Seasonal variations of aerosol residence time in the lower atmospheric boundary layer

During a one year period, from Jan. 2002 up to Dec. 2002, approximately 130 air samples were analyzed to determine the atmospheric air activity concentrations of short- and long-lived (222Rn) decay products 214Pb and 210Pb. The samples were taken by using a single-filter technique and gamma-spectrometry was applied to determine the activity concentrations. A seasonal fluctuation in the concentration of 214Pb and 210Pb in surface air was observed. The activity concentrations of both radionuclides were observed to be relatively higher during the winter/autumn season than in spring/summer season. The mean activity concentration of 214Pb and 210Pb within the whole year was found to be 1.4+/-0.27 Bq m(-3) and 1.2+/-0.15 mBq m(-3), respectively. Different 210Pb:214Pb activity ratios during the year varied between 1.78 x 10(-4) and 1.6 x 10(-3) with a mean value of 8.9 x 10(-4) +/- 7.6 x 10(-5). From the ratio between the activity concentrations of the radon decay products 214Pb and 210Pb a mean residence time (MRT) of aerosol particles in the atmosphere of about 10.5+/-0.91 d could be estimated. The seasonal variation pattern shows relatively higher values of MRT in spring/summer season than in winter/autumn season. The MRT data together with relative humidity (RH), air temperature (T) and wind speed (WS), were used for a comprehensive regression analysis of its seasonal variation in the atmospheric air.     

Detection of 210Po on filter papers 16 years after use for the collection of short-lived radon progeny in a room

Radon gas was allowed to accumulate in its radium source and then injected into a 36 m(3) test room, resulting in an initial radon concentration of 15 kBq m(-3). Filter papers were used to collect the short-lived radon progeny and thus to measure the Potential Alpha Energy Concentration (PAEC) in-situ in the year 1984 at different times and conditions according to the experimental design. The radon progeny collected on the filter papers were studied as a function of aerosol particle concentration ranging from 10(2)-10(5) particles cm(-3) in three different experiments. The highest aerosol particle concentration was generated by indoor cigarette smoking. Those filters were stored after the experiment, and were used after 16 years to study the activity of the radon long-lived alpha emitter progeny, (210)Po (T(1/2)=138 days). This isotope is separated from the short-lived progeny by (210)Pb beta emitter with 22.3 years half-life. After 16 years' storage of these filters, each filter paper was sandwiched and wrapped between two CR-39 nuclear track detectors, to put the detectors in contact with the surfaces of different filters, for 337 days. Correlation between the PAEC measured using filter papers in the year 1984 and the activity of long-lived alpha emitter (210)Po on the same filter papers measured in the year 2000 were studied. The results of the (210)Po activity showed a very good correlation of 0.92 with the PAEC 16 years ago. The results also depict that the PAEC and (210)Po activity in indoor air increased with the increase of aerosol particle concentration, which shows the attachment of short-lived radon progeny with the aerosol particles. The experiment proves that indoor cigarette smoking is a major source of aerosol particles carrying radon progeny and, thus, indoor cigarette smoking is an additional source of internal radiation hazard to the occupants whether smoker or non-smoker.     

Radioactive fallout in Norway from atmospheric nuclear weapons tests

Historical data on radioactivity in air and precipitation samples have been collected and analysed from study sites in Norway. The purpose of the study was to investigate the correlation between air concentration, precipitation and deposition, and identify areas with high deposition. Areas with high precipitation have been compared with monitoring stations in other countries. The base line data contain measurements of total beta in air and precipitation on a daily basis for the period 1956-1982. Radioactive fallout correlated strongly with annual precipitation which varies from 280 to 4200mm per year in Norway. The deposition of 137Cs was calculated to be 3.23+/-1.20kBq/m2 per 1,000 mm precipitation for the period 1955-1975. Also, the relationship between total beta and 137Cs has been investigated, in order to estimate the age of fallout. The age of fallout in Norway ranges from 3 to 9 months during the test periods, which is considerably shorter than the global average, where the mean residence time for debris in the lower stratosphere is estimated to be 1.3 years. There is no evidence of local fallout from tests on Novaya Zemlya reaching Norwegian areas.     

Factors influencing ambient concentrations of (210)Pb and (7)Be over the city of Edinburgh (55.9 degrees N, 03.2 degrees W)

Concentrations of (210)Pb and (7)Be in air were continuously monitored, using a high-volume air sampler and a high-resolution gamma-ray spectrometer, during the period of July 2002 to June 2003 at the University of Edinburgh 55.9 degrees N, 03.2 degrees W. The time series of both radio-isotopes show seasonality, dependence on air-mass origin, residence time and precipitation. Surface air concentrations of (210)Pb and (7)Be ranged from 0.01 to 0.74 mBq m(-3) and 0.63-6.54 mBq m(-3), respectively. The measurements indicate that the average concentrations of both (210)Pb and (7)Be in surface air were 0.21+/-0.01 and 2.50+/-0.04 mBq m(-3), respectively; which agrees closely with the corresponding values reported for coastal air measurements in Europe.     

Seasonal variation of 210Pb activity concentration in outdoor air of Milan (Italy)

Weekly measurements of 210Pb activity concentration on aerosol particles were performed at ground level in outdoor air in Milan (Italy) during the years 2000-2001. The experimental method was based on the delayed alpha spectrometry of in-grown 210Po activity detected on airborne particles collected on a filter support. On the same filter the 214Pb activity concentration was also measured during the sampling. 210Pb weekly concentration values showed a great variability and the average monthly values exhibited a seasonal pattern characterised by maxima in winter and minima in spring-summer. The same seasonal trend was also observed in 214Pb concentration values. 210Pb average yearly values were 0.70 and 0.82 mBq/m3 in 2000 and 2001, respectively, in good agreement with literature data registered at continental sites of similar latitude and longitude. The activity ratio 210Pb/214Pb was used to evaluate the residence time of fine aerosols in the urban air of Milan, which was 1-2 days.     

Factors controlling 7Be and 210Pb atmospheric deposition as revealed by sampling individual rain events in the region of Geneva, Switzerland

Bulk atmospheric deposition of 7Be and 210Pb has been measured at Versoix, close to Geneva, Switzerland. Collectors were continuously deployed from November 1997 through November 1998 for periods from 1 to 22 days depending on the frequency of rain. The activities of 7Be and 210Pb integrated over the sampling interval were moderately well correlated with rainfall (r2 of 0.66 and 0.55, respectively; p < 0.001) and well correlated one with the other (r2 of 0.91; p < 0.001). The 7Be/210Pb activity ratio is close to 13.5, except for samples collected in the periods of very low precipitation which have a distinctly lower ratio. A simple model accounting for rainfall, seasonal variations and reload of the local atmosphere after a rain event explains 90% of the variance of 7Be and 210Pb deposition. Concentrations of 210Pb and Ca++ in rain were correlated with transport time of air masses over the continent as indicated by reconstruction of air mass trajectories over three days.     

Inventories of fallout 210Pb and 137Cs radionuclides in moorland and woodland soils around Edinburgh urban area (UK)

Inventories of fallout (210)Pb and (137)Cs have been measured in moorland and woodland soils around the Edinburgh urban area, using a high purity germanium detector. The (210)Pb inventories in moorland soils were relatively uniform, with a mean value of 2520+/-270Bqm(-2). The mean (137)Cs inventory in moorland soils varied greatly from 1310 to 2100Bqm(-2), with a mean value of 1580+/-310Bqm(-2). The variability was ascribed mainly to the non-uniform distribution of fallout Chernobyl (137)Cs. The mean (210)Pb and (137)Cs inventories in woodland canopy soils were found to be 3630+/-380Bqm(-2) and 2510+/-510Bqm(-2), respectively. At sites for which both moorland and woodland data were available, the mean inventories provided fairly similar average enhancements of (47+/-7)% and (46+/-18)% of (210)Pb and (137)Cs under woodland canopy soils relative to open grassland soils, respectively. The enhancement factors are broadly in line with other independent findings in literature. Enhancement of both (210)Pb and (137)Cs in woodland soils relative to moorland soils is, in part, due to deposition by impaction during air turbulence, wash-off, gravitational settling and deposition during leaf senescence. Results of this study suggest that these processes affect both (210)Pb and (137)Cs carrier aerosols in a similar way.     

High (210)Po atmospheric deposition flux in the subtropical coastal area of Japan

Bulk atmospheric deposition fluxes of (210)Po and (210)Pb were measured at three coastal regions of Japan, the Pacific Ocean coastal area of the Japanese mainland (Odawa Bay), the Chinese continental side of Japanese coastal area (Tsuyazaki), and an isolated island near Okinawa (Akajima). Wet and dry fallout collectors were continuously deployed from September 1997 through August 1998 for periods of 3 to 31 days depending on the frequency of precipitation events. Annual (210)Pb deposition fluxes at Odawa Bay (35 degrees N 139 degrees E), Tsuyazaki (33 degrees N 130 degrees E) and Akajima (26 degrees N 127 degrees E) were 73.3+/-8.0, 197+/-35 and 78.5+/-8.0 Bqm(-2)y(-1), respectively. Higher (210)Pb deposition was observed at the Chinese continental side of Japanese coast than at the Pacific Ocean coastal site. The high (210)Pb atmospheric flux at the Chinese continental side coast was thought to be attributable to (222)Rn-rich air-mass transport from the Chinese continent during the winter monsoon. In contrast, the annual (210)Po deposition fluxes at the three study sites were 13.0+/-2.3 (Odawa Bay), 21.9+/-4.4 (Tsuyazaki) and 58.4+/-7.7 (Akajima)Bqm(-2)y(-1), respectively, indicating unusual high (210)Po deposition at Akajima during winter. Anomalous unsupported (210)Po input was observed during summer 1997, suggesting unknown source of (210)Po at this area.     

A study on natural radiation exposure in different realistic living rooms

In the first part of the paper, the factors affecting 222Rn properties in 25 different realistic living rooms (with low ventilation rates) of different houses in El-Minia City (Upper Egypt) have been studied; they included the activity concentration of 222Rn gas (C(o)), the unattached fraction (f(p)) of 218Po and 214Pb, the unattached potential alpha energy concentration (PAEC) and the equilibrium factor (F). The activity distributions of unattached 218Po and 214Pb as well as for the PAEC were determined. With a dosimetric model calculation [ICRP, 1994b. Human Respiratory Tract Model For Radiological Protection. Pergamon Press, Oxford. ICRP Publication 66] the total deposition fraction of unattached 218Po and 214Pb in human respiratory tract was evaluated to determine the total equivalent dose. An electrostatic precipitation method and a wire screen diffusion battery technique were both employed for the determination of 222Rn gas concentration and its unattached decay products, respectively. The mean activity concentration of 222Rn gas (C(o)) was found to be 110+/-20 Bq m(-3). The mean unattached activity concentrations of 218Po and 214Pb were found to be 0.6 and 0.35 Bq m(-3), respectively. A mean unattached fraction (f(p)) of 0.09+/-0.01 was obtained at a mean aerosol particle concentration (Z) of (2.9+/-0.23) x 10(3)cm(-3). The mean equilibrium factor (F) was determined to be 0.31+/-0.02. The mean PAEC of unattached 218Po and 214Pb was found to be 8.74+/-2.1 Bq m(-3). The activity distributions of 218Po and 214Pb show mean activity median diameters (AMD) of 1.5 and 1.85 nm with mean geometric standard deviations (SD) of 1.33 and 1.45, respectively. The mean activity distribution of the PAEC shows an AMD of 1.65 nm with a geometric standard deviation of 1.25. At a total deposition fraction of about 97% the total equivalent dose to the lung was determined to be about 133 microSv. The second part of this paper deals with a study of natural radionuclide contents of samples collected from the building materials of the rooms under investigations in part one. Analyses were performed in Marinelli beakers with a gamma multichannel analyzer equipped with a NaI(Tl) detector. The samples revealed the presence of the uranium-radium and thorium radioisotopes as well as 40K. Nine gamma-lines of the natural radioisotopes corresponding to 212Pb, 214Pb, 214Bi, 228Ac, 40K and 208Tl were detected and measured. The activity concentrations of 226Ra, 232Th and 40K were determined with mean activity concentrations of 58+/-19, 31+/-11 and 143+/-62 Bq kg(-1), respectively. These activities amount to a radium equivalent (Ra(eq)) of 113 Bq kg(-1) and to a mean value of external hazard index of 0.31.     

汉江流域降水结构时空特征及影响因素分析

利用汉江流域32个气象站1961~2016年逐日降水资料，分析了汉江流域降水时空分布特征，并探讨了海温及大气环流对流域降水的影响。结果表明：雨量和雨日空间分布相似，小雨、中雨的雨量和雨日由西南向东北递减，降水中心位于西南和东南部；流域东北部大雨以上量级降水由偏少转为偏多，而雨强空间分布则没有明显规律。流域降水集中度自东南向西北逐渐增加，降水集中期逐渐推迟。海温对降水的影响存在季节差异，春季、夏季和秋季降水分别受前期南印度洋、热带北大西洋和热带中东太平洋海温影响，冬季降水则受海温影响不明显；大尺度大气环流对降水存在影响，冬季欧亚遥相关型和春季西太平洋遥相关型均引起冬季风强度变化来影响冬季和春季降水，夏季副高位置和乌山阻高以及秋季巴湖低槽和印缅槽强度则均通过冷空气和暖湿气流强度及交汇位置来影响夏季和秋季降水。     

Derivation of 137Cs deposition density from measurements of 137Cs inventories in undisturbed soils

The 137Cs inventories in undisturbed soils were measured for 292 locations across the territory of Vietnam. The logarithmic inventory values were regressed against characteristics of sampling sites, such as geographical coordinates, annual rainfall and physico-chemical parameters of soil. The regression model containing latitude and annual rainfall as determinants could explain 76% of the variations in logarithmic inventory values across the territory. The model part was interpreted as the logarithmic 137Cs deposition density. At the 95% confidence level, 137Cs deposition density could be predicted by the model within +/- 7% relative uncertainty. The latitude mean 137Cs deposition density increases northward from 237 Bq m(-2) to 1097 Bq m(-2), while the corresponding values derived from the UNSCEAR (1969) global pattern are 300 Bq m(-2) and 600 Bq m(-2). High 137Cs inputs were found in high-rainfall areas in northern and central parts of the territory.     

Importance of atmospherically deposited nitrogen to the annual nitrogen budget of the Neuse River estuary,North Carolina

Wet deposition of nitrogen, as NH(4)(+), NO(3)(-), and organic N, contributes up to 50% of the total externally supplied or 'new' N flux to the Neuse River Estuary (North Carolina). Excessive nitrogen (N) loading to N-sensitive waters such as the Neuse River Estuary has been linked to changes in microbial and algal community composition and function (harmful algal blooms), hypoxia/anoxia, and fish kills. In a 4-year study from July 1996 to July 2000, the weekly wet deposition of NH(4)(+), NO(3)(-), and dissolved organic N was calculated, based on concentration and precipitation measurements, at 11 sites on a northwest-southeast transect in the watershed. Data from this period indicate that the annual mean total wet atmospherically deposited (AD)-N flux was 11 kg ha(-1) year(-1). Deposition was fairly evenly distributed between nitrate, ammonium, and organics (32%, 32%, and 36%, respectively). Seasonally, the summer (June-August) months contained the highest weekly wet total N deposition; this trend was not driven by precipitation amount. Estimates of watershed N retention and in-stream riverine processing revealed that the AD-N flux contributed an estimated 20% (range of 15-51%) of the total 'new' N flux to the estuary, with direct deposition of N to the estuary surface accounting for 6% of the total 'new' N flux. This study did not measure the dry depositional flux, which may double the contribution of AD-N to the estuary. The AD-N is an important source of 'new' N to the Neuse River Estuary as well as other estuarine and coastal ecosystems downwind of major emission sources. As such, AD-N should be included in effective nutrient mitigation and management efforts for these N-sensitive waters.     

华东沿海热带气旋移动和降水特征研究

基于TRMM 3B42RT 3 h降水资料和欧洲中期天气预报中心（ECMWF）的500 hPa分析场资料,借助于GIS空间分析方法,对热带气旋降水大值区的分布落区与移动路径之间的空间关系进行了统计叠置,分析了2000～2009年共29个登陆华东沿海或进入华东近海海域的热带气旋的路径、强度、降水的空间分布以及500 hPa环流形势对其影响的规律。结果表明：不同500 hPa环流形势对登陆热带气旋的移动路径及降水的空间分布型态有规律可循,其中中高纬西风带环流形势（50°N以北）以及副高西脊点所处的位置在热带气旋路径和降水分布型的业务预报中起着重要的指示作用     

Beryllium-7 in near-surface air and deposition at Brisbane, Australia

Measurements of 7Be concentrations in near-surface air and 7Be deposition were carried out at Brisbane, Australia. Concentrations of 7Be in near-surface air measured over 4 years show seasonal variations with values above the annual mean occurring mainly in the spring and summer months of each year. These higher concentrations coincide with the expected influx of stratospheric air to the planetary boundary layer in early spring and higher rates of convective circulation within the troposphere during summer. 7Be deposition measurements over 3 years show seasonal variations similar to the seasonal rainfall pattern. There is a statistically significant (p<0.001) linear relationship between monthly (7)Be deposition and rainfall amount. This relationship is used to calculate the net cumulative (7)Be areal activity density.     

7Be to 210Pb concentration ratio in ground level air in Belgrade area

7Be to 210Pb concentration ratios in ground level air on two monitoring stations (MS1 and MS2) in Belgrade area were determined from 1996 to 2001. The average monthly concentrations of 7Be in ground level air were in the range of 0.6-18.3 mBq/m3 and exhibited one or two summer/early fall maxims and one minimum in winter. The maximum concentrations for 210Pb were generally observed in the fall, with the average concentrations in the range of 1.09 x 10(-4) to 30.9 x 10(-4) Bq/m3. The 7Be/210Pb ratios were in the range of 1.7-12.7 (MS1) and 1.8-11.3 (MS2), with summer maxims and late fall/winter minimums. The mean Radionuclides Loading Indices values approach zero except for 1996/1997 (MS1) and 2001 (MS2) due to higher concentrations of 7Be and 210Pb. The mean monthly concentrations of both radionuclides exhibited lognormal distributions. There is significant correlation between the 7Be/210Pb activities ratio and the air stability classes A + B + C for both monitoring stations (correlation coefficients 0.61-0.65), and no correlation with D class and E + F classes. Correlation was found between the activity of 7Be and air stability classes A + B + C (0.46-0.68), and E + F (0.38 for MS1), while for 210Pb, a moderate correlation (0.38-0.40) was found with the E + F air stability classes.     

Temporal variation of 212Pb concentration in outdoor air of Milan and a comparison with 214Bi

Continuous measurement of hourly concentrations of 212Pb attached to aerosol particles was carried out during the whole year 2000 in the outdoor air of Milan (Italy). An improved experimental method based on on-line alpha spectroscopy during atmospheric particulate matter sampling allowed the contemporary determination of 212Pb and 214Bi through the deconvolution of the alpha energy spectral distribution analysis. The 212Pb hourly concentrations were about 100 times lower than 214Bi but showed a similar characteristic diurnal time trend. However, the influence of meteorological parameters such as rain and wind was more evident in 212Pb than in 214Bi concentrations. The 212Pb average annual concentration was 0.090 +/- 0.060 Bq/m3 with daily mean concentration varying from 0.013 to 0.333 Bq/m3.     

Precipitation scavenging of 7Be and 137Cs radionuclides in air

Atmospheric depositional fluxes of the naturally occurring 7Be of cosmogenic origin and 137Cs from fallout of the Chernobyl accident were measured over a 6-year period (January 1987-December 1992) at Thessaloniki, Greece (40 degrees 38'N, 22 degrees 58'E). Total precipitation accumulation during 1987-1992 varied between 33.7 cm and 65.2 cm, reflecting a relatively dry (precipitation-free) climate. The activity concentrations of 7Be and 137Cs in rainwater depended on the precipitation rate, being higher for low precipitation rates and lesser for high precipitation rates. 137Cs was removed by rain and snow more efficiently than 7Be. Snowfall was more efficient than rainfall in removing the radionuclides from the atmosphere. The annual bulk depositional fluxes of 7Be varied between 477 and 1133 Bq m(-2) y(-1) and this variability was attributed to the amount of precipitation and the variations of the atmospheric concentrations of 7Be. The annual bulk depositional fluxes of 137Cs showed a significant decrease over time from 1987 to 1992, resulting in a removal half-life of 1.33 years. The presence of 137Cs in air, and therefore in rainwater and snow, long after the Chernobyl accident (26 April 1986) was mainly due to the resuspension process. The normalized depositional fluxes of both radionuclides showed maximal values during the spring season where the maximum amount of precipitation occurred. The relatively high positive correlation between 7Be and 137Cs normalized depositional fluxes indicates that the scavenging process of local precipitation controlled the fluxes of both radionuclides. The dry depositional flux of 7Be was less than 9.37% of total (wet and dry) depositional flux. The fraction of dry-to-total depositional flux of 137Cs was much higher than that of 7Be, due to the resuspended soil.     

A 10-year study of the 137Cs distribution in soil and a comparison of Cs soil inventory with precipitation-determined deposition

During a 10-year period, 1988-1998, surface soil samples have been collected at Blentarp in southern Sweden and analysed for 137Cs from the Chernobyl accident and from the nuclear weapons tests. The distance between the sampling plots on the different sampling occasions has been no more than 3 m. The results show that the depth distribution of 137Cs is very similar for each of the sampling occasions, indicating that the caesium migration at this site is very small. The total activity measured in the soil cores is in agreement with the calculated activity of 137Cs deposited at the site after nuclear weapons tests and the Chernobyl accident, based on air activity concentration and the amount of precipitation. The calculated deposition of 137Cs originating from the bomb tests amounts to 1.41 kBq m-2 for the period 1962-1986, which is in agreement with the activity of nuclear weapons fallout measured in the soil samples (1.60 kBq m-2 as a mean value of the first four years of sampling). The calculated activity of 137Cs of Chernobyl origin was 0.79 kBq m-2, which agrees well with the value of 0.79 kBq m-2 measured in the soil samples in 1988.     

淮河流域近50年降水异常及其大尺度环流特征

根据国家气象中心整编的全国714站月平均降水量资料，运用REOF分析、Morlet小波分析、差值分析等方法，通过对淮河流域代表站点的选取，分析了1960～2009年淮河流域降水的趋势变化特征、周期特征，以及多雨、少雨年的大气环流异常特征。结果表明：（1）淮河流域年降水总量呈缓慢增长趋势，20世纪80年代初期由负距平转为正距平。冬季和夏季降水量呈显著增长趋势，春季和秋季降水量呈显著减少趋势，80年代前期为降水变化的转折期；(2)淮河流域夏季降水存在准3 a的显著振荡周期和准10 a的次显著振荡周期，同时在60～90年代还存在准6 a振荡周期；（3）淮河流域多雨年，500 hPa经向风偏强且范围广，850 hPa上从孟加拉湾经南海向华东地区的水汽输送明显偏强，在江苏、安徽地区有水汽的正涡度辐合区；少雨年，经向风偏弱，华东地区方向的水汽输送明显减弱；（4）多雨年与少雨年的500 hPa风场差值场、高度场差值场分析表明，多雨年贝加尔湖西部和鄂霍次克海地区阻塞高压活动频繁，东北冷涡异常活跃，副高偏强，3者共同作用使得降水偏多。500 hPa温度场差值场分析表明，多雨年中国东部、华北和东北地区冷空气偏强，同时南方大部分地区暖空气也偏强，冷暖空气共同作用使降水偏多     

Variation of the activity concentrations and fluxes of natural (210Po, 210Pb) and anthropogenic (239,240Pu, 137Cs) radionuclides in the Strait of Gibraltar (Spain)

The activity concentrations and fluxes of natural (210Pb, 210Po) and anthropogenic (239,240Pu, 137Cs) radionuclides have been determined in the different water masses crossing the Strait of Gibraltar. New data have been gathered during four multidisciplinary and multinational sampling campaigns, performed between 1997 and 1999 within the framework of the CANIGO-FLUGIST Project. Mean activity concentrations of 210Po (1.53+/-0.34 Bq m(-3), n = 30) and 210Pb (1.16+/-0.50 Bq m(-3), n = 31) in the Atlantic water entering the Mediterranean basin are about double those measured in the Mediterranean outflow, namely 0.84+/-0.34 Bq m(-3) (n = 22) for 210Po and 0.66+/-0.34 Bq m(-3) (n = 22) for 210Pb. The opposite trend is observed for 231,240Pu, with average concentrations of 9.9+/-3.0 mBq m(-3) (n = 29) in the incoming Atlantic flow and 22.0+/-3.0 mBq m(-3) (n = 22) in the outpouring Mediterranean water. In the case of 137Cs, the same concentrations were quantified in the waters moving inwards (2.52+/-0.28 Bq m(-3), n = 27) and outwards (2.14+/-0.52 Bq m(-3), n = 21) from the Mediterranean Sea. On this basis, the Mediterranean basin experiences a net annual input flux of 14 TBq of 210Pb and 19 TBq of 210Po, and a net annual loss of 0.34 TBq of 239,240Pu, while--at present--137Cs input and output fluxes appear to be balanced.