全文获取类型
收费全文 | 345篇 |
免费 | 0篇 |
国内免费 | 11篇 |
专业分类
安全科学 | 8篇 |
废物处理 | 26篇 |
环保管理 | 26篇 |
综合类 | 34篇 |
基础理论 | 51篇 |
环境理论 | 1篇 |
污染及防治 | 169篇 |
评价与监测 | 19篇 |
社会与环境 | 19篇 |
灾害及防治 | 3篇 |
出版年
2023年 | 9篇 |
2022年 | 20篇 |
2021年 | 19篇 |
2020年 | 7篇 |
2019年 | 7篇 |
2018年 | 9篇 |
2017年 | 19篇 |
2016年 | 8篇 |
2015年 | 9篇 |
2014年 | 9篇 |
2013年 | 44篇 |
2012年 | 17篇 |
2011年 | 25篇 |
2010年 | 16篇 |
2009年 | 10篇 |
2008年 | 12篇 |
2007年 | 20篇 |
2006年 | 23篇 |
2005年 | 10篇 |
2004年 | 13篇 |
2003年 | 9篇 |
2002年 | 7篇 |
2001年 | 5篇 |
2000年 | 4篇 |
1998年 | 2篇 |
1997年 | 3篇 |
1996年 | 4篇 |
1995年 | 1篇 |
1994年 | 2篇 |
1993年 | 1篇 |
1991年 | 1篇 |
1990年 | 1篇 |
1989年 | 1篇 |
1988年 | 1篇 |
1987年 | 1篇 |
1985年 | 1篇 |
1983年 | 2篇 |
1982年 | 1篇 |
1980年 | 1篇 |
1978年 | 2篇 |
排序方式: 共有356条查询结果,搜索用时 211 毫秒
81.
A procedure for the determination of 13 organophosphate insecticides (OPs) in water, sediment and biota at low ppb levels is described. Samples were extracted with dichloromethane or acetone/hexane and cleaned up with micro-column silica gel chromatography. Measurements were made by dual capillary column gas chromatography using both nitrogen-phosphorus (NPD) and electron capture (ECD) detection. Recoveries from fortified water samples ranged from 76% to 102% for all sample types. Practical detection limits ranged between 0.003 and 0.029 microg/l in natural water samples, 0.0004-0.005 microg/g w.w. for sediments, and 0.001-0.005 microg/g w.w for biota using the NPD and ECD method. Losses in sediments were experienced when sulphur was removed. Precision and accuracy were not affected in sediment samples where sulphur was not removed. 相似文献
82.
Preparation of sulfurized powdered activated carbon from waste tires using an innovative compositive impregnation process 总被引:1,自引:0,他引:1
Yuan CS Lin HY Wu CH Liu MH Hung CH 《Journal of the Air & Waste Management Association (1995)》2004,54(7):862-870
The objective of this study is to develop an innovative compositive impregnation process for preparing sulfurized powdered activated carbon (PAC) from waste tires. An experimental apparatus, including a pyrolysis and activation system and a sulfur (S) impregnation system, was designed and applied to produce sulfurized PAC with a high specific surface area. Experimental tests involved the pyrolysis, activation, and sulfurization of waste tires. Waste-tire-derived PAC (WPAC) was initially produced in the pyrolysis and activation system. Experimental results indicated that the Brunauer-Emmett-Teller (BET) surface area of WPAC increased, and the average pore radius of WPAC decreased, as water feed rate and activation time increased. In this study, a conventional direct impregnation process was used to prepare the sulfurized PAC by impregnating WPAC with sodium sulfide (Na2S) solution. Furthermore, an innovative compositive impregnation process was developed and then compared with the conventional direct impregnation process. Experimental results showed that the compositive impregnation process produced the sulfurized WPAC with high BET surface area and a high S content. A maximum BET surface area of 886 m2/g and the S content of 2.61% by mass were obtained at 900 degrees C and at the S feed ratio of 2160 mg Na2S/g C. However, the direct impregnation process led to a BET surface area of sulfurized WPAC that decreased significantly as the S content increased. 相似文献
83.
Hung Ming-Feng Chie Bin-Tzong Huang Tai-Hsin 《Environmental Economics and Policy Studies》2017,19(2):249-268
Environmental Economics and Policy Studies - Residential water demand has long been an important topic of empirical research. How to estimate water waste, however, has rarely been touched. Using... 相似文献
84.
Hanh Pham Thi Minh Nghi Duong Thanh Lan Tran Dinh Van Quan Nguyen Ba Dang The Viet Pham Hung 《Environmental geochemistry and health》2019,41(1):381-390
Environmental Geochemistry and Health - Polychlorinated biphenyls (PCBs), well-known as an important scientific achievement, are now considered as one of the most persistent organic pollutants... 相似文献
85.
Abstract Total organic carbon, humic substances, and the species of trace metals (including Cu, Zn, Pb, Cd, Cr, Mn and Fe) in six and seven phases, such as bioexchangeable (P1), skeletal (carbonates, P2), easily reducible (Fe and Mn oxides, P3), moderately reducible (crystalline Mn oxides, P4), organic matters with sulphides (P5), and detritus with minerals (P6) as well as organic with humic substances (PB4) and organic residues (PB6), were analyzed in sediments from the Taiwan Erhjin coastal (including river and estuarine) area, where places we found the copper pollution. Results indicate that higher percentages of P1 and P2 for copper, zinc, lead, cadmium and manganese in samples collected in March and September of 1990 were much higher than those in P3-P6. High percentages of chromium and iron in samples respectively collected in March and September of 1990 were found in P6. for the seven phase analysis, higher percentages of copper species in PB4 and PB6 as well as iron species in PB7 were observed. On the other hand, purified humic acid with the high contents of manganese and iron in humic acid as well as purified fulvic acids were generally found at the upstream stations; and low values at coastal stations. However, extremely high copper (as high as 1750μg g?1, dry weight in fulvic acid and 820μg g?1 in humic acid) and lead (821μg g?1 in humic acid) concentrations with relatively high manganese and iron concentrations were observed in humic substances from the station near the copper recycling area. Comparing the results obtained from the Antarctic Ocean sediments with those from the Taiwan Erhjin Chi coastal sediments, the human impacts on the latter are evaluated. 相似文献
86.
87.
There is a lack of information concerning human health risks due to exposure to mercury contained in shark fins, through dietary intake. Health risk assessment of shark fins, collected from 5 cities in China: Hong Kong (HK), Beijing, Shanghai (SH), Haikou (HN) and Wenzhou (WZ), was conducted, based on total mercury and methylmercury, and analyzed by a cold vapor atomic fluorescence spectrometry equipped with high-performance liquid chromatography, respectively. The results showed that 16.8 % samples from HK, 8.3 % from SH, 33.3 % from HN, and 16.8 % from WZ were regarded as unsafe for human consumption. Extremely high consumption rates of shark fins for an adult and a child (0.150 and 0.0807 kg/day, respectively), at 95th centile, samples from WZ demonstrated high non-cancer risks (adverse health effects) (Hazard Quotient = 16.0) on adults (aged 25–65), and samples from SH, HN and WZ also showed high non-cancer risks (Hazard Quotient = 12.9, 21.0, and 34.4, respectively) on children (aged 1–7). Consumption of shark fins may be detrimental to human health. 相似文献
88.
Total organic carbon, humic substances, and the species of trace metals (including Cu, Zn, Pb, Cd, Cr, Mn and Fe) in six and seven phases, such as bioexchangeable (P1), skeletal (carbonates, P2), easily reducible (Fe and Mn oxides, P3), moderately reducible (crystalline Mn oxides, P4), organic matters with sulphides (P5), and detritus with minerals (P6) as well as organic with humic substances (PB4) and organic residues (PB6), were analyzed in sediments from the Taiwan Erhjin coastal (including river and estuarine) area, where places we found the copper pollution. Results indicate that higher percentages of P1 and P2 for copper, zinc, lead, cadmium and manganese in samples collected in March and September of 1990 were much higher than those in P3-P6. High percentages of chromium and iron in samples respectively collected in March and September of 1990 were found in P6. for the seven phase analysis, higher percentages of copper species in PB4 and PB6 as well as iron species in PB7 were observed. On the other hand, purified humic acid with the high contents of manganese and iron in humic acid as well as purified fulvic acids were generally found at the upstream stations; and low values at coastal stations. However, extremely high copper (as high as 1750μg g-1, dry weight in fulvic acid and 820μg g-1 in humic acid) and lead (821μg g-1 in humic acid) concentrations with relatively high manganese and iron concentrations were observed in humic substances from the station near the copper recycling area. Comparing the results obtained from the Antarctic Ocean sediments with those from the Taiwan Erhjin Chi coastal sediments, the human impacts on the latter are evaluated. 相似文献
89.
This study investigates the distributions and enrichments of trace metals in suspended and sinking particulate matter from southern East China Sea (ECS) north of Taiwan during the period April 1992 to April 1993. According to these results, concentration of suspended particulate matter in the inner shelf of southern China Sea, the upwellinginfluenced shelf break, and in Kuroshio water are 1.30 (surface)-4.2 (bottom) mg1-1, ca. 0.4 mg1-1 and 0.1-0.2 mg1-1, respectively, reflecting various influences of terrestrial inputs. A benthic nepheloid layer (BNL), apparently owing to resuspension of local and/or remote bottom sediments, formed over the shelf region. Temporal variations in trace metal contents and enrichments in suspended matter from the shelf region reflect the variation of metal inputs from Chinese rivers, particularly from the Changjiang runoff. the enriched metals are more likely to be derived from anthropogenic input, rather than from biological accumulation. in addition, a decrease in metal contents and an increase in salinity confirm the transport of suspended particulate metals from the East China Sea shelf to the open ocean. the feature of metal plume in the intermediate layer (550-800m) of Kuroshio water also verifies this occurrence. Moreover, the sinking particles collected from a sediment trap on the upper slope are relatively enriched in lithogenic matter and trace metals, suggesting the deposit of anthropogenic metals in the slope area. 相似文献
90.
Kosuke Toshiki Pham Quy Giang Kevin Roy B.Serrona Takahiro Sekikawa Jeoung-soo Yu Baasandash Choijil Shoichi Kunikane 《环境科学学报(英文版)》2015,28(2):178-186
Currently, most developing countries have not set up municipal solid waste management systems with a view of recovering energy from waste or reducing greenhouse gas emissions. In this article, we have studied the possible effects of introducing three energy recovery processes either as a single or combination approach, refuse derived fuel production,incineration and waste power generation, and methane gas recovery from landfill and power generation in Ulaanbaatar, Mongolia, as a case study. We concluded that incineration process is the most suitable as first introduction of energy recovery. To operate it efficiently,3Rs strategies need to be promoted. And then, RDF production which is made of waste papers and plastics in high level of sorting may be considered as the second step of energy recovery.However, safety control and marketability of RDF will be required at that moment. 相似文献