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101.
102.
Photocatalytic degradation of gaseous toluene by using immobilized titania/silica on aluminum sheets
Minoo Tasbihi Marko Kete Ashok M. Raichur Nata?a Novak Tu?ar Ur?ka Lavren?i? ?tangar 《Environmental science and pollution research international》2012,19(9):3735-3742
Purpose
The aim of this study was to prepare a highly active immobilized titania/silica photocatalyst and to test its performance in situ toward degradation of toluene as one of the major toxic indoor contaminants.Methods
In this work, two different titania layers immobilized on Al sheets were synthesized via low temperature sol?Cgel method employing presynthesized highly active titania powders (Degussa P25 and Millennium PC500, mass ratio 1:1): (a) with a silica/titania binder and a protective layer and (b) without the binder. The photocatalysts were characterized by X-ray diffraction, nitrogen sorption measurements, scanning electron microscopy (SEM), infrared spectroscopy, and UV?Cvis diffuse reflectance spectroscopy (DRS). The in situ photocatalytic degradation of gaseous toluene was selected as a probe reaction to test photocatalytic activity and to verify the potential application of these materials for air remediation.Results
Results show that nontransparent highly photocatalytically active coatings based on the silica/titania binder and homogeneously dispersed TiO2 powders were obtained on the Al sheets. The crystalline structure of titania was not altered upon addition of the binder, which also prevented inhomogeneous agglomeration of particles on the photocatalyst surface. The photoactivity results indicate that the adsorption properties and photocatalytic activity of immobilized photocatalysts with the silica/titania binder and an underlying protective layer were very effective and additionally, they exhibited considerably improved adhesion and uniformity.Conclusion
We present a new highly photocatalytically active immobilized catalyst on a convenient metallic support, which has a potential application in an air cleaning device. 相似文献103.
Milana Rakić Maja Karaman Sofija Forkapić Jan Hansman Marko Kebert Kristina Bikit Dušan Mrdja 《Environmental science and pollution research international》2014,21(19):11283-11292
Edible and medicinal macrofungi used in human diet represent not only important sources of nutritive elements but toxic substances as well (heavy metals and radionuclides). Radioactivity levels of four radionuclides (40K, 137Cs, 226Ra, 228Ra) were determined in the basidiomata (fruiting bodies of a Basidiomycetes) of six lignicolous (Fomitopsis pinicola, Ganoderma applanatum, Hericium clathroides, Megacollybia platyphylla, Pluteus cervinus, Trametes gibbosa) and three mycorrhizal (Boletus luridus, Boletus sp. 1, Boletus sp. 2) species as well as their soil (wood) substrates by gamma spectrometry (high-resolution high-purity germanium (HPGe) detector). The aim was to investigate their ability for radionuclide absorption according to transfer factors (from soil and wood), to predict potential bioindicator species as well as species with potential risk for human use. Samples were taken during years 2011 and 2012, at two sites in forest ecosystem of Tara Mountain (Serbia). Observed concentration ranges per dry weight were as follows: 29–3,020 Bq/kg (40K), 21.9–735 Bq/kg (137Cs), 3–39 Bq/kg (226Ra), and 2.0–18 Bq/kg (228Ra). Obtained results indicate that the type of basidiome (fleshy/tough), most likely due to a different metabolic rate, has a very important role in radionuclide accumulation. The highest activity concentrations of all analyzed radionuclides were found in species with fleshy basidiomata—P. cervinus, H. clathroides, M. platyphylla, and Boletus species. A species-specific influence on radionuclide uptake was more prominent comparing to habitat differences and the role of fungal trophic mode. No significant variations were observed regarding radionuclide activity among the same fungal species from different sampling sites. 相似文献
104.
Marko S. Markov 《The Environmentalist》2012,32(2):119-120
105.
Out of three perceptual characteristics of the colour of any substance, the hue depends mostly on the spectral properties
of a substance, while the brightness and saturation depend also on the concentration of a substance and its thickness. Here,
we report that evident change of the hue of the colour (i.e., from green to red) is due to a change in concentration or the
thickness of a layer in some exceptional substances such as pumpkin seed oil or an aqueous solution of bromophenol blue. In
some regions of Central Europe, salad dressing is made preferably with the pumpkin seed oil, which has a strong characteristic
nut-like taste and remarkable properties of the colour: it appears red in a bottle, but green when served as a salad dressing.
The colour of the pumpkin seed oil was previously described as brownish yellow, dark green, dark green to red ochre or dark
reddish brown to light yellow green. We elucidated the physicochemical and physiological basis of such dichromatism by Beer-Lambert
law and by the characteristics of human colour perception. Our concept was corroborated by the outcome of calculations of
colour from spectral properties using colour matching functions. We found that dichromatism is observed if the absorption
spectrum of any substance has at least two local minima: one wide but shallow and one narrow but deep local minimum. 相似文献
106.
In countries having limited resources, it is difficult to assess urban air quality on contemporaneously, due to the absence of on-line information about air pollution levels and emission rates. An alternative approach is recommended for smaller cities with lower demands of resources. The applied scheme consists of a database of air pollution sources (NO
x
and CO from industry, traffic, and domestic heating), the simple Gaussian-plume model AEROPOL and a series of measurements by passive monitors. This method was used in Tartu, a small city situated in the valley of the river Emajõgi, within a landscape with noteworthy topographical variations. Simulations of annual average and maximal concentrations were performed, and a fair agreement obtained with NO2 monitoring results from passive Palmes monitors. Inventories of pollution sources in 1998 revealed that official statistics of stationary sources covered 64% of SO2,36% of CO, 37% of NO
x
and 32% of total particulate matter emissions. Recommendations for measures for reducing air pollution levels and for further investigations towards improving air quality assessment and management, are given. 相似文献
107.
Keskinen M 《Ambio》2008,37(3):193-198
The Mekong River Basin is facing rapid changes, including intensive plans for water development. While the different development projects are considered to be important for economic development, the negative impacts that they are likely to cause for ecosystems and livelihoods are estimated to be remarkable. Yet, existing impact assessment processes seem in many cases to be inadequate to capture even the actual magnitude of the impacts at different levels. This article looks at the different impact assessment processes and their challenges in the basin. It is argued that impact assessment in this kind of dynamic and complex setting requires better coordination between assessments at different levels. Basinwide impact assessment would benefit from a more adaptive, multilevel approach that makes better use of assessments from local levels up to the regional level and builds on more participatory and interdisciplinary methods. Successful impact assessment also requires the recognition of the highly political nature of water development and related planning processes. 相似文献
108.
In this paper we study optimal harvesting of the Norwegian spring-spawning herring stock. The biological model is described
by a discrete time age-structured model. The optimal harvesting patterns are studied numerically and the results show that
when using a linear cost function and constant price in the optimisation model, the optimal harvesting pattern is pulse fishing.
However, optimal constant fishing effort gives only slightly lower profit. Moreover, when price is made responsive to harvest
the optimal harvesting strategy is substantially smoothed.
This revised version was published online in July 2006 with corrections to the Cover Date. 相似文献
109.
Results of 2 years monitoring of 210Po and 210Pb activity concentrations in soft tissue of the species Mytilus galloprovincialis from Croatian part of the Adriatic coast are presented. The samples were collected at thirteen coastal stations (some of which are also a part of the Mediterranean Mussel Watch Project) in spring and autumn of 2010 and 2011. The collected mussels were ranging between 4 cm and 6 cm in shell length. After sample pre-treatment lead and polonium were radiochemically separated on Sr resin. 210Po was determined by alpha-particle spectrometry and 210Pb was determined, via 210Bi, by a low-level gas proportional counter. The results of 210Po activity concentrations were found to vary between (104 ± 11) and (1421 ± 81) Bq kg−1 dry weight while 210Pb activity concentrations were much lower and in range (8.2 ± 5.3)–(94.1 ± 29.8) Bq kg−1 dry weight. Higher 210Po and 210Pb activity concentrations were determined in spring period. The inter-site differences seen in their activity concentrations can be due to natural background levels of sites. The 210Po/210Pb activity concentration ratios in all cases exceeded unity for all mussel samples and ranged between 4.0 and 47.9. 相似文献
110.
Electromagnetic therapy devices designed over the last 45 years have been based on empirical (trial-and-error) techniques. This paper presents a novel approach to designing and engineering therapeutic devices. Based upon using a superconductive quantum interference device (SQUID) magnetometer for registration of the magnetic field emitted by specific organs in norm and after the injury/pathology, this approach avoids empirical engineering. The signal parameters recorded by the SQUID magnetometer allow one to derive tissue- and/or disease-specific signals. This is made possible using contemporary, state-of-the-art controls with engineering and computer science techniques. 相似文献