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排序方式: 共有501条查询结果,搜索用时 234 毫秒
451.
Weijia Zhao Hongyun Niu Yongliang Yang Hongzhou Lv Jungang Lv Yaqi Cai 《环境科学学报(英文版)》2022,34(2):244-257
The construction of heterojunction photocatalysts for efficiently utilizing solar energy has attracted considerable attention to solve the energy crisis and reduce environmental pollution. In this study, we use the energy released from an easily-occurred exothermic chemical reaction to serve as the drive force to trigger the formation of Cd S and C3N4 nanocomposites which are successfully fabricated with cadmium nitrate and thiourea without addition of any solvents and prot... 相似文献
452.
Enhui Wu Daifeng Lin Yinye Chen Xiaoshan Feng Kui Niu Yongjin Luo Baoquan Huang Jianbin Qiu Qingrong Qian Qinghua Chen 《环境科学学报(英文版)》2022,34(6):79-89
A series of nitrogen-doped CoAlO (N-CoAlO) were constructed by a hydrothermal route combined with a controllable NH3 treatment strategy. The effects of NH3 treatment on the physico-chemical properties and oxidation activities of N-CoAlO catalysts were investigated. In comparison to CoAlO, a smallest content decrease in surface Co3+ (serving as active sites) while a largest increased amount of surface Co2+ (contributing to oxygen species) are obtained over N-CoAlO/4h among the N-CoAlO catalysts. Meanwhile, a maximum N doping is found over N-CoAlO/4h. As a result, N-CoAlO/4h (under NH3 treatment at 400°C for 4 hr) with rich oxygen vacancies shows optimal catalytic activity, with a T90 (the temperature required to reach a 90% conversion of propane) at 266°C. The more oxygen vacancies are caused by the co-operative effects of N doping and suitable reduction of Co3+ for N-CoAlO/4h, leading to an enhanced oxygen mobility, which in turn promotes C3H8 total oxidation activity dominated by Langmuir-Hinshelwood mechanism. Moreover, in situ diffuse reflectance infrared Fourier transform spectroscopy (DRIFTs) analysis shows that N doping facilities the decomposition of intermediate species (propylene and formate) into CO2 over the catalyst surface of N-CoAlO/4h more easily. Our reported design in this work will provide a promising way to develop abundant oxygen vacancies of Co-based catalysts derived from hydrotalcites by a simple NH3 treatment. 相似文献
453.
采用混凝沉淀法处理污泥水中的悬浮固体和磷,考察了聚合氯化铝(PAC)、聚硫氯化铝(PACS)以及PAC和阴离子聚丙烯酰胺(aPAM)复配不同投加量对污泥水沉降性能和磷去除的影响。实验结果表明,PAC和PACS混凝处理污泥水效果基本一致,会恶化污泥水沉降,且随PAC投药量的增加,污泥水SV30越大。PAC与aPAM复配混凝处理污泥水,也难以改善污泥水的沉降性能。结果表明,铝盐混凝剂不适合同步去除污泥水悬浮固体和磷,建议先寻求其它混凝剂改善污泥水沉降再用铝盐除磷。 相似文献
454.
Size and elemental composition of dry-deposited particles during a severe dust storm at a coastal site of Eastern China 总被引:1,自引:0,他引:1
Hongya Niu Daizhou Zhang Wei Hu Jinhui Shi Ruipeng Li Huiwang Gao Wei Pian Min Hu 《环境科学学报(英文版)》2016,28(2):161-168
Dry-deposited particles were collected during the passage of an extremely strong dust storm in March, 2010 at a coastal site in Qingdao(36.15°N, 120.49°E), a city located in Eastern China. The size, morphology, and elemental composition of the particles were quantified with a scanning electron microscope equipped with an energy dispersive X-ray instrument(SEM–EDX). The particles appeared in various shapes, and their size mainly varied from 0.4to 10 μm, with the mean diameters of 0.5, 1.5, and 1.0 μm before, during, and after the dust storm, respectively. The critical size of the mineral particles settling on the surface in the current case was about 0.3–0.4 μm before the dust storm and about 0.5–0.7 μm during the dust storm. Particles that appeared in high concentration but were smaller than the critical size deposited onto the surface at a small number flux. The elements Al, Si and Mg were frequently detected in all samples, indicating the dominance of mineral particles. The frequency of Al in particles collected before the dust storm was significantly lower than for those collected during and after the dust storm. The frequencies of Cl and Fe did not show obvious changes, while those of S, K and Ca decreased after the dust arrival. These results indicate that the dust particles deposited onto the surface were less influenced by anthropogenic pollutants in terms of particle number. 相似文献
455.
为明确自行筛选开发的高效降解菌对鸡粪发酵的影响,分析研究了其堆肥的主要腐熟指标。结果表明,加入高效降解菌剂的堆肥处理方法温度相对较高,脱水快,pH值适宜,C/N调整较好,种子发芽指数高,堆肥后营养养分含量高,且大肠菌群数量少,堆肥效果较好。 相似文献
456.
Niu Yayi Li Yuqiang Wang Mingming Wang Xuyang Chen Yun Duan Yulong 《Environmental science and pollution research international》2022,29(4):5295-5312
Environmental Science and Pollution Research - Sandy cropland ecosystems are major terrestrial ecosystems in semi-arid regions of northern China’s Horqin Sandy Land, where they play an... 相似文献
457.
Yang Ping Wang Nai’ang Zhao Liqiang Su Bingjie Niu Zhenmin Zhao Hang 《Environmental science and pollution research international》2022,29(50):75805-75821
Environmental Science and Pollution Research - Studying the effects of precipitation on carbon exchange in grassland ecosystems is critical for revealing the mechanisms of the carbon cycle. In this... 相似文献
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