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Masahide Aikawa Toshimasa Ohara Takatoshi Hiraki Okihiro Oishi Akihiro Tsuji Makiko Yamagami Kentaro Murano Hitoshi Mukai 《Atmospheric environment (Oxford, England : 1994)》2010,44(3):381-391
We found a significant geographic gradient (longitudinal and latitudinal) in the sulfate (SO42?) concentrations measured at multiple sites over the East Asian Pacific Rim region. Furthermore, the observed gradient was well reproduced by a regional chemical transport model. The observed and modeled SO42? concentrations were higher at the sites closer to the Asian continent. The concentrations of SO42? from China as calculated by the model also showed the fundamental features of the longitudinal/latitudinal gradient. The proportional contribution of Chinese SO42? to the total in Japan throughout the year was above 50–70% in the control case, using data for Chinese sulfur dioxide (SO2) emission from the Regional Emission Inventory in Asia (40–60% in the low Chinese emissions case, using Chinese SO2 emissions data from the State Environmental Protection Administration of China), with a winter maximum of approximately 65–80%, although the actual concentrations of SO42? from China were highest in summer. The multiple-site measurements and the model analysis strongly suggest that the SO42? concentrations in Japan were influenced by the outflow from the Asian continent, and this influence was greatest in the areas closer to the Asian continent. In contrast, we found no longitudinal/latitudinal gradient in SO2 concentrations; instead SO2 concentrations were significantly correlated with local SO2 emissions. Our results show that large amounts of particulate sulfate are transported over long distances from the East Asian Pacific Rim region, and consequently the SO42? concentrations in Japan are controlled by the transboundary outflow from the Asian continent. 相似文献
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Reiji Noda Masanori Komatsu Eriko Sumi Tadao Kasakura 《Journal of Material Cycles and Waste Management》2001,3(2):118-125
“Zero emissions” is a concept envisaging the creation of a sustainable society with minimal disposal of resources. In order
to realize zero emissions for plastics, it is important to establish a method for quantitatively evaluating candidate recycling
processes. In this study, the principle of the substitution factor (SF) is introduced. A quantitative evaluation of the recycling
process for plastics was then carried out. The production process for monofilament plastics was examined. The recycling of
plastics discarded during the production process could be substituted in small amounts for virgin materials, giving reduced
CO2 emissions. Furthermore, production using recycled material mixed with virgin material was more effective in reducing CO2 emissions than when recycled materials only were used.
Received: November 19, 1999 / Accepted: November 28, 2000 相似文献
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Kimitaka Nishitani Shinji Kaneko Hidemichi Fujii Satoru Komatsu 《Journal of Cleaner Production》2011,19(17-18):1956-1964
This paper analyzes whether the reduction of pollution emissions improves a firm’s economic performance through the increase in sales to environmentally conscious customers and the cost reductions associated with the improvement in productivity. Because the selection of the control (end-of-pipe) or prevention (cleaner production) approach differently influences the effect through the improvement in productivity, this is also considered. Using panel data for Japanese manufacturing firms over the period 2002–2008, the findings indicate that firms that have reduced their pollution emissions can increase their economic performance through the increase in demand for their products and an improvement in productivity. However, the latter is conditional, and so the prevention approach is preferred. 相似文献
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Wickramarachchi P Kawamoto K Hamamoto S Nagamori M Moldrup P Komatsu T 《Waste management (New York, N.Y.)》2011,31(12):2464-2472
Landfill sites are emerging in climate change scenarios as a significant source of greenhouse gases. The compacted final soil cover at landfill sites plays a vital role for the emission, fate and transport of landfill gases. This study investigated the effects of dry bulk density, ρ(b), and particle size fraction on the main soil-gas transport parameters - soil-gas diffusivity (D(p)/D(o), ratio of gas diffusion coefficients in soil and free air) and air permeability (k(a)) - under variably-saturated moisture conditions. Soil samples were prepared by three different compaction methods (Standard and Modified Proctor compaction, and hand compaction) with resulting ρ(b) values ranging from 1.40 to 2.10 g cm(-3). Results showed that D(p) and k(a) values for the '+gravel' fraction (<35 mm) became larger than for the '-gravel' fraction (<2mm) under variably-saturated conditions for a given soil-air content (ε), likely due to enhanced gas diffusion and advection through less tortuous, large-pore networks. The effect of dry bulk density on D(p) and k(a) was most pronounced for the '+gravel' fraction. Normalized ratios were introduced for all soil-gas parameters: (i) for gas diffusivity D(p)/D(f), the ratio of measured D(p) to D(p) in total porosity (f), (ii) for air permeability k(a)/k(a)(,pF4.1), the ratio of measured k(a) to k(a) at 1235 kPa matric potential (=pF 4.1), and (iii) for soil-air content, the ratio of soil-air content (ε) to total porosity (f) (air saturation). Based on the normalized parameters, predictive power-law models for D(p)(ε/f) and k(a)(ε/f) models were developed based on a single parameter (water blockage factor M for D(p) and P for k(a)). The water blockage factors, M and P, were found to be linearly correlated to ρ(b) values, and the effects of dry bulk density on D(p) and k(a) for both '+gravel' and '-gravel' fractions were well accounted for by the new models. 相似文献
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Adsorption of 2,4-dichlorophenoxyacetic acid by an Andosol 总被引:1,自引:0,他引:1
To identify the important soil components involved in 2,4-dichlorophenoxyacetic acid (2,4-D) adsorption on Andosols, 2,4-D adsorption on a surface horizon of an Andosol was compared with that on hydrogen peroxide (H2O2)-treated (soil organic matter [SOM] was removed), acid-oxalate (OX)-treated (active metal hydroxides and SOM were removed), and dithionite-citrate-bicarbonate (DCB)-treated (free and active metal [hydr]oxides and SOM were removed) soil samples at equilibrium pHs ranging from 4 to 8. Although the untreated soil contained a large amount of organic C (71.9 g kg-1), removal of SOM had little effect on 2,4-D adsorption. Active surface hydroxyls, which were attached to the active and free metal (hydr)oxides and metal SOM complexes, were identified as the most important soil functional group for 2,4-D adsorption. The dominant mechanism of the 2,4-D adsorption was a ligand exchange reaction in which the carboxylic group of 2,4-D displaced the active surface hydroxyl associated with metals and formed a strong coordination bond between the 2,4-D molecule and soil solid phase. The ligand exchange reaction reasonably accounted for the selective adsorption of 2,4-D over Cl-, competitive adsorption of phosphate over 2,4-D, reduction in plant-growth-inhibitory activity of soil-adsorbed 2,4-D, and the high 2,4-D adsorption ability of Andosols. Although a humic acid purified from the soil did not adsorb 2,4-D, the presence of the humic acid increased 2,4-D adsorption on Al and Fe, probably by inhibiting the hydrolysis and polymerization of Al and Fe resulting in the preservation of available adsorption sites on these metals. The adsorption behavior of 2,4-D on soils could be a good index for predicting the adsorption behavior of other organic acids in soils. 相似文献
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IntroductionHakataBayisasemi enclosedbay(from 33°34′Nto 33°41′Nandfrom 1 30°1 3′Eto 1 30°2 6′E)locatedatthenorthsideofKyushuIsland ,Japan .ThelengthandwidthofHakataBayisabout2 0kmand 1 0kmrespectively .Thesurfaceareaisabout 1 33km2 andthemeanwaterdepthisabout1 0 .5m .Thebaymout… 相似文献