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1.
全(多)氟烷基化合物(per(poly)fluoroalkyl substances,PFASs)在环境各个介质及人体样品中广泛被检出,近年,在室内空气和灰尘中也普遍发现PFASs.研究表明,室内空气中PFASs的含量普遍高于室外空气,室内空气和灰尘中的PFASs可能是室外空气的污染来源及人体暴露源,因此室内环境中PFASs成为环境领域的又一个研究热点.但目前为止,我国还没有开展室内空气中PFASs的相关研究,室内灰尘中PFASs的研究也相对较少.本文就室内空气和灰尘中PFASs的采样与分析方法、污染现状、来源分析及人体暴露等4个方面进行了综合阐述,以期为我国室内环境中PFASs的研究提供参考. 相似文献
2.
Background, Aim and Scope Air quality is an field of major concern in large cities. This problem has led administrations to introduce plans and regulations
to reduce pollutant emissions. The analysis of variations in the concentration of pollutants is useful when evaluating the
effectiveness of these plans. However, such an analysis cannot be undertaken using standard statistical techniques, due to
the fact that concentrations of atmospheric pollutants often exhibit a lack of normality and are autocorrelated. On the other
hand, if long-term trends of any pollutant’s emissions are to be detected, meteorological effects must be removed from the
time series analysed, due to their strong masking effects.
Materials and Methods The application of statistical methods to analyse temporal variations is illustrated using monthly carbon monoxide (CO) concentrations
observed at an urban site. The sampling site is located at a street intersection in central Valencia (Spain) with a high traffic
density. Valencia is the third largest city in Spain. It is a typical Mediterranean city in terms of its urban structure and
climatology. The sampling site started operation in January 1994 and monitored CO ground level concentrations until February
2002. Its geographic coordinates are W0°22′52″ N39°28′05″ and its altitude is 11 m. Two nonparametric trend tests are applied.
One of these is robust against serial correlation with regards to the false rejection rate, when observations have a strong
persistence or when the sample size per month is small. A nonparametric analysis of the homogeneity of trends between seasons
is also discussed. A multiple linear regression model is used with the transformed data, including the effect of meteorological
variables. The method of generalized least squares is applied to estimate the model parameters to take into account the serial
dependence of the residuals of this model. This study also assesses temporal changes using the Kolmogorov-Zurbenko (KZ) filter.
The KZ filter has been shown to be an effective way to remove the influence of meteorological conditions on O3 and PM to examine underlying trends.
Results The nonparametric tests indicate a decreasing, significant trend in the sampled site. The application of the linear model
yields a significant decrease every twelve months of 15.8% for the average monthly CO concentration. The 95% confidence interval
for the trend ranges from 13.9% to 17.7%. The seasonal cycle also provides significant results. There are no differences in
trends throughout the months. The percentage of CO variance explained by the linear model is 90.3%. The KZ filter separates
out long, short-term and seasonal variations in the CO series. The estimated, significant, long-term trend every year results
in 10.3% with this method. The 95% confidence interval ranges from 8.8% to 11.9%. This approach explains 89.9% of the CO temporal
variations.
Discussion The differences between the linear model and KZ filter trend estimations are due to the fact that the KZ filter performs the
analysis on the smoothed data rather than the original data. In the KZ filter trend estimation, the effect of meteorological
conditions has been removed. The CO short-term componentis attributable to weather and short-term fluctuations in emissions.
There is a significant seasonal cycle. This component is a result of changes in the traffic, the yearly meteorological cycle
and the interactions between these two factors. There are peaks during the autumn and winter months, which have more traffic
density in the sampled site. There is a minimum during the month of August, reflecting the very low level of vehicle emissions
which is a direct consequence of the holiday period.
Conclusions The significant, decreasing trend implies to a certain extent that the urban environment in the area is improving. This trend
results from changes in overall emissions, pollutant transport, climate, policy and economics. It is also due to the effect
of introducing reformulated gasoline. The additives enable vehicles to burn fuel with a higher air/fuel ratio, thereby lowering
the emission of CO. The KZ filter has been the most effective method to separate the CO series components and to obtain an
estimate of the long-term trend due to changes in emissions, removing the effect of meteorological conditions.
Recommendations and Perspectives Air quality managers and policy-makers must understand the link between climate and pollutants to select optimal pollutant
reduction strategies and avoid exceeding emission directives. This paper analyses eight years of ambient CO data at a site
with a high traffic density, and provides results that are useful for decision-making. The assessment of long-term changes
in air pollutants to evaluate reduction strategies has to be done while taking into account meteorological variability 相似文献
3.
4.
Influence of new town development on the urban heat island - The case of the Bundang area 总被引:3,自引:0,他引:3
SONG Young-bae 《环境科学学报(英文版)》2005,17(4):641-645
Five new towns have been developed around the Seoul metropolitan area since 1996. However, these new towns generate lots of traffic and related problems in the areas including those new towns and Seoul as a result of increases in population and a lack of ecological-self-sufficiency. Currently, construction of another new town is under deliberation, and what should be a major consider is the notion that the new town be located within a wide, green zone. Many studies have revealed that green space can play an important role in improving urban eco-meteorological capability and air quality. In order to analyze the urban heat island which will be created by the new urban development, and to investigate the local thermal environment and its negative effects caused by a change of land use type and urbanization, Landsat TM images were used for extraction of urban surface temperature according to changes of land use over the last 15 years. These data are analyzed together with digital land use and topographic information. As a study result, it was found the urban heat island of the study area from 198.5 to 1999 rapidly developed which showed a difference of mean temperature above 2.0. Before the Bundang new town construction the temperature of the residential area was the same as a forest, but during the new town construction in 1991 analysis revealed the creation of an urban heat island. The temperature of a forest whose size is over 50% of the investigation area was lowest, and thus the presence of a forest is believed to have a direct cooling effect on the urban environment and its surroundings. The mean temperature of the residential and commercial areas in the study was found to be 4.5 higher than the forest, and therefore this part of land use is believed to be the main factor causing the temperature increase of the urban heat island. 相似文献
5.
We report a gas chromatographic-mass spectrometric method which allows the very long chain fatty acids content of trophoblastic tissue to be directly measured in samples collected by biopsy between 8 and 11 weeks of gestation. This method has been successfully applied to the detection of fetal Zellweger syndrome in two pregnant women who had previously delivered affected infants. In one of them, increased concentrations of C26:0 (0.254 versus 0.108±0.035 μ/mg proteins) and C24:0 (1.32 versus 0.815±0.325 μ/mg proteins) in trophoblast indicated that the fetus had Zellweger syndrome, a diagnosis confirmed by pathological findings after abortion. In the second case, the pregnancy was allowed to proceed, on the basis of normal concentrations of very long chain fatty acids in trophoblastic tissue, and its outcome was actually a healthy newborn. 相似文献
6.
7.
铁路运输安全事故灰色预测方法研究 总被引:6,自引:1,他引:6
近年来 ,我国铁路运输发展迅猛 ,尤其是列车运行多次提速 ,列车运行密度加大 ,对铁路运输安全管理不断提出了新的要求。依靠科技进步 ,尽量防止或减少安全事故的发生 ,要应用安全信息技术 ,使安全管理人员对铁路运输安全现状及未来事故发展趋势有所了解 ,提高安全防范意识及事故处理能力 ,同时还要不断提高员工的安全意识和安全文化素质 ,这些方法对于提高安全管理水平 ,降低事故的发生 ,保护人民的生命安全与健康具有重要意义。铁路运输安全事故预测技术就可很好解决上述问题。笔者应用灰色预测理论 ,建立了铁路运输安全事故预测模型 ,开发了安全事故预测软件系统 ,并以某铁路运输企业为例 ,介绍了研制的灰色预测系统软件的应用效果 相似文献
8.
中国交通安全技术分析 总被引:6,自引:6,他引:6
笔者在分析和比较中、美、日等国道路交通现状、交通安全的发展趋势、已采取相应对策及其实施效果的基础上 ,对我国现阶段交通特点、交通安全的状况、交通安全技术特征以及发展趋势进行了研讨和分析 ,并强调在交通安全管理的总体框架下 ,交通安全技术手段的提高是我国交通安全管理面临的迫切需要解决的问题 ,从而提出只有通过实施分阶段的、递进的安全管理对策和开展长效管理 ,提高交通安全技术 ,建立“点—线—面”的立体控制系统和道路交通安全保障体系 ,才能提高我国交通系统的整体安全性能 相似文献
9.
测定环境空气中微量氟的方法一般采用滤膜法,但此法工作量大,针对这种情况,本文作两点改进:一是将采集的两张滤膜同时测定;二是将测定过程中的搅拌时间缩短,这样不影响测定结果的准确性,而且降低了工作量。 相似文献
10.
乌鲁木齐空气微生物含量的测定 总被引:2,自引:0,他引:2
用自然平皿沉降法对乌鲁木齐市13个室内外空气测点作了微生物含量的测定,结果表明平均室外空气的细菌、真菌、总菌含量及F/T%分别为28583 8、780 5、29364 3CFU·m-3及2 7,证实了该市空气处于中度微生物污染状态。少量测点显示其空气已受到严重污染,空气质量不佳。室内空气微生物污染也重。空气微生物污染以细菌为主。分析了室外空气微生物含量的时空分布特点差异,探讨了其成因,并与其他城市作了比较。文章指出增强环境忧患意识,采用切实而有效措施,减少环境污染的必要性。 相似文献