersion model USPR: plume rise for single stack emissions

Despite proliferation of the use of air pollution models for regulatory application, major discrepancies still occur between models and also between models and observations, especially when oversimplistic models are used. The problem of predicting plume rise (and subsequently ground level concentrations) from a single source is evaluated here in terms of an integral plume rise and dispersion model (USPR) which encompasses both bouyant rise and turbulent spreading; thus avoiding the problems of the concatenation of separate plume rise and dispersion models. The wide range of validity of the USPR model is demonstrated is terms of plume rise by comparison with the highly buoyant GCOS and Kincaid plumes as well as with dense effluents. It is also shown to be in agreement with Briggs' two-thirds law when the restrictions applicable to the latter model are imposed.     

Simulating property exchange in estuarine ecosystem models at ecologically appropriate scales

A computational scheme has been developed and tested to simulate property exchange by advection and dispersion in estuaries at time and space scales that are well suited to ecological and management simulations, but are coarse relative to the demands of physical hydrodynamic models. An implementation of the Regional Ocean Model System (ROMS) for the Providence River and Narragansett Bay (RI, USA) was used to determine property exchanges between the spatial elements of an ecological box model. The basis for the method is the statistical tabulation of numerical dye experiments done with the full ROMS physical model. The ROMS model domain was subdivided into fifteen coarse boxes, each with two vertical layers, defining 30 elements that were used for the box model simulations. Dye concentrations were set to arbitrary initial concentrations for all ROMS grids in the large elements, and the ROMS model was run for 24 h. The final distribution of the dye among the elements was used as a tracer for property exchange over that day and was used to develop an exchange matrix. Box model predictions of salinity over 77 days in each element compared favorably with ROMS simulated salinity averaged over the same spatial elements, although the disparity was greater in areas where large river inflows caused strong gradients in ROMS within elements assumed to be homogeneous in the box model. The 77-day simulation included periods of high and low river flow. Despite the large size of the spatial elements, dispersion artifacts were small, much less than the modeled daily exchanges. While others have taken a similar approach, we found a number of theoretical and practical considerations deserved careful attention for this approach to perform satisfactorily. Whereas the full ROMS model takes 9 days on a powerful computing cluster to compute the physics simulation for 77 days, the box model simulates physics and biology for the same interval in 5 s on a personal computer, and a full year in under 1 min. The exchange matrix mixing model is a fast, cost effective, and convenient way to simulate daily variation of complex estuarine physics in ecological modeling at appropriate scales of space and time.     

BP-4的模拟生物降解特性研究

为研究紫外吸收剂2-羟基-4-甲氧基二苯甲酮-5-磺酸(BP-4)的最大生物降解能力,采用欧洲经济合作与发展组织(OECD)生物降解测试标准方法——303A模拟试验-污水好氧处理:活性污泥单元法,建立并进行了城市污水处理厂曝气池环境模拟试验。研究结果表明:在单一新鲜活性污泥作为接种物条件下,BP-4在第47天达到降解稳定期,溶解性有机碳(DOC)去除率平均值为36.90%±5.68%(n=18)。在以10种不同来源混合接种物条件下,BP-4在第41天达到降解稳定期,去除率平均值为33.11%±4.87%(n=17)。研究结果表明BP-4在环境中的降解能力有限,在本模拟方法试验条件下只能部分降解。     

Photodegradation of fungicide triadimefon and pesticide pirimicarb in aqueous TIO2 suspension

Two agrochemicals composed of nitrogen‐containing heterocyclic ring, triadimefon and pirimicarb, were degraded photocatalytically. The disappearance and TOC elimination rates of triadimefon were close to those of pirimicarb, whereas the photolysis of triadimefon was 4 times slower than that of pirimicarb. For triadimefon its aromatic moiety degraded quickly and Cl^‐ was released immediately, while triazole moiety degraded slowly. The formation rates of NH⁺ ₄ and NO₃ ^‐ by the degradation of triazole moiety were influenced by the rest of the molecule. The difference between disappearance and TOC elimination rates of both triadimefon and pirimicarb were far larger than those of aromatic compounds.     

Chemical Tracking and Marine Environmental Impact of Ocean Disposal of Calcium Carbonate Residue in the North Yellow Sea

The objective of this study is to determine the sedimentation rate and dispersion area of calcium carbonate residue dumped at sea and the impact to marine environment of dumping by a laboratory simulation experiment; chemical tracking in the field with the help of acoustic and optical tracking; and a comparative study of baseline conditions and marine environmental impact after dumping. Turbidity, pH and phosphate are selected as the chemical tracers to be monitored.

Results show that in the dumping area of 15 square miles with water depth of 50 m, if 217 t calcium carbonate residue is dumped (spot dumping) in the presence of a pycnocline with a current velocity of 60 cm/s (close to the maximum) the maximum dispersion distance of the calcium carbonate residue plume front is less than 2100 m; the dispersion area is less than 0.56 km²; and the maximum dispersion time is about 60 min when the turbidity and pH in the whole dispersion area return to background level. Therefore, the ocean disposal of calcium carbonate residue is feasible.     

Traps and transformations influencing the financial viability of tourism on private‐land conservation areas

The ability of private conservation organizations to remain financially viable is a key factor influencing their effectiveness. One‐third of financially motivated private‐land conservation areas (PLCAs) surveyed in South Africa are unprofitable, raising questions about landowners’ abilities to effectively adapt their business models to the socioeconomic environment. In any complex system, options for later adaptation can be constrained by starting conditions (path dependence). We tested 3 hypothesized drivers of path dependence in PLCA ecotourism and hunting business models: (H1) the initial size of a PLCA limits the number of mammalian game and thereby predators that can be sustained; (H2) initial investments in infrastructure limit the ability to introduce predators; and (H3) rainfall limits game and predator abundance. We further assessed how managing for financial stability (optimized game stocking) or ecological sustainability (allowing game to fluctuate with environmental conditions) influenced the ability to overcome path dependence. A mechanistic PLCA model based on simple ecological and financial rules was run for different initial conditions and management strategies, simulating landowner options for adapting their business model annually. Despite attempts by simulated landowners to increase profits, adopted business models after 13 years were differentiated by initial land and infrastructural assets, supporting H1 and H2. A conservation organization's initial assets can cause it to become locked into a financially vulnerable business model. In our 50‐year simulation, path dependence was overcome by fewer of the landowners who facilitated natural ecological variability than those who maintained constant hunting rates and predator numbers, but the latter experienced unsustainably high game densities in low rainfall years. Management for natural variability supported long‐term ecological sustainability but not shorter term socioeconomic sustainability for PLCAs. Our findings highlight trade‐offs between ecological and economic sustainability and suggest a role for governmental support of the private conservation industry.     

Chemical Tracking and Marine Environmental Impact of Ocean Disposal of Calcium Carbonate Residue in the North Yellow Sea

The objective of this study is to determine the sedimentation rate and dispersion area of calcium carbonate residue dumped at sea and the impact to marine environment of dumping by a laboratory simulation experiment; chemical tracking in the field with the help of acoustic and optical tracking; and a comparative study of baseline conditions and marine environmental impact after dumping. Turbidity, pH and phosphate are selected as the chemical tracers to be monitored.

Results show that in the dumping area of 15 square miles with water depth of 50 m, if 217 t calcium carbonate residue is dumped (spot dumping) in the presence of a pycnocline with a current velocity of 60 cm/s (close to the maximum) the maximum dispersion distance of the calcium carbonate residue plume front is less than 2100 m; the dispersion area is less than 0.56 km²; and the maximum dispersion time is about 60 min when the turbidity and pH in the whole dispersion area return to background level. Therefore, the ocean disposal of calcium carbonate residue is feasible.