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Removal of copper from aqueous solution by Ascophyllum nodosum immobilised in hydrophilic polyurethane foam 总被引:2,自引:0,他引:2
The seaweed Ascophyllum nodosum was pre-treated by successive washes in distilled water and dilute acid, dried, and pulverised to produce particles of <150 microm. These were immobilised during the manufacturing process of Hypol 2002 polymer to form a biomass/polymer matrix that was stable and easy to handle. In making the composite a mixing speed of 360 rpm for 20-30 s with 2% (w/w) addition of surfactant to pre-polymer was found to be ideal. The average pore sizes for different water polymer mixes (expressed as volume ratios) were 1.66 mm +/- 0.98 (ratio 0.75:1), 1.58 mm +/- 0.76 (ratio 1:1), 1.64 mm +/- 0.6 (ratio 1.5:1) and 1.11 mm +/- 0.615 (ratio 2:1). The biomass/polymer was used alongside free native biomass in an initial adsorption experiment using a 0.0315 mmol dm(-3) Cu (II) solution and gave a copper uptake capacity [Formula: see text] of 0.037 mmol Cu g(-1) dry weight seaweed in both cases which represented approximately 85% of total initially available copper. In later adsorption isotherm experiments using Cu concentrations between 0.0315 and 0.944 mmol dm(-3) at pH 5.0 and immobilized biomass over five consecutive adsorption/desorption cycles the biomass/polymer showed an initial lowering of adsorption capacity but stabilised at 0.23 mmol g(-1) dry weight by the third re-use. The q(max) of the immobilised biomass decreased from 0.55 and 0.416 mmol of Cu g(-1) dry weight when pH was lowered from 4.0 to 3.0, and increased from 0.576 mmol g(-1) dry weight (biomass) at 283 K to 0.636 mmol g(-1)(biomass) at 303 K. 相似文献
44.
F.E. Banks 《Resources Policy》1977,3(1):2-12
This paper treats some of the more important aspects of natural resource availability. This includes a definition of real or opportunity costs in resource extraction as compared to money costs; some economics of secondary materials and recycling; energy resources; and a demonstration of the effect of exponential growth in resource use on the time to resource exhaustion. The paper concludes with a short note on econometrics and commodity models. 相似文献
45.
Glenn Banks 《Natural resources forum》2003,27(3):223-234
The involvement of local communities as equity holders in major mineral resource developments dates back over a decade in Papua New Guinea. This article reviews the history and result of landowner equity at two of Papua New Guinea's major mines (Porgera and Lihir), with a particular focus on the contribution of these equity holdings to local sustainable development. It is found that while an equity holding can provide significant returns to a local community, it also exposes them to significant financial risk. A second major area of concern is the structures and instruments by which revenues generated from the equity are distributed and utilized within the local community. Further research and policy redirection is required before local equity holding can be viewed as making a significant contribution to local sustainable development. 相似文献
46.
Banks D Adam AM Bayliss V Hogg GM Bleuten W Dees M Karnachuk OV Le Blansch K Marquand J 《Environmental management》2000,26(1):35-46
/ Implementation of environmental management in Russia is undergoing rapid changes. Federal responsibility rests with the Russian Federation State Committee for Environmental Protection (RFSCEP) and is delegated at regional level to local State Committees for Environmental Protection (SCEPs). This paper focuses on the functioning of the SCEP for Tomsk oblast' (region) in Siberia, which is strongly committed to forging constructive links with regional government, academia, industry, and environmental NGOs. Considerable difficulties exist for SCEPs in Russia, however, and prominent among these are (1) a rigidly vertical civil service structure, with separate organs having responsibility for different natural resources, persisting from Soviet times, which hinders effective intergrated and holistic environmental management; and (2) a lack of open access to environmental information from military and quasi-military sites. 相似文献
47.
Contaminated sediments dredged from navigable waterways often are placed in confined disposal facilities to prevent further spread of the pollutants. Reducing contaminants to acceptable levels would allow for disposal of the sediments and further dredging activity. A greenhouse study was conducted to evaluate plant treatments and the addition of an organic amendment to decrease the concentration of PCB congeners found in Arochlor 1260. Sediment treated with the amendment and either low transpiring plants or no plants had the greatest removal of the PCB congeners. High-transpiring plants apparently prevented the highly reducing conditions required for reductive dechlorination of highly chlorinated PCBs. Most likely, the amendment provided labile carbon that initiated the reducing conditions needed for dechlorination. The sediment moisture content and moisture-related plant parameters were significant predictors of the PCB loss. Carex aquatalis and Spartina pectinata are predicted to be the most effective plant treatments for phytoremediation of PCBs. 相似文献
48.
We investigated the effects of a warmer climate, and seasonal trends, on the fate of oil spilled in the Arctic. Three well blowout scenarios, two shipping accidents and a pipeline rupture were considered. We used ensembles of numerical simulations, using the OSCAR oil spill model, with environmental data for the periods 2009–2012 and 2050–2053 (representing a warmer future) as inputs to the model. Future atmospheric forcing was based on the IPCC’s A1B scenario, with the ocean data generated by the hydrodynamic model SINMOD. We found differences in “typical” outcome of a spill in a warmer future compared to the present, mainly due to a longer season of open water. We have demonstrated that ice cover is extremely important for predicting the fate of an Arctic oil spill, and find that oil spills in a warming climate will in some cases result in greater areal coverage and shoreline exposure. 相似文献
49.
The application of digital technology in conservation holds much potential for advancing the understanding of, and facilitating interaction with, the natural world. In other sectors, digital technology has long been used to engage communities and share information. Human development—which holds parallels with the nature conservation sector—has seen a proliferation of innovation in technological development. Throughout this Perspective, we consider what nature conservation can learn from the introduction of digital technology in human development. From this, we derive a charter to be used before and throughout project development, in order to help reduce replication and failure of digital innovation in nature conservation projects. We argue that the proposed charter will promote collaboration with the development of digital tools and ensure that nature conservation projects progress appropriately with the development of new digital technologies. 相似文献
50.
Elina Tampio Satu Ervasti Teija Paavola Sonia Heaven Charles Banks Jukka Rintala 《Waste management (New York, N.Y.)》2014,34(2):370-377
Anaerobic digestion of autoclaved (160 °C, 6.2 bar) and untreated source segregated food waste (FW) was compared over 473 days in semi-continuously fed mesophilic reactors with trace elements supplementation, at organic loading rates (OLRs) of 2, 3, 4 and 6 kg volatile solids (VS)/m3 d. Methane yields at all OLR were 5–10% higher for untreated FW (maximum 0.483 ± 0.013 m3 CH4/kg VS at 3 kg VS/m3 d) than autoclaved FW (maximum 0.439 ± 0.020 m3 CH4/kg VS at 4 kg VS/m3 d). The residual methane potential of both digestates at all OLRs was less than 0.110 m3 CH4/kg VS, indicating efficient methanation in all cases. Use of acclimated inoculum allowed very rapid increases in OLR. Reactors fed on autoclaved FW showed lower ammonium and hydrogen sulphide concentrations, probably due to reduced protein hydrolysis as a result of formation of Maillard compounds. In the current study this reduced biodegradability appears to outweigh any benefit due to thermal hydrolysis of ligno-cellulosic components. 相似文献