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61.
Anwar Zahid M. Q. Hassan G. N. Breit K.-D. Balke Matthias Flegr 《Environmental geochemistry and health》2009,31(Z1):69-84
Accumulations of iron, manganese, and arsenic occur in the Chandina alluvium of southeastern Bangladesh within 2.5 m of the
ground surface. These distinctive orange-brown horizons are subhorizontal and consistently occur within 1 m of the contact
of the aerated (yellow-brown) and water-saturated (gray) sediment. Ferric oxyhydroxide precipitates that define the horizons
form by oxidation of reduced iron in pore waters near the top of the saturated zone when exposed to air in the unsaturated
sediment. Hydrous Fe-oxide has a high specific surface area and thus a high adsorption capacity that absorbs the bulk of arsenic
also present in the reduced pore water, resulting in accumulations containing as much as 280 ppm arsenic. The steep redox
gradient that characterizes the transition of saturated and unsaturated sediment also favors accumulation of manganese oxides
in the oxidized sediment. Anomalous concentrations of phosphate and molybdenum also detected in the ferric oxyhydroxide-enriched
sediment are attributed to sorption processes. 相似文献
62.
Matthias Demuzere Nicole P.M. van Lipzig 《Atmospheric environment (Oxford, England : 1994)》2010,44(10):1341-1355
In order to make projections for future air-quality levels, a robust methodology is needed that succeeds in reconstructing present-day air-quality levels. At present, climate projections for meteorological variables are available from Atmospheric-Ocean Coupled Global Climate Models (AOGCMs) but the temporal and spatial resolution is insufficient for air-quality assessment. Therefore, a variety of methods are tested in this paper in their ability to hindcast maximum 8 hourly levels of O3 and daily mean PM10 from observed meteorological data. The methods are based on a multiple linear regression technique combined with the automated Lamb weather classification. Moreover, we studied whether the above-mentioned multiple regression analysis still holds when driven by operational ECMWF (European Center for Medium-Range Weather Forecast) meteorological data. The main results show that a weather type classification prior to the regression analysis is superior to a simple linear regression approach. In contrast to PM10 downscaling, seasonal characteristics should be taken into account during the downscaling of O3 time series. Apart from a lower explained variance due to intrinsic limitations of the regression approach itself, a lower variability of the meteorological predictors (resolution effect) and model deficiencies, this synoptic-regression-based tool is generally able to reproduce the relevant statistical properties of the observed O3 distributions important in terms of European air quality Directives and air quality mitigation strategies. For PM10, the situation is different as the approach using only meteorology data was found to be insufficient to explain the observed PM10 variability using the meteorological variables considered in this study. 相似文献
63.
Jörn Budde Monika Heiermann Teresa Suárez Quiñones Matthias Plöchl 《Waste management (New York, N.Y.)》2014,34(2):522-529
Lab-scale experiments were conducted to assess the impact of thermobarical treatment of cattle waste on anaerobic digestion. Treatment was at temperatures of 140–220 °C in 20 K steps for a 5-min duration. Methane yields could be increased by up to 58% at a treatment temperature of 180 °C. At 220 °C the abundance of inhibitors and other non-digestible substances led to lower methane yields than those obtained from untreated material. In an extended analysis it could be demonstrated that there is a functional correlation between the methane yields after 30 days and the formation rate and methane yield in the acceleration phase. It could be proved in a regression of these correlation values that the optimum treatment temperature is 164 °C and that the minimum treatment temperature should be above 115 °C. 相似文献
64.
Zhi C. Lin John M. Ondov W. Robert Kelly Paul J. Paulsen Robert K. Stevens 《Journal of the Air & Waste Management Association (1995)》2013,63(8):1057-1062
Stable isotopic tracers were used in Roanoke, Virginia, to tag particulate emissions from diesel trucks and residential oil furnaces, two sources of soot and PAHs which cannot be differentiated on the basis of known constituents. Approximately 1.6 g of enriched 149Sm were used to tag 264 m3 of diesel fuel burned by the city bus and truck fleets; 0.39 g of 150Sm were used to tag 106 m3 of residential heating oil. Picogram amounts of the tracers were determined simultaneously by thermal-ionization mass spectrometry in fine particles collected within the city at signal-to-noise ratios as large as 6000. These results demonstrate the feasibility of tracing particles from multiple combustion sources with stable, separated isotopes. 相似文献
65.
Wolke Tobón Tania Urquiza‐Haas Patricia Koleff Matthias Schröter Rubén Ortega‐Álvarez Julio Campo Roberto Lindig‐Cisneros José Sarukhán Aletta Bonn 《Conservation biology》2017,31(5):1086-1097
Ecological restoration has become an important strategy to conserve biodiversity and ecosystems services. To restore 15% of degraded ecosystems as stipulated by the Convention on Biological Diversity Aichi target 15, we developed a prioritization framework to identify potential priority sites for restoration in Mexico, a megadiverse country. We used the most current biological and environmental data on Mexico to assess areas of biological importance and restoration feasibility at national scale and engaged stakeholders and experts throughout the process. We integrated 8 criteria into 2 components (i.e., biological importance and restoration feasibility) in a spatial multicriteria analysis and generated 11 scenarios to test the effect of assigning different component weights. The priority restoration sites were distributed across all terrestrial ecosystems of Mexico; 64.1% were in degraded natural vegetation and 6% were in protected areas. Our results provide a spatial guide to where restoration could enhance the persistence of species of conservation concern and vulnerable ecosystems while maximizing the likelihood of restoration success. Such spatial prioritization is a first step in informing policy makers and restoration planners where to focus local and large‐scale restoration efforts, which should additionally incorporate social and monetary cost–benefit considerations. 相似文献
66.
Baumann Matthias Israel Christoph Piquer-Rodríguez María Gavier-Pizarro Gregorio Volante José Norberto Kuemmerle Tobias 《Regional Environmental Change》2017,17(4):1179-1191
Regional Environmental Change - The dry forests of Latin America are among the most dynamic deforestation frontiers in the world and are important carbon and biodiversity reservoirs. Our knowledge... 相似文献
67.
68.
Lakes in surface mining areas are often subject to continuous loads of acid mine drainage. The knowledge of internal alkalinity generation in a lake is necessary to predict if the lake will stay circumneutral or may acidify. The most important processes of alkalinity production in lakes are sulfate reduction, denitrification, and the burial of N in the sediment. By summarizing data from the literature, we present probable rates of these different processes in circumneutral mining lakes. The critical acidity load that can probably be compensated for by internal processes, is 5.09 mmol(-) m(-2) d(-1) in productive lakes and 0.50 mmol(-) m(-2) d(-1) in less productive lakes. Under the assumption that methanogenesis is inhibited by high sulfate concentrations, the highest probable acidity loads in such lakes are 6.85 mmol(-) m(-2) d(-1) and 1.06 mmol(-) m(-2) d(-1), respectively. Denitrification, sulfate reduction, and N burial contributed significantly to total alkalinity production. Sulfate reduction had the largest potential. However, existing models cannot predict alkalinity generation from sulfate concentrations alone because the long-term stability of reduced S compounds in the sediment is crucial for a sustainable biological alkalinity generation. The larger acid-neutralizing potential of higher trophic lakes is caused both by higher rates of microbial activity and by a greater stability of reduced reaction products in the sediment. The largest uncertainties in our knowledge with respect to the total alkalinity budget are related to microbial processes in sulfate-rich freshwater lakes and the long-term stability of reduced reaction products in the sediment. 相似文献
69.
We used stable isotopes to examine the incorporation of plant carbon into the belowground food web of an agricultural system. Plots were established and planted with maize (Zea mays) in a rye field (Secale cereale) near G?ttingen (northern Germany) in May 1999. In October 1999, April 2000, and October 2000, meso- and macrofauna and maize and rye litter were collected in each plot and analyzed for 13C and 15N content. 15N signatures suggested that the soil animal species analyzed span three trophic levels with the trophic position of species varying little in time. The species investigated formed a continuum from primary to secondary decomposers to predators. On average, predator species differed from primary and secondary decomposers by 3.9 sigma15N suggesting that they fed on a mixed diet of both decomposer groups. The combined analysis of 13C and 15N signatures allowed us to identify links between prey and consumer species. In October 1999, shortly after maize residues had been incorporated into the plots, maize-born carbon was present in each of the animal species investigated, including top predators. The incorporation of maize carbon into the belowground food web increased during the following 12 months but the concentration of maize-born carbon never exceeded 50% in any of the species. Furthermore, the ranks of the incorporation of maize-born carbon of the species changed little. The results suggest that the belowground food web relies heavily on carbon originating from plant residues from before the recent two growing seasons. In most species the amount of maize-born carbon increased continuously; however, in some species it decreased during winter, suggesting that these species switched to a diet based more on C3 plants during winter, or predominantly metabolized carbon incorporated during the last growing season. The study documents that the combined analysis of 13C and 15N signatures in soil invertebrate species, after replacement of C3 by C4 plants, is a powerful tool to better understand the structure of the belowground food web and the flux of carbon through it. 相似文献
70.
Charkovska Nadiia Halushchak Mariia Bun Rostyslav Nahorski Zbigniew Oda Tomohiro Jonas Matthias Topylko Petro 《Mitigation and Adaptation Strategies for Global Change》2019,24(6):907-939
Mitigation and Adaptation Strategies for Global Change - Industrial processes cause significant emissions of greenhouse gases (GHGs) to the atmosphere and, therefore, have high mitigation and... 相似文献