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971.
Although the approach using non-thermal plasma (NTP) for deNOx has been studied for over 15 years, how to achieve higher removal
e ciency with lower cost is still a barrier for its industrial application. In order to investigate the impact of the argon additive on electron
density, energy and nitric oxide reduction process in plasma, the spectrum of the dielectric barrier discharge at atmospheric pressure in
a coaxial reactor was measured using the monochromater with high resolution. The comparative experiments for NO reduction were
carried out simultaneously in N2/O2/NO plasma stream with and without argon, respectively. The nitrogen molecular spectrum which
is attributed to the energy level transition (C3 u ! B3 g) was compared in the wavelength range 300–480 nm and the electron density
and temperature were determined based on the relative intensities and Stark broadening width of spectral lines. The spectrum results
indicated that the argon additive could enhance the intensity of emissive spectrum of plasma, thus the electron concentration as well as
the energy was increased, and finally prompted the ionization rate to produce active N, O and O3. The results of NO reduction showed
that NO conversion e ciency increased in the range of 10%–30% with 5% addition of argon in stream comparing with the condition
without argon additive. This study will play a positive role in the industrial application of dielectric barrier discharge deNOx reactor. 相似文献
972.
973.
垃圾渗滤液是一种成分复杂、有机物、氨氮浓度高的难处理废水,介绍了高级氧化技术在垃圾渗滤液处理中的研究与应用现状。主要介绍了臭氧氧化、光催化氧化、Fenton试剂、电氧化以及湿式氧化在处理垃圾渗滤液中的应用,分析了高级氧化技术处理垃圾渗滤液的原理,对国内外各种氧化技术在垃圾渗滤液处理中的应用进行了总结,并探讨了它们的优缺点。最后,提出了当前应用高级氧化技术处理垃圾渗滤液所存在的问题和发展方向。 相似文献
974.
Huilong Wang Shuqin Liu Hui Wang Wenfeng Jiang 《Frontiers of Environmental Science & Engineering》2010,4(3):311-320
Multi-walled carbon nanotubes (MWCNTs)/TiO2 composite photocatalysts with high photoactivity were prepared by sol-gel process and further characterized by X-ray diffraction (XRD), scanning electron microscopy (SEM), Fourier transform infrared (FT-IR), and UV-vis absorption spectra. Compared to pure TiO2, the combination of MWCNTs with titania could cause a significant absorption shift toward the visible region. The photocatalytic performances of the MWCNTs/TiO2 composite catalysts were evaluated for the decomposition of Reactive light yellow K-6G (K-6G) and Mordant black 7 (MB 7) azo dyes solution under solar light irradiation. The results showed that the addition of MWCNTs enhanced the adsorption and photocatalytic activity of TiO2 for the degradation of azo dyes K-6G and MB 7. The effect of MWCNTs content, catalyst dosage, pH, and initial dye concentration were examined as operational parameters. The kinetics of photocatalytic degradation of two dyes was found to follow a pseudo-first-order rate law. The photocatalyst was used for seven cycles with photocatalytic degradation efficiency still higher than 98%. A plausible mechanism is also proposed and discussed on the basis of experimental results. 相似文献
975.
基于土地利用变化的小江流域非点源污染特征 总被引:9,自引:2,他引:7
选取三峡库区典型支流——小江流域为研究对象,以GIS软件为分析工具,在L-THIA模型的基础上,分析小江流域非点源污染物负荷量随土地利用方式改变而产生的时空变化特征. 结果表明:2007年小江流域非点源污染物TN和TP总负荷量分别为5 563.11和1 550.65 t,其中旱地的污染物负荷量最大,TN和TP负荷量分别达到4 633.43和1 368.96 t,占总负荷量的83.29%和88.29%;从空间分布上看,非点源污染主要集中在旱地较多的东河流域和南河流域;而从时间分布上看,随着旱地面积的大幅增加,1995—2007年小江流域污染物负荷量明显增加. 相似文献
976.
Wang Chunlei Yang Ye Wu Nanxiang Gao Ming Tan Yufeng 《Environmental Chemistry Letters》2019,17(4):1693-1706
Environmental Chemistry Letters - Co-occurrence of pyrethroid insecticides and heavy metals in the environment may produce combined toxic effects that are higher or lower than toxic... 相似文献
977.
Jiaquan Zhang Shihua Qi Xinli Xing Lingzhi Tan Wei Chen Ying Hu Dan Yang Chenxi Wu 《Frontiers of Environmental Science & Engineering》2012,6(2):177-183
Soil is an important source to other environmental media and organisms for organochlorine pesticides (OCPs) bioaccumulation. Twenty-four representative surface soil samples were collected from the lower reaches of the Jiulong River, China, in 2009. The concentrations of hexachlorocyclohexane isomers (HCHs) ranged from 0.38 to 39.52 ng·g?1, with a mean value of 9.51 ng·g?1. The concentrations of dichlorodiphenyltrichloroethanes (DDTs) and their metabolites were within the ranges of 0.94–700.99 ng·g?1, with a mean value of 71.17 ng·g?1. The concentrations of HCHs and DDTs in the soil were lower than the first grade level (50 ng·g?1) of the Chinese Environmental Quality Standard (GB15618-1995). Hierarchical Cluster Analysis (HCA) and Pearson’s bivariate Correlations Analysis (PCA) were used to analyse the distribution and contamination levels of OCPs in this region. The results showed that DDTs were the major contaminants and there were no significant correlations between various OCPs concentrations and the total organic carbon (TOC) contents. A significant positive correlation was observed between HCHs and DDTs (p<0.01), which indicates that HCHs and DDTs may have similar sources and fate in the study area. 相似文献
978.
979.
华北典型污灌区有机氯农药残留特征及健康风险评价 总被引:2,自引:0,他引:2
在我国华北地区由于水资源的匮乏及农业生产的需要,采用污水灌溉与施用有机氯农药(OCPs)结合的农业管理方式普遍存在。大量OCPs则被引入到当地环境中,进而可能对该地区的居民产生潜在的健康风险。本研究分析石家庄市汪洋沟污灌区OCPs的残留状况,探讨污水灌溉条件下土壤-作物系统OCPs残留对土壤质量影响,并评价经口摄入及皮肤接触两种暴露途径下对人体产生的健康风险。结果表明:汪洋沟污灌区地表水、沉积物、土壤和玉米籽粒中检出了14种OCPs,其平均残留浓度分别为36.5 ng·L~(-1)、62.9 ng·g~(-1)、57.3 ng·g~(-1)和27.0 ng·g~(-1),滴滴涕(DDTs)是其最主要的污染物,占OCPs的73%以上,其次是六六六(HCHs)和甲氧滴滴涕。р,р'-DDT是DDTs的最主要成分,其主要来源于污水灌溉或近期DDTs的使用。γ-HCH是环境HCHs残留的主要成分,其主要来源于林丹的输入和使用。此外,在该地区污灌条件下OCPs残留对土壤中C、N循环及有机S的矿化产生一定的负面影响。研究区OCPs残留对人体产生的非致癌风险和致癌风险均不超过控制标准,但经口摄入所引致的非致癌风险应予以关注,其中р,р'-DDT与γ-HCH为主要风险物质。 相似文献
980.
The adsorption of six PCB congeners to natural sediments from the Yangtse River was investigated. Experiments were conducted at different PCB concentrations to get the adsorption isotherm for each compound. Analytical determinations were carried out using gas chromato‐graphy with ECD detector. Results showed that the adsorption mechanism of PCBs on Yangtse River sediment fitted the best to the Langmuir adsorption model. It was also found that the adsorption rate decreased as the solubility increased or the octanol‐water partition coefficient decreased for each compound. 相似文献