Concentrations of long-lived artificial radionuclides in the moss-lichen cover of mountain plant communities

Specific features of⁹⁰Sr and¹³⁷Cs accumulation in individual lichen species and in the moss-lichen cover of plant communities were studied in some mountain ranges of the Polar and Northern Urals. The results showed that the amounts of radionuclides in lichens and mosses of mountain plant communities are at the level characteristic of the moss-lichen cover of flat ecosystems, and their accumulation depends on⁹⁰Sr and¹³⁷Cs input with the global radioactive fallout. The radionuclide contents in lichens and mosses sampled from different mountain rocks, slopes, and elevations fluctuate around this level. The differences depend both on the structural and functional properties of plants and on the climatic and ecological features of their environment.     

Effect of liming on the behaviour of (90)Sr and (137)Cs in a lake ecosystem

Liming of lakes is considered one possible remedial action to reduce the accumulation of radionuclides into fish in the case of a radiological accident. These responses were tested in field conditions in a small acidified lake that was divided into two parts: one limed with CaCO₃ and the other half left as an unlimed control. The transfer of ⁹⁰Sr from water into fish decreased on average by 50% during the first year after liming. However, at the same time the ⁹⁰Sr concentration in water increased, reaching a maximum within 6 months after liming. Approximately 50% more ⁹⁰Sr was detected in water in the limed part of the lake than on control side during the first year. ⁹⁰Sr was most probably released from the sediment as the Ca concentration and pH of the water increased. As a result of these two processes, which counterbalanced each other (increased release of ⁹⁰Sr into water from sediment and decreased transfer of ⁹⁰Sr from water into fish), the ⁹⁰Sr concentration in fish did not notably differ between the limed and control sides of the lake. Liming may only be suitable as a remedial action if carried out immediately after a radiological accident, before significant amounts of radionuclides have been deposited in lake sediments. In the case of ¹³⁷Cs, the effect of liming was less pronounced. ¹³⁷Cs activity concentration in water increased in the first year by 20% and uptake by fish decreased by 20%.     

137Cs and 90Sr in live and dead reindeer lichens (genera Cladonia) from the "Kraton-3" underground nuclear explosion site

The contents of 137Cs and 90Sr have been determined in 29 samples of live and dead reindeer lichens (genera Cladonia) collected at the "Kraton-3" underground nuclear explosion site (65.9 degrees N 112.3 degrees E, event year--1978) in Yakutia, Russia in 2002. The area contamination was within the range of 0.36-700 and 0.13-770 kBq m(-2) for 137Cs and 90Sr, respectively. The dead organisms were on average much more contaminated than the live ones. Vertical fractionation of the live lichen carpet demonstrated maximal activity concentrations of both radionuclides in the lower older section of the plants, while for the dead lichens the maximal activity concentrations of 137Cs were detected in the upper part. The vertical distribution of 90Sr was more or less homogeneous in the cushions of dead lichens. Elevated levels of 137Cs and 90Sr activity concentrations were also detected in the re-establishing young lichens growing over the residua of some dead lichens.     

Anthropogenic radionuclides in sediment in the Japan Sea: distribution and transport processes of particulate radionuclides

Distributions of anthropogenic radionuclides (⁹⁰Sr, ¹³⁷Cs and ^239+240Pu) in seabed sediment in the Japan Sea were collected during the period 1998–2002. Concentration of ⁹⁰Sr, ¹³⁷Cs and ^239+240Pu in seabed sediment was 0.07–1.6 Bq kg⁻¹, 0.4–9.1 Bq kg⁻¹ and 0.002–1.9 Bq kg⁻¹, respectively. In the northern basin of the sea (Japan Basin), ^239+240Pu/¹³⁷Cs ratios in seabed sediment were higher and their variation was smaller compared to that in the southeastern regions of the sea. The higher ^239+240Pu/¹³⁷Cs ratios throughout the Japan Basin were considered to reflect production of Pu-enriched particles in the surface layer and substantial sinking of particulate materials in this region. In the southern regions of the Japan Sea (<38°N), both inventories and ^239+240Pu/¹³⁷Cs ratios in sediment were larger than those in the other regions. In the southern Japan Sea, observations suggested that supply of particulate radionuclides by the Tsushima Warm Current mainly enhanced accumulation of the radionuclides in this region.     

Migration of Cs and Sr in undisturbed soil profiles under controlled and close-to-real conditions

Migration of ¹³⁷Cs and ⁹⁰Sr in undisturbed soil was studied in large lysimeters three and four years after contamination, as part of a larger European project studying radionuclide soil–plant interactions. The lysimeters were installed in greenhouses with climate control and contaminated with radionuclides in an aerosol mixture, simulating fallout from a nuclear accident. The soil types studied were loam, silt loam, sandy loam and loamy sand. The soils were sampled to 30–40 cm depth in 1997 and 1998. The total deposition of ¹³⁷Cs ranged from 24 to 45 MBq/m², and of ⁹⁰Sr from 23 to 52 MBq/m². It was shown that migration of ¹³⁷Cs was fastest in sandy loam, and of ⁹⁰Sr fastest in sandy loam and loam. The slowest migration of both nuclides was found in loamy sand. Retention within the upper 5 cm was 60% for both ¹³⁷Cs and ⁹⁰Sr in sandy loam, while in loamy sand it was 97 and 96%, respectively. In 1998, migration rates, calculated as radionuclide weighted median depth (migration centre) divided by time since deposition were 1.1 cm/year for both ¹³⁷Cs and ⁹⁰Sr in sandy loam, 0.8 and 1.0 cm/year, respectively, in loam, 0.6 and 0.8 cm/year in silt loam, and 0.4 and 0.6 cm/year for ¹³⁷Cs and ⁹⁰Sr, respectively, in loamy sand. A distinction is made between short-term migration, caused by events soon after deposition and less affected by soil type, and long-term migration, more affected by e.g. soil texture. Three to four years after deposition, effects of short-term migration is still dominant in the studied soils.     

Long-term dynamics of technogenic radionuclide concentrations in moss-lichen cover

Ample factual data has been used to analyze the long-term dynamics of ⁹⁰Sr and ¹³⁷Cs concentrations in moss-lichen cover. The stocks of radionuclides in lichens, mosses, and the moss-lichen cover of northern regions of the Urals and Siberia has been estimated for the first time. The data on recent ranges of ⁹⁰Sr and ¹³⁷Cs concentrations in lichens and mosses can serve as a basis for determining the background levels of radionuclide contamination for long-term monitoring and prognostic radioecological studies.     

Transfer factors of 137Cs and 90Sr from soil to trees in arid regions

Transfer factors of (137)Cs and (90)Sr from contaminated soil (Aridisol) to olive, apricot trees and grape vines were determined under irrigated field conditions for four successive years. The transfer factors (calculated as Bqkg(-1) dry plant material per Bqkg(-1) dry soil) of both radionuclides varied among tree parts and were highest in olive and apricot fruits. However, the values for (90)Sr were much higher than those for (137)Cs in all plant parts. The geometric mean of the transfer factors in olives, apricots and grapes were 0.007, 0.095 and 0.0023 for (137)Cs and 0.093, 0.13 and 0.08 for (90)Sr, respectively, and were negligible in olive oil for both radionuclides. The transfer factors of both radionuclides were similar to, or in the lower limits of, those obtained in other areas of the world. This could be attributed to differences in soil characteristics: higher pH, lower organic matter, high clay content, and higher exchangeable potassium and calcium.     

Soil to leaf transfer factor for the radionuclides ²²⁶Ra, ⁴⁰K, ¹³⁷Cs and ⁹⁰Sr at Kaiga region, India

Transfer factors are the most important parameters required for mathematical modeling used for environmental impact assessment of radioactive contamination in the environment. In this paper soil to leaf transfer factor for the radionuclides ⁴⁰K, ²²⁶Ra, ¹³⁷Cs and ⁹⁰Sr is estimated for Kaiga region in Karnataka state, India. Among the plants in which study is carried out, ²²⁶Ra, ⁴⁰K, ¹³⁷Cs and ⁹⁰Sr activity in leaves of herbaceous plants is higher than that of tree leaves. Soil to leaf transfer factor for ²²⁶Ra, ⁴⁰K, ¹³⁷Cs and ⁹⁰Sr was found to be in the range of 0.03-0.65, 0.32-8.04, 0.05-3.03 and 0.42-2.67 respectively.     

Current Contents of 90Sr and 137Cs in the Moss–Lichen Cover of Piedmont and Mountain Landscapes of the Northern Urals

The contents of long-lived artificial radionuclides, ⁹⁰Sr and ¹³⁷Cs, were determined in lichens and mosses of different taxa and in the samples of moss–lichen cover taken from the mountain and lowland plant communities of the Northern Urals. The effects of Chernobyl fallout and the dynamics of radionuclide contents in lichens and mosses were analyzed. The concentration of ¹³⁷Cs in the moss–lichen cover was higher in the mountain ecosystems than in the lowland plant communities.     

Uptake and distribution of 137Cs and 90Sr in salix viminalis plants

Agricultural areas in middle and northern parts of Sweden were contaminated with radionuclides after the Chernobyl accident in 1986. Alternative crops in these areas are biomass plantations with fast-growing Salix clones for energy purposes. The uptake and internal distribution of 137Cs and 90Sr in Salix viminalis were studied. Plants were grown in microplots under field conditions. The soils in the experimental site had been contaminated in 1961 with 35.7 and 13.4 MBq m(-2) of 137Cs and 90Sr, respectively. The experiment was carried out during three years. The plots were fertilised with 60 kg N ha(-1) and three treatments of K, consisting of 0, 80 and 240 kg K ha(-1) during the first two years. The activity concentration of 137Cs in the different plant parts varied between 140 and 20,000 Bq kg(-1) and was ranked in the following order: lowest in stems < cuttings < leaves < roots. The fine roots (0-1 mm) had the highest 137Cs activity concentration. One-year-old stems had higher 137Cs activity concentrations than two-year-old stems. The activity concentration of 137Cs in the plants was significantly affected by K-supply and was higher in the 0 kg K treatment than in the 80 or 240kg K treatment. Leaves contained more 90Sr than stems and cuttings.     

Distribution of 137Cs in the Tree Layer of Forest Ecosystems in the Zone of the Accident at the Chernobyl Nuclear Power Plant

Trends in ¹³⁷Cs distribution over the parts of coniferous (Pinus sylvestrisL.) and deciduous (Betula pendula Rocht.) trees are described. The trees have been selected in the stationary experimental plots located in southwestern Bryansk oblast, Russian Federation. The distribution of ¹³⁷Cs in the wood along the trunk height is shown to be nonuniform. The effects of ¹³⁷Cs content in the xylem sap on the accumulation of this radionuclide in the leaves and needles are assessed. The factors controlling ¹³⁷Cs accumulation in the components of woody plants are revealed, and their significance is estimated.     

Inventory and vertical migration of 90Sr fallout and 137Cs/90Sr ratio in Spanish mainland soils

In this paper the inventory of ⁹⁰Sr in 34 points distributed along the Spanish peninsular territory is presented. Obtained values range between 173 Bq/m² and 2047 Bq/m². From these data set and those ¹³⁷Cs data obtained in a previous work the ¹³⁷Cs/⁹⁰Sr activity ratio has been established, laying this value between 0.9 and 3.6. Also the migration depth of both radionuclides has been analysed obtaining for ¹³⁷Cs an average value 57% lower than that obtained for ⁹⁰Sr.Additionally, this paper presents the results obtained in 11 sampling points in which the activity vertical profile has been measured. These profiles have been analysed to state the behaviour of strontium in soils and after, by using a convective-diffusive model, the parameters of the model which governs the vertical migration of ⁹⁰Sr in the soil, v (apparent convection velocity) and D (apparent diffusion coefficient) have been evaluated. Mean values obtained are 0.20 cm/year and 3.67 cm²/year, respectively.     

Anthropogenic radionuclides in sediment in the Japan Sea: distribution and transport processes of particulate radionuclides

Distributions of anthropogenic radionuclides ((90)Sr, (137)Cs and (239+240)Pu) in seabed sediment in the Japan Sea were collected during the period 1998-2002. Concentration of (90)Sr, (137)Cs and (239+240)Pu in seabed sediment was 0.07-1.6 Bq kg(-1), 0.4-9.1 Bq kg(-1) and 0.002-1.9 Bq kg(-1), respectively. In the northern basin of the sea (Japan Basin), (239+240)Pu/(137)Cs ratios in seabed sediment were higher and their variation was smaller compared to that in the southeastern regions of the sea. The higher (239+240)Pu/(137)Cs ratios throughout the Japan Basin were considered to reflect production of Pu-enriched particles in the surface layer and substantial sinking of particulate materials in this region. In the southern regions of the Japan Sea (<38 degrees N), both inventories and (239+240)Pu/(137)Cs ratios in sediment were larger than those in the other regions. In the southern Japan Sea, observations suggested that supply of particulate radionuclides by the Tsushima Warm Current mainly enhanced accumulation of the radionuclides in this region.     

Application of the ERICA Assessment Tool to freshwater biota in Finland

In recent years there has been growing international interest in the assessment of doses and risks from ionising contaminants to biota. In this study the ERICA Tool, developed within the EC 6th Framework Programme, was applied to estimate incremental dose rates to biota in freshwater ecosystems in Finland mainly resulting from exposure to the Chernobyl-derived radionuclides ¹³⁷Cs, ¹³⁴Cs and ⁹⁰Sr. Data sets consisting of measured activity concentrations in fish, aquatic plants, lake water and sediment for three selected lakes located in a region with high ¹³⁷Cs deposition were applied in the assessment. The dose rates to most species studied were clearly below the screening level of 10 μGy h⁻¹, indicating no significant impact of the Chernobyl fallout on these species. However, the possibility of higher dose rates to certain species living on or in the bottom sediment cannot be excluded based on this assessment.     

Long-term dynamics of radioactive <Superscript>90</Superscript>Sr and <Superscript>137</Superscript>Cs contamination of small mammals in the Chernobyl zone

Between 1986 and 1994, a decrease in nonalimentary ⁹⁰Sr and ¹³⁷Cs intake and changes in the accessibility of radionuclides in the soil-plant link of their cycle resulted in a 10-to 100-fold decrease in their specific activity (SA) in the bodies of small mammals inhabiting the Chernobyl zone, and a similar decrease was observed in the radionuclide transition factor (TF) in the soil-animal chain. Between 1995 and 2005, no consistent increase or decrease in SA or TF could be revealed against the background of a combined effect of different physicochemical and ecological factors. It is suggested that subsequent changes in the level of radioactive contamination of small mammals will generally reflect only the dynamics of physical ⁹⁰Sr and ¹³⁷Cs decay, but, nevertheless, seasonal and local variations in this level will be significant.     

Anthropogenic radionuclides in the Japan Sea: their distributions and transport processes

The anthropogenic radionuclides, (90)Sr, (137)Cs and (239+240)Pu, were measured in the water column of the Japan Sea/East Sea during 1997-2000. The vertical profiles of radionuclide concentrations showed: exponential decrease with depth for (90)Sr and (137)Cs, and surface minimum/subsurface maximum for (239+240)Pu. These results do not differ substantially from results reported previously. The area-averaged concentrations of radionuclides in the Japan Sea are higher than those found in the Northwest Pacific Ocean below surface layer showing the accumulation of the radionuclides in the deep waters in the Japan Sea. Concerning spatial distributions, the area of high (137)Cs inventory extends from the Japan Basin into the Yamato Basin. It is suggested that wintertime convection of water, occurring mainly in the Japan Basin, causes the radionuclides to sink. The nuclides then advect into the Yamato Basin after detouring around the Yamato Rise.     

The influence of hot particle contamination on Sr and Cs transfers to milk and on time-integrated ingestion doses

Most models for transfers of radionuclides through the food chain typically assume that the radioactivity is initially deposited in chemically available forms. It is known, however, that releases of radionuclides in the form of hot particles may significantly influence their environmental transfers and uptake to the food chain. This study presents models for time changes in ⁹⁰Sr and ¹³⁷Cs in milk which incorporate hot particle contamination using observed rates of hot particle dissolution following the Chernobyl accident. A general equation is presented for the influence of hot particles on overall ingestion doses. As expected from previous work, fallout of hot particles significantly influences time changes in radionuclide activity concentrations in foodstuffs. It is also shown that incorporation of radionuclides in hot particles influences time-integrated ingestion doses. For a situation in which a large proportion (90–100%) of fallout is in slowly dissolving hot particles, time-integrated ingestion doses from ⁹⁰Sr and ¹³⁷Cs are reduced by a factor of approximately two compared to the case where all radioactivity is deposited in bioavailable forms. However, the influence of rapidly dissolving hot particles on time-integrated ingestion doses is relatively minor. Remaining significant uncertainties in dose estimates are discussed.     

Vertical distribution of radionuclides in soil of a grassland site in Chernobyl exclusion zone

Five soil profiles from a site about 8 km SE of the Chernobyl NPP were investigated for the vertical distribution of radionuclides. The average (137)Cs-inventory at the site is about 2.6 MBq/m(2) (reference date 1 May 1986). Apart from (137)Cs, the following radionuclides have been identified (their activity ratios to (137)Cs in brackets): (134)Cs (0.537), (125)Sb (0.068), (60)Co (0.0022), (154)Eu (0.016), (155)Eu (0.020), (94g)Nb (9.5E-5), (239/240)Pu (0.0088), (238)Pu (0.040), (90)Sr (0.30) and (241)Am (0.011). Apparent vertical migration velocities are between 0.14 and 0.26 cm/a, apparent dispersion coefficients range from 0.02 to 0.13 cm(2)/a. The rankings of the velocities v for different radionuclides are (Sr, Cs, Sb, Co, Pu)< Am < Eu and Sr < (Cs, Nb), for D, the following rankings have been found: (Nb, Sr, Cs) < Am < Eu, Cs相似文献   

Sources and pathways of Sr in the North Atlantic–Arctic region: present day and global warming

The spatial and temporal distributions of the anthropogenic radionuclides ¹³⁷Cs and ⁹⁰Sr, originating from nuclear bomb testing, the Sellafield reprocessing plant in the Irish Sea (UK), and from the Ob and Yenisey river discharges to the Arctic Ocean, have been simulated using the global version of the Miami Isopycnic Coordinate Ocean Model (MICOM). The physical model is forced with daily atmospheric re-analysis fields for the period of 1948–1999. Comparison of the temporal evolution of the observed and the simulated concentrations of ⁹⁰Sr has been performed in the Kara Sea. The relative contributions of the different sources on the temporal and spatial distributions of the surface ⁹⁰Sr are quantified over the simulated period. It follows that the Ob river discharge dominated the surface ⁹⁰Sr over most of the Arctic Ocean and along the eastern and western coasts of Greenland before 1960. During the period of 1980–1990, the atmospheric fallout and the Ob river discharge were equally important for the ⁹⁰Sr distribution in the Arctic Ocean. Furthermore, an attempt has been made to explore the possible dispersion of accidental released ⁹⁰Sr from the Ob and Yenisey rivers under a global warming scenario (2 × CO₂). The difference between the present-day and the global warming scenario runs indicates that more of the released ⁹⁰Sr from the Ob and Yenisey rivers is confined to the Arctic Ocean in the global warming run, particularly in the near coastal, non-European part of the Arctic Ocean.