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1.
An analysis of sporocarps of ectomycorrhizal fungi Suillus variegatus assessed whether cesium (133Cs and 137Cs) uptake was correlated with potassium (K) or rubidium (Rb) uptake. The question was whether intraspecific correlations of Rb, K and 133Cs mass concentrations with 137Cs activity concentrations in sporocarps were higher within, rather than among, different fungal species, and if genotypic origin of sporocarps within a population affected uptake and correlation. Sporocarps (n = 51) from a Swedish forest population affected by the fallout after the Chernobyl accident were studied. The concentrations were 31.9 ± 6.79 g kg−1 for K (mean ± SD, dwt), 0.40 ± 0.09 g kg−1 for Rb, 8.7 ± 4.36 mg kg−1 for 133Cs and 63.7 ± 24.2 kBq kg−1 for 137Cs. The mass concentrations of 133Cs correlated with 137Cs activity concentrations (r = 0.61). There was correlation between both 133Cs concentrations (r = 0.75) and 137Cs activity concentrations (r = 0.44) and Rb, but the 137Cs/133Cs isotopic ratio negatively correlated with Rb concentration. Concentrations of K and Rb were weakly correlated (r = 0.51). The 133Cs mass concentrations, 137Cs activity concentrations and 137Cs/133Cs isotopic ratios did not correlate with K concentrations. No differences between, within or, among genotypes in S. variegatus were found. This suggested the relationships between K, Rb, 133Cs and 137Cs in sporocarps of S. variegatus is similar to other fungal species.  相似文献   

2.
Motivated by the detection of 131I in river sediment in routine long-term surveillance samples, a systematic short-term study of the wastewater treatment chain was planned and conducted. Inflow, effluent and primary sludge were collected on a daily basis during two weeks at a regional wastewater treatment plant. Samples were investigated by gamma spectroscopy. Four medically used isotopes could be identified (131I and 99mTc regularly, 153Sm and 123I sporadically). The concentration levels coincide well with literature data for 131I, and with our own long-term data for 131I and 99mTc for the same plant. Cosmogenic 7Be activity in primary sludge correlated well with rainfall intensity. Surface sediment was sampled at low tide at both shores of the river, up- and downstream of the plant. 131I was identified in all samples, with a sharp maximum (about 100 Bq kg−1 d.m.) at the discharge point of the plant and lower levels elsewhere, decreasing monotonically in downstream direction. 7Be and 137Cs showed the same behaviour, but no peak at the discharge point. Predictions from simple equilibrium models for the transport and sedimentation of 131I show good agreement with the experimental data and suggest that the wastewater treatment plant is the main source for this isotope.  相似文献   

3.
We investigated the vertical profiles of 239+240Pu, 137Cs, and excess 210Pb (210Pbex) in sediment core samples obtained from two freshwater lakes and two brackish lakes situated near the first commercial spent nuclear fuel reprocessing plant in Rokkasho, Japan, before the final test of the plant using actual spent nuclear fuel. The inventory of 239+240Pu in those lakes was larger than that in soil in Rokkasho, which indicated the inflow of 239+240Pu from the catchment area in addition to direct deposition on the lake surfaces. The 137Cs inventory in sediments of the brackish lakes was lower than that in the soil, which showed that part of the 137Cs was removed from the sediments by the brackish water or that it was not deposited into the sediments, because of the high solubility of Cs in brackish water. The 137Cs inventory in sediments of the freshwater lakes was higher than that of the brackish lakes, and comparable with that in soil except for one core sample out of four. The 239+240Pu/137Cs ratio in freshwater lake sediments was higher than that in soil, and that indicated that part of the 137Cs was lost from the sediments. The low inventory of 137Cs may be attributable to competition for absorption sites in sediments with ammonium ions formed in the reducing environment which occurs from summer to fall in the sediments. Those data will be used as background data on the artificial radionuclides in the lakes to assess the effect of released radionuclides on their concentrations.  相似文献   

4.
Samples of summer pasture plants that reindeer feed on were collected in order to study 137Cs concentrations in different plant species and in species nested in certain site types, and to study the regional distribution of 137Cs in the Finnish reindeer management area. Plant species were categorized by the site types of mineral soil forest (xeric heath forest and mesic heath forest) and peatland. A third category called ’other plant species’ included plants with various site types, poorly determined species and species with poor statistics. The 137Cs concentrations in different site types differed significantly. The mean 137Cs concentrations of the whole reindeer management area in the xeric heath forest plant species was 44 ± 27 Bq/kg dw, in the mesic heath forest plant species 75 ± 59 Bq/kg dw and in the peatland plant species 219 ± 150 Bq/kg dw. The peatland species uptake 137Cs more efficiently than plant species of mineral soil forests. A particularly efficient collector of 137Cs was Trichophorum sp. It is suggested that Trichophorum sp. could be used as an indicator species for reindeer summer fodder plants. The highest concentrations of 137Cs were found in Southern Lapland and the lowest in Northern Lapland. Today, the concentrations of 137Cs in summer pasture plants that reindeer feed on in Finland are at such a level that there is no need to avoid any plant species. In the case of future nuclear fallout, reindeer grazing in peatlands would increase concentrations of 137Cs in reindeer meat.  相似文献   

5.
A sediment core collected from the sub-aqueous delta of the Yangtze River estuary was subjected to analyses of 137Cs and plutonium (Pu) isotopes. The 137Cs was measured using γ-spectrometry at the laboratories at the Nanjing University and Pu isotopes were determined with Accelerator Mass Spectrometry (AMS), measurements made at the Australian National University. The results show considerable structure in the depth concentration profiles of the 137Cs and 239+240Pu. The shape of the vertical 137Cs distribution in the sediment core was similar to that of the Pu. The maximum 137Cs and 239+240Pu concentrations were 16.21 ± 0.95 mBq/g and 0.716 ± 0.030 mBq/g, respectively, and appear at same depth. The average 240Pu/239Pu atom ratio was 0.238 ± 0.007 in the sediment core, slightly higher than the average global fallout value. The changes in the 240Pu/239Pu atom ratios in the sediment core indicate the presence of at least two different Pu sources, i.e., global fallout and another source, most likely close-in fallout from the Pacific Proving Grounds (PPG) in the Marshall Islands, and suggest the possibility that Pu isotopes are useful as a geochronological tool for coastal sediment studies. The 137Cs and 239+240Pu inventories were estimated to be 7100 ± 1200 Bq/m2 and 407 ± 27 Bq/m2, respectively. Approximately 40% of the 239+240Pu inventory originated from the PPG close-in fallout and about 50% has derived from land-origin global fallout transported to the estuary by the river. This study confirms that AMS is a useful tool to measure 240Pu/239Pu atom ratio and can provide valuable information on sedimentary processes in the coastal environment.  相似文献   

6.
The present study was conducted to compare the 137Cs, 40K, 232Th, and 238U activity concentrations in epigeic moss (Hypnum cupressiforme) and lichen (Cladonia rangiformis). The activity levels in 37 moss and 38 lichen samples collected from the Marmara region of Turkey were measured using a gamma spectrometer equipped with a high purity germanium (HPGe) detector. The activity concentrations of 137Cs, 40K, 232Th, and 238U in the moss samples were found to be in the range of 0.36-8.13, 17.1-181.1, 1.51-6.17, and 0.87-6.70 Bq kg−1 respectively, while these values were below detection limit (BDL)-4.32, 16.6-240.0, 1.32-6.47, and BDL-3.57 Bq kg−1 respectively in lichen. The average moss/lichen activity ratios of 137Cs, 40K, 232Th, and 238U were found to be 1.32 ± 0.57, 2.79 ± 1.67, 2.11 ± 0.82, and 2.19 ± 1.02, respectively. Very low 137Cs concentrations were observed in moss and lichen samples compared to soil samples collected from the same locations in a previous study. Seasonal variations of the measured radionuclide activities were also examined in the three sampling stations.  相似文献   

7.
Fukushima fallout in Northwest German environmental media   总被引:1,自引:0,他引:1  
Traces of short- and long-lived fallout isotopes (131I, 134Cs and 137Cs) were found in environmental samples collected in Northwest Germany (rain water, river sediment, soil, grass and cow milk) from March to May 2011, following the radioactivity releases after the nuclear accident in Fukushima, Japan. The measured concentrations are consistent with reported concentrations in air, amount of rainfall and expected values applying simple radioecological models. The [134Cs]/[137Cs] ratio reported for air (about 1) allows for discrimination between “recent” and “old” 137Cs. Expected 136Cs values fell below the detection limits of the instrumentation, despite large sample masses and long counting times.  相似文献   

8.
We summarize the patterns of 137Cs activity concentrations and transfer into fish and other biota in four small forest lakes in southern Finland during a twenty-year period following the Chernobyl accident in April 1986. The results from summer 1986 showed fastest accumulation of 137Cs into planktivorous fishes, i.e. along the shortest food chains. Since 1987, the highest annual mean values of 137Cs have been recorded in fish occupying the highest trophic levels, for perch (Perca fluviatilis) 13,600 Bq/kg (ww) and for pike (Esox lucius) 20,700 Bq/kg (ww). At the same time, activity concentrations of 137Cs in crustacean zooplankton and Asellus aquaticus have ranged between 1000 and 19,500 Bq/kg (dw). In 2006, 5-28% of the 1987 137Cs activity concentration levels were still present in perch and pike. Since 1989 their 137Cs activity concentrations in oligohumic seepage lakes have remained significantly higher than in polyhumic drainage lakes due to the increased transfer of 137Cs into fish in the seepage lakes with lower electrolyte concentrations, longer water retention times and lower sedimentation rate.  相似文献   

9.
Anthropogenic radionuclides in seawater have been used as transient tracers of processes in the marine environment. Especially, plutonium in seawater is considered to be a valuable tracer of biogeochemical processes due to its particle-reactive properties. However, its behavior in the ocean is also affected by physical processes such as advection, mixing and diffusion. Here we introduce Pu/137Cs ratio as a proxy of biogeochemical processes and discuss its trends in the water column of the North Pacific Ocean. We observed that the 239,240Pu/137Cs ratio in seawater exponentially increased with increasing depth (depth range: 100–1000 m). This finding suggests that the profiles of the 239,240Pu/137Cs ratios in shallower waters directly reflect biogeochemical processes in the water column. A half-regeneration depth deduced from the curve fitting the observed data, showed latitudinal and longitudinal distributions, also related to biogeochemical processes in the water column.  相似文献   

10.
The vertical distribution of 137Cs activity in peat soil profiles and 137Cs activity concentration in plants of various species was studied in samples collected at two sites on a raised bog in central Sweden. One site (open bog) was in an area with no trees and only a few sparsely growing plant species, while the other (low pine) was less than 100 m from the open bog site and had slowly growing Scots pine, a field layer dominated by some ericaceous plants and ground well-covered by plants. The plant samples were collected in 2004–2007 and were compared with samples collected in 1989 from the same open bog and low pine sites. Ground deposition of 137Cs in 2005 was similar at both sites, 23?000 Bq m−2. In the open bog peat profile it seems to be an upward transport of caesium since a clear peak of 137Cs activity was found in the uppermost 1–4 cm of Sphagnum layers, whereas at the low pine site 137Cs was mainly found in deeper (10–12 cm) layers. The migration rate was 0.57 cm yr−1 at the open bog site and the migration centre of 137Cs was at a depth of 10.7, while the rate at the low pine site was 0.78 cm yr−1 and the migration centre was at 14.9 cm. Heather (Calluna vulgaris) was the plant species with the highest 137Cs activity concentrations at both sites, 43.5 k Bq−1 DM in 1989 decreasing to 20.4 in 2004–2007 on open bog and 22.3 k Bq kg−1 DM in 1989 decreasing to 11.2 k Bq−1 DM by the period 2004–2007 on the low pine site. 137Cs transfer factors in plants varied between 0.88 and 1.35 on the open bog and between 0.48 and 0.69 m2 kg−1 DM at the low pine site.  相似文献   

11.
Liming of lakes is considered one possible remedial action to reduce the accumulation of radionuclides into fish in the case of a radiological accident. These responses were tested in field conditions in a small acidified lake that was divided into two parts: one limed with CaCO3 and the other half left as an unlimed control. The transfer of 90Sr from water into fish decreased on average by 50% during the first year after liming. However, at the same time the 90Sr concentration in water increased, reaching a maximum within 6 months after liming. Approximately 50% more 90Sr was detected in water in the limed part of the lake than on control side during the first year. 90Sr was most probably released from the sediment as the Ca concentration and pH of the water increased. As a result of these two processes, which counterbalanced each other (increased release of 90Sr into water from sediment and decreased transfer of 90Sr from water into fish), the 90Sr concentration in fish did not notably differ between the limed and control sides of the lake. Liming may only be suitable as a remedial action if carried out immediately after a radiological accident, before significant amounts of radionuclides have been deposited in lake sediments. In the case of 137Cs, the effect of liming was less pronounced. 137Cs activity concentration in water increased in the first year by 20% and uptake by fish decreased by 20%.  相似文献   

12.
A microcosm laboratory experiment was conducted to determine the impact of biological reworking by the ragworm Nereis diversicolor on the redistribution of particle-bound radionuclides deposited at the sediment-water interface. Over the course of the 40-day experiment, as much as 35% of a 137Cs-labelled particulate tracer deposited on the sediment surface was redistributed to depths of up to 11 cm by the polychaete. Three different reworking models were employed to model the profiles and quantify the biodiffusion and biotransport coefficients: a gallery-diffuser model, a continuous sub-surface egestion model and a biodiffusion model. Although the biodiffusion coefficients obtained for each model were quite similar, the continuous sub-surface egestion model provided the best fit to the data. The average biodiffusion coefficient, at 1.8 ± 0.9 cm2 y−1, is in good agreement with the values quoted by other workers on the bioturbation effects of this polychaete species. The corresponding value for the biotransport coefficient was found to be 0.9 ± 0.4 cm y−1. The effects of non-local mixing were incorporated in a model to describe the temporal evolution of measured 99Tc and 60Co radionuclide sediment profiles in the eastern Irish Sea, influenced by radioactive waste discharged from the Sellafield reprocessing plant. Reworking conditions in the sediment column were simulated by considering an upper mixed layer, an exponentially decreasing diffusion coefficient, and appropriate biotransport coefficients to account for non-local mixing. The diffusion coefficients calculated from the 99Tc and 60Co cores were in the range 2-14 cm2 y−1, which are consistent with the values found by other workers in the same marine area, while the biotransport coefficients were similar to those obtained for a variety of macrobenthic organisms in controlled laboratories and field studies.  相似文献   

13.
In this paper the inventory of 90Sr in 34 points distributed along the Spanish peninsular territory is presented. Obtained values range between 173 Bq/m2 and 2047 Bq/m2. From these data set and those 137Cs data obtained in a previous work the 137Cs/90Sr activity ratio has been established, laying this value between 0.9 and 3.6. Also the migration depth of both radionuclides has been analysed obtaining for 137Cs an average value 57% lower than that obtained for 90Sr.Additionally, this paper presents the results obtained in 11 sampling points in which the activity vertical profile has been measured. These profiles have been analysed to state the behaviour of strontium in soils and after, by using a convective-diffusive model, the parameters of the model which governs the vertical migration of 90Sr in the soil, v (apparent convection velocity) and D (apparent diffusion coefficient) have been evaluated. Mean values obtained are 0.20 cm/year and 3.67 cm2/year, respectively.  相似文献   

14.
Discharges of the nuclides 129I, 137Cs and 99Tc from the nuclear reprocessing facilities at Sellafield (UK) and La Hague (France) are very useful as oceanic tracers. On the basis of 129I/127I, 137Cs and 99Tc measurements in archived seaweeds, the ratios of 129I/127I, 129I/137Cs and 129I/99Tc have been estimated in seawater at two locations (Utsira and Kiberg) in the Norwegian Coastal Current from 1980 to 1998. These ratios, which vary up to two orders of magnitude over this period, are potentially very interesting for determining "transit times" in the Arctic and North Atlantic oceans. While the long-term trends in these ratios are quite clear, measurements in monthly and bimonthly samples show considerable structure. Further studies are required to determine the exact origin of this structure, which may be a limiting factor in the time resolution that can be obtained with these parameters.  相似文献   

15.
Increasing use of wood fuels for energy production in Finland since the 1990s implies that large quantities of the generated ashes will be available for forest fertilization. The aim of this study was to analyse the effect of wood ash application on 137Cs activity concentrations in Scots pine (Pinus sylvestris L.) needles and certain berries and mushrooms on drained peatlands. The study was based on field experiments carried out on two mires in Finland in 1997-1998. Two different types of wood ash were applied at dosages of 3500, 3700, 10 500 and 11 100 kg ha−1. Wood ash did not increase 137Cs activity concentration in plants in the second growing season following application. On the contrary, a decrease in 137Cs activity concentration was seen in the plants of the ecosystem on drained peatlands. This result is of importance, for instance, when recycling of ash is being planned.  相似文献   

16.
Migration of 137Cs and 90Sr in undisturbed soil was studied in large lysimeters three and four years after contamination, as part of a larger European project studying radionuclide soil–plant interactions. The lysimeters were installed in greenhouses with climate control and contaminated with radionuclides in an aerosol mixture, simulating fallout from a nuclear accident. The soil types studied were loam, silt loam, sandy loam and loamy sand. The soils were sampled to 30–40 cm depth in 1997 and 1998. The total deposition of 137Cs ranged from 24 to 45 MBq/m2, and of 90Sr from 23 to 52 MBq/m2. It was shown that migration of 137Cs was fastest in sandy loam, and of 90Sr fastest in sandy loam and loam. The slowest migration of both nuclides was found in loamy sand. Retention within the upper 5 cm was 60% for both 137Cs and 90Sr in sandy loam, while in loamy sand it was 97 and 96%, respectively. In 1998, migration rates, calculated as radionuclide weighted median depth (migration centre) divided by time since deposition were 1.1 cm/year for both 137Cs and 90Sr in sandy loam, 0.8 and 1.0 cm/year, respectively, in loam, 0.6 and 0.8 cm/year in silt loam, and 0.4 and 0.6 cm/year for 137Cs and 90Sr, respectively, in loamy sand. A distinction is made between short-term migration, caused by events soon after deposition and less affected by soil type, and long-term migration, more affected by e.g. soil texture. Three to four years after deposition, effects of short-term migration is still dominant in the studied soils.  相似文献   

17.
In this study the total activity of 137Cs deposited per unit area over the Spanish peninsular territory was analysed using a 150 × 150 km2 mesh grid, with samples taken from 29 points. The deposited activities ranged between 251 and 6074 Bq/m2. A linear relationship was obtained between these values and the mean annual rainfall at each sampling point which allowed a map to be drawn, using GIS software, which shows the distribution of total deposited 137Cs activity across the Spanish mainland. At twelve of these sampling points the vertical migration profile of 137Cs was obtained. These profiles are separated into two groups with different behaviour, one of which includes clay and loam soils and the other containing sandy soils. For both groups of profiles the parameters of the convective-diffusive model, which describes the vertical migration of 137Cs in the soil, v (apparent convection velocity) and D (apparent diffusion coefficient) were calculated.  相似文献   

18.
Fruiting bodies of fungi belonging to more than 70 species were collected within a few thousand square meter area of one forest during 2006 and 2007. The soil profile was collected to check the cumulative deposition of 137Cs, which was relatively high, equal to 64 ± 2 kBq/m2 (calculated for October 2006). The majority of this activity was in the first 6 cm. Fruitbodies were analyzed for radiocesium and 40K by means of gamma-spectrometry. The highest 137Cs activity was 54.1 ± 0.7 kBq/kg (dry weight) for a sample of Lactarius helvus collected in 2006. The results for 2006 were higher than those for 2007. In a few cases the traces of short-lived (T1/2 = 2.06 a) 134Cs were still found in samples. The importance of mycorrhizal fungi for radiocesium accumulation is confirmed. The differences in activity among the species are discussed in relation to observations and predictions from previous studies, where the change in relative accumulation between fruiting bodies of different species was at least partially explained by the differences in the depth of the mycelium localization in a litter/soil system. It is concluded that in some cases, such as Boletus edulis and Xerocomus badius, this prediction is fulfilled and therefore this explanation confirmed.  相似文献   

19.
To evaluate the quantities of 137Cs from past nuclear tests being transported to and deposited in Japan by naturally-occurring phenomena, the authors developed long-range transport models for 137Cs considering Asian dust. The simulation using these models backed the observed recent increase of 137Cs deposition along the coast of the Sea of Japan in early spring. For the sake of public safety, it is vital to ascertain whether an increase of radioactive deposition is caused by natural phenomena or a nuclear accident. The observations in recent years have suggested that dust and soil containing 137Cs is transported from the regions around Inner Mongolia to Japan by the wind. In this paper, using observation data from the early spring of 2002 and 2006, the authors have found good agreement between the simulations and the measurements. The simulations reproduced the entrainment of 137Cs and subsequent transport to Japan caused by strong winds associated with low pressure areas around the Inner Mongolian grasslands. The most likely cause of high-level 137Cs deposition over northern Japan during March 2002 was 137Cs associated with particles transported at low-altitude (1 km) and subjected to precipitation on the 22nd to 24th.  相似文献   

20.
Following the Chernobyl accident, 137Cs contamination levels of wild boar in some districts of Southern Germany are still exceeding thousands of Bq kg−1. While the long term 137Cs concentration in forest plants, mushrooms, and roe deer meat has decreased significantly, for wild boar it has remained constant during the last decade. Between 1998 and 2008, we analysed the muscle meat of 656 wild boars shot in the district (“Landkreis”) Ravensburg. The 137Cs activity concentration showed considerable variability from less than 5 up to 8266 Bq kg−1 and it followed a seasonal pattern, which is attributed to changes in dietary habits, fodder availability, meteorological conditions and specific behaviour of 137Cs in wild boar organism. Tag values for wild boars from the district Ravensburg varied from 0.008 to 0.062 m2 kg−1 during 2000–2008.  相似文献   

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