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671.
L.-J. Sally Liu Harish C. Phuleria Whitney Webber Mark Davey Douglas R. Lawson Robert G. Ireson Barbara Zielinska John M. Ondov Christopher S. Weaver Charles A. Lapin Michael Easter Thomas W. Hesterberg Timothy Larson 《Atmospheric environment (Oxford, England : 1994)》2010,44(28):3422-3431
We monitored two Seattle school buses to quantify the buses’ self pollution using the dual tracers (DT), lead vehicle (LV), and chemical mass balance (CMB) methods. Each bus drove along a residential route simulating stops, with windows closed or open. Particulate matter (PM) and its constituents were monitored in the bus and from a LV. We collected source samples from the tailpipe and crankcase emissions using an on-board dilution tunnel. Concentrations of PM1, ultrafine particle counts, elemental and organic carbon (EC/OC) were higher on the bus than the LV. The DT method estimated that the tailpipe and the crankcase emissions contributed 1.1 and 6.8 μg m?3 of PM2.5 inside the bus, respectively, with significantly higher crankcase self pollution (SP) when windows were closed. Approximately two-thirds of in-cabin PM2.5 originated from background sources. Using the LV approach, SP estimates from the EC and the active personal DataRAM (pDR) measurements correlated well with the DT estimates for tailpipe and crankcase emissions, respectively, although both measurements need further calibration for accurate quantification. CMB results overestimated SP from the DT method but confirmed crankcase emissions as the major SP source. We confirmed buses’ SP using three independent methods and quantified crankcase emissions as the dominant contributor. 相似文献
672.
Research on precipitation carried out systematically at the University station at Jeziory in the Wielkopolski National Park
(western Poland) allowed the determination of pollutants deposited with precipitation in this forest ecosystem. During 13 years
of study, the pH of precipitation was found to persist at a low level (4.33 on average), which resulted a substantial deposition
of H+. Values of acidifying and basic ions deposited in this area were determined and compared with the respective figures obtained
at selected EMEP stations studying background pollution, the means for Poland, and areas subjected to considerable human impact.
The use of the critical load function made it possible to establish that the S and N deposition for 2002–2005 were below its
line. 相似文献
673.
Weili Liu Jaymin Kwon Clifford Weisel Barbara Turpin Lin Zhang 《Journal of the Air & Waste Management Association (1995)》2013,63(8):1196-1204
Abstract This paper presents the analysis of ambient air concentrations of 10 carbonyl compounds (aldehydes and ketones) measured in the yards of 87 residences in the city of Elizabeth, NJ, throughout 1999–2001. Most of these residences were measured twice in different seasons; the sampling duration was 48 hr each time. The authors observed higher concentrations for most of the measured carbonyl compounds on warmer days, reflecting larger contributions of photochemical reactions on warmer days. The estimated contributions of photochemical production varied substantially across the measured carbonyl compounds and could be as high as 60%. Photochemical activity, however, resulted in a net loss for formaldehyde. The authors used stepwise multiple linear regression models to evaluate the impact of traffic sources and meteorological conditions on carbonyl concentrations using the data collected on colder days (with lower photochemical activities). They found that the concentrations of formal-dehyde, acetaldehyde, acrolein, propionaldehyde, crotonaldehyde, benzaldehyde, glyoxal, and methylglyoxal significantly decreased with increasing distance between a measured residence and one or more major roadways. They also found significant negative associations between concentrations for most of the measured carbonyl compounds and each of the following meteorological parameters: mixing height, wind speed, and precipitation. 相似文献
674.
Discussions about the potential role of academic and research institutions in regional sustainability initiatives (RSIs) inevitably raise the issue of the role of science in society in general. In democratic societies, it can be argued that science–society relationships should be based on establishing and institutionalizing mutual dialogues, making public concerns not only visible but the public as equal partner. In order to fulfil the social responsibilities of academic institutions involved in RSIs through establishing dialogues with diverse stakeholders, a possible methodology is conducting participatory action research (PAR) combined with the educational model of service learning. The PAR project reported here aims at facilitating a bottom-up, micro-region level sustainability planning and development process in one of the most socio-economically disadvantaged rural areas of north-east Hungary. Some of the main results of this university–community partnership were its contribution to sustainability, including the activation of local capabilities and networking across various local stakeholder groups through various small-scale projects and the co-production of a socially grounded and landscape-based rural development plan for the micro-region. 相似文献
675.
Francesca Romana Grati Denise Molina Gomes Jose Carlos Pinto B. Ferreira Celine Dupont Viola Alesi Laetitia Gouas Nina Horelli-Kuitunen Kwong Wai Choy Sandra García-Herrero Alberto Gonzalez de la Vega Krzysztof Piotrowski Rita Genesio Gloria Queipo Barbara Malvestiti Bérénice Hervé Brigitte Benzacken Antonio Novelli Philippe Vago Kirsi Piippo Tak Yeung Leung Federico Maggi Thibault Quibel Anne Claude Tabet Giuseppe Simoni François Vialard 《黑龙江环境通报》2015,35(8):801-809
676.
Quantifying MTBE biodegradation in the Vandenberg Air Force Base ethanol release study using stable carbon isotopes 总被引:1,自引:1,他引:0
McKelvie JR Mackay DM de Sieyes NR Lacrampe-Couloume G Sherwood Lollar B 《Journal of contaminant hydrology》2007,94(3-4):157-165
Compound-specific isotope analysis (CSIA) was used to assess biodegradation of MTBE and TBA during an ethanol release study at Vandenberg Air Force Base. Two continuous side-by-side field releases were conducted within a preexisting MTBE plume to form two lanes. The first involved the continuous injection of site groundwater amended with benzene, toluene and o-xylene ("No ethanol lane"), while the other involved the continuous injection of site groundwater amended with benzene, toluene and o-xylene and ethanol ("With ethanol lane"). The delta(13)C of MTBE for all wells in the "No ethanol lane" remained constant during the experiment with a mean value of -31.3 +/- 0.5 per thousand (n=40), suggesting the absence of any substantial MTBE biodegradation in this lane. In contrast, substantial enrichment in (13)C of MTBE by 40.6 per thousand, was measured in the "With ethanol lane", consistent with the effects of biodegradation. A substantial amount of TBA (up to 1200 microg/L) was produced by the biodegradation of MTBE in the "With ethanol lane". The mean value of delta(13)C for TBA in groundwater samples in the "With ethanol lane" was -26.0 +/- 1.0 per thousand (n=32). Uniform delta(13)C TBA values through space and time in this lane suggest that substantial anaerobic biodegradation of TBA did not occur during the experiment. Using the reported range in isotopic enrichment factors for MTBE of -9.2 per thousand to -15.6 per thousand, and values of delta(13)C of MTBE in groundwater samples, MTBE first-order biodegradation rates in the "With ethanol lane" were 12.0 to 20.3 year(-1) (n=18). The isotope-derived rate constants are in good agreement with the previously published rate constant of 16.8 year(-1) calculated using contaminant mass-discharge for the "With ethanol lane". 相似文献
677.
678.
679.
Judy Z. Drexier Barbara L. Bedford Arthur T DeGaetano Donald I. Siegel 《Journal of the American Water Resources Association》1999,35(4):753-769
ABSTRACT: Few water budgets exist for specific types of wetlands such as peatlands, even though such information provides the basis from which to investigate linkages between wetlands and upland ecosystems. In this study, we first determined the water budget and then estimated nutrient loading from an upland farm field into a 1.5 ha, kettle-block peatland. The wetland contains highly anisotropic peat and has no distinct, active layer of groundwater flow. We estimated the depth of the active layer using Fick's law of diffusion and quantified groundwater flow using a chemical mass balance model. Evapotranspiration was determined using MORECS, a semi-physical model based on the Penman-Monteith approach. Precipitation and surface outflow were measured using physical means. Groundwater provided the major inflow, 84 percent (44,418 m3) in 1993 and 88 percent (68,311 m3) in 1994. Surface outflow represented 54 percent (28,763 m3) of total outflows in 1993 and 48 percent (37,078 m3) in 1994. A comparison of several published water budgets for wetlands and lakes showed that error estimates for hydrologic components in this study are well within the range of error estimates calculated in other studies. Groundwater inflow estimates and nutrient concentrations of three springs were used to estimate agricultural nutrient loading to the site. During the study period, nutrient loading into the peatland via groundwater discharge averaged 24.74 kg K ha-1, 1.83 kg total inorganic P had, and 21.81 kg NO3-N ha-1. 相似文献
680.
Chromated copper arsenate (CCA) treated wood has been used for more than 50 years. Recent attention has been focused on appropriate disposal of CCA-treated wood when its service life ends. Groups in the US and Europe concerned with the possibility of arsenic migration to groundwater from disposed CCA-treated wood have proposed that consumers be required to dispose of the wood as a hazardous waste, in the most protective of landfills. We examined available data for evidence of arsenic migration from unlined construction and demolition (C&D) debris landfills in Florida, where CCA-treated wood is disposed. Florida was chosen because soil, groundwater, landfill design, weather, and levels of CCA-treated wood use make the state a uniquely sensitive indicator for observing arsenic migration from CCA-treated wood disposal sites, should it occur. We developed and quality-checked a CCA-treated wood disposal model to estimate the amount of wood and associated arsenic disposed. By 2000, an estimated 13 million kg of arsenic in CCA-treated wood was disposed in Florida; however, groundwater monitoring data do not indicate that arsenic is migrating from unlined C&D landfills. Our results provide evidence that highly stringent regulation of CCA-treated wood disposal, such as treatment as a hazardous waste, is unnecessary. 相似文献