首页 | 本学科首页   官方微博 | 高级检索  
文章检索
  按 检索   检索词:      
出版年份:   被引次数:   他引次数: 提示:输入*表示无穷大
  收费全文   3806篇
  免费   99篇
  国内免费   1437篇
安全科学   211篇
废物处理   214篇
环保管理   304篇
综合类   1860篇
基础理论   691篇
环境理论   1篇
污染及防治   1629篇
评价与监测   147篇
社会与环境   124篇
灾害及防治   161篇
  2024年   2篇
  2023年   63篇
  2022年   183篇
  2021年   126篇
  2020年   95篇
  2019年   88篇
  2018年   146篇
  2017年   161篇
  2016年   205篇
  2015年   249篇
  2014年   303篇
  2013年   365篇
  2012年   327篇
  2011年   305篇
  2010年   233篇
  2009年   271篇
  2008年   265篇
  2007年   221篇
  2006年   209篇
  2005年   150篇
  2004年   114篇
  2003年   143篇
  2002年   128篇
  2001年   109篇
  2000年   120篇
  1999年   130篇
  1998年   142篇
  1997年   84篇
  1996年   77篇
  1995年   74篇
  1994年   59篇
  1993年   55篇
  1992年   48篇
  1991年   15篇
  1990年   19篇
  1989年   11篇
  1988年   12篇
  1987年   5篇
  1986年   6篇
  1985年   2篇
  1984年   2篇
  1983年   2篇
  1982年   2篇
  1981年   7篇
  1979年   2篇
  1977年   2篇
  1975年   1篇
  1974年   1篇
  1972年   1篇
  1971年   2篇
排序方式: 共有5342条查询结果,搜索用时 15 毫秒
71.
Zha  Zhenqiu  Li  Guoao  Lv  Yili  Liu  Lingli  He  Jialiu  Xu  Wei  Dai  Dan  Liu  Zhirong  Huang  Fen 《Environmental science and pollution research international》2022,29(30):45716-45729
Environmental Science and Pollution Research - Recently, the burden of lung cancer (LC) has attracted global attention. Meanwhile, LC has become the leading cause of death in China. Many studies...  相似文献   
72.

The interaction of nanoplastics (NPls) and engineered nanoparticles (ENPs) with organic matter and environmental pollutants is particularly important. Therefore, their behavior should be investigated under the different salinity conditions, mimicking rivers and coastal environments, to understand this phenomenon in those areas. In this work, we analyzed the elementary characteristics of polystyrene-PS (unmodified surface and modified with amino or carboxyl groups) and titanium dioxide-TiO2 nanoparticles. The effect of salinity on their colloidal properties was studied too. Also, the interaction with different types of proteins (bovine serum albumin-BSA and tilapia proteins), as well as the formation of the BSA corona and its effect on the colloidal stability of nanoparticles, were evaluated. The morphology and dispersion of sizes were more uniform in unmodified-surface PS-NPs (70.5?±?13.7 nm) than in TiO2-NPs (131.2?±?125.6 nm). Likewise, Rama spectroscopy allowed recognizing peaks associated with the PS phenyl group aromatic ring in unmodified-surface PS-NPs (621, 1002, 1582, and 1602 cm?1). For TiO2-NPs, the data suggest belonging to the tetragonal form, also known as rutile (445, 610 cm?1). The elevation of salinity dose-dependently decreased NP colloid stability, with more significant variation in the PS-NPs compared to TiO2-NPs. The organic matter is also involved in this phenomenon, differentially as a function of time compared to its absence (unmodified-surface PS-NPs 30 psu/TOC 5 mgL?1/24 h: 2876.6?±?378.03 nm; unmodified-surface PS-NPs 30 psu/24 h: 2133?±?49.57 nm). In general, the TiO2-NPs demonstrated greater affinity with all proteins tested (0.066 g/L). It was observed that morphology, size, and surface chemical modification intervene in a relevant way in the interaction of the nanoparticles with bovine serum albumin (unmodified-surface PS-NPs 298 K: 6.08E+02; 310 K: 6.63E+02; TiO2-NPs 298 K: 8.76E+02; 310 K: 1.05E+03 L mol?1) and tilapia tissues proteins (from blood, gills, liver, and brain). Their morphology and size also determined the protein corona formation and the NPs’ agglomeration. These findings can provide references during knowledge transfer between NPls and ENPs.

  相似文献   
73.
Environmental Science and Pollution Research - Energy-related carbon emissions take a large proportion in China, and the interregional trade caused by provincial disparities has led to significant...  相似文献   
74.
Environmental Science and Pollution Research - To assess the status of hotspots and research trends on geographic information system (GIS)–based landslide susceptibility (LS), we analysed...  相似文献   
75.
Huang Q  Hong CS 《Chemosphere》2000,41(6):871-879
Titanium dioxide-mediated photodegradation of Polychlorinated biphenyls (PCBs) in soil/aqueous systems with added fluorinated surfactant was investigated. PCBs can bind tightly to organic matter in the soil, especially in aged, contaminated soil. Experiments showed an effective PCB photocatalytic degradation in mixed systems of soil/clay with anionic fluorinated surfactant FC-143 and TiO2. The FC-143 surfactant is stable in this photochemical process. PCB degradation rates in samples followed the order: spiked clay > spiked soil > Hudson River bank soil. The results suggest that anionic fluorinated surfactant may form semimicelles and/or admicelles on the surface of positively charged TiO2. The hydrophobic surface of TiO2 can provide a nonpolar phase that acts as a partioning medium for hydrophobic PCBs. Therefore, PCBs in soil can be released to the semimicelle and/or admicelle on the TiO2 surface and are effectively photodegraded in a dispersion containing anionic fluorinated surfactant. The combination of surfactant extraction and photooxidation forms the basis for a novel two-stage process for the removal and destruction of PCBs from soil.  相似文献   
76.
Wang CC  Lee CM  Lu CJ  Chuang MS  Huang CZ 《Chemosphere》2000,41(12):1873-1879
In this study, pure strains that are capable of utilizing 2,4,6-trichlorophenol have been isolated from the mixed culture grown on substrates containing chlorophenolic compounds. Studies have been carried out on the capability of these isolated pure strains in suspended and immobilized forms to decompose 2,4,6-trichlorophenol. Additionally, the influence of primary substrates (e.g., phenol, 2-chlorophenol, 3-chlorophenol, 4-chlorophenol, 2,4-dichlorophenol) on the decomposition of 2,4,6-trichlorophenol by the isolated pure strains grown in immobilized form is also investigated. The results are: Through bacterial isolation and identification, three pure strains have been obtained: Pseudomonas spp. strain 01, Pseudomonas spp. strain 02 and Agrobacterium spp. Whether in suspended or immobilized forms, all strains have poor removal efficiencies of 2,4,6-trichlorophenol. However, addition of 200 mg/l phenol will enable the immobilized Pseudomonas spp. strain 01, and Pseudomonas spp. strain 02 to achieve 65% and 48% removal of 2,4,6-trichlorophenol, respectively. Addition of phenol will assist the immobilized Pseudomonas spp. strain 02 in achieving removal of 2,4,6-trichlorophenol but the removal efficiency is not good if the phenol concentration is too low. The optimum phenol concentration should be between 200 and 400 mg/l.  相似文献   
77.
This study explores ambient air quality forecasts using the conventional time-series approach and a neural network. Sulfur dioxide and ozone monitoring data collected from two background stations and an industrial station are used. Various learning methods and varied numbers of hidden layer processing units of the neural network model are tested. Results obtained from the time-series and neural network models are discussed and compared on the basis of their performance for 1-step-ahead and 24-step-ahead forecasts. Although both models perform well for 1-step-ahead prediction, some neural network results reveal a slightly better forecast without manually adjusting model parameters, according to the results. For a 24-step-ahead forecast, most neural network results are as good as or superior to those of the time-series model. With the advantages of self-learning, self-adaptation, and parallel processing, the neural network approach is a promising technique for developing an automated short-term ambient air quality forecast system.  相似文献   
78.
Environmental Science and Pollution Research - Increasing research suggested that green spaces are associated with many health benefits, but evidence for the quantitative relationship between green...  相似文献   
79.
Li  Yongjun  Qiao  Jing  Xie  Lei  Huang  Lingyan  Su  Yue  Zhou  Mengmeng  Wang  Ke  Zhang  Jing  He  Shan  Huang  Lu 《Environmental science and pollution research international》2022,29(31):46751-46766

To achieve urban sustainability, it is critical to enhance the environment, economy, and society simultaneously. This study adopted the revised genuine progress indicator (GPI) and ecological footprint (EF) to evaluate the ecological efficiency and economic sustainability of the Yangtze River Delta from 2000 to 2018. Spatial analysis was utilized to identify spatial autocorrelation. A total of 27 cities were then partitioned through k-means cluster analysis. The results showed that GPI and ecological efficiency improved rapidly, but economic sustainability showed a downward trend. GPI and GDP had a high degree of spatial correlation, especially in Suzhou-Wuxi-Changzhou Metropolitan Area. However, no spatial correlation existed between GPI and EF. The city with high GEE can reach 3000 $/gha, indicating the city consumed 1 global hectare to create $3000 of genuine economic growth. Shanghai, Hangzhou, and Taizhou were cities with the highest level of economic sustainability and ecological efficiency. The spatiotemporal characteristics of economic sustainability and ecological efficiency revealed in this study will provide theoretical guidance for alleviating ecological pressure and promoting economic sustainable development.

  相似文献   
80.
在活性污泥系统优化设计模型参数不确定性分析的基础上,考察了进水负荷、生物动力学参数、曝气设备性能参数和二沉池浓缩常数变化对优化设计的影响。灵敏度分析结果表明,对优化设计影响较大的参数为:进水水量水质、与氧转移效率相关的校正参数以及二沉池的浓缩常数等。研究结果对于低灵敏度系统的设计,提高优化设计结果的工程实用性具有重要的意义。  相似文献   
设为首页 | 免责声明 | 关于勤云 | 加入收藏

Copyright©北京勤云科技发展有限公司  京ICP备09084417号