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81.
Herbicides of the chlorinated phenoxyalkanoic acid group like 2,4-D, 2,4-DP and MCPP, belong to the most commonly used pesticides. This is also true for the Land Brandenburg. Therefore, this substance group was integrated in the current state monitoring programme for ground and surface water quality. Starting in 2001, the analysis was carried out complying with DIN 38407-20 by gas chromatography and mass spectrometric detection after enrichment with solid phase extraction and following derivatization with diazomethane-forming methyl esters. Quantifying 2,4-D considering selected ions in a surface water sample from the river Oder, a remarkable peak pattern was observed. A second peak with identical spectrum was found about 0.7 minutes earlier than the 2,4-D calibrated peak. Its intensity suggested a concentration 10–20 fold higher than the 2,4-D level. This unknown peak was identified as 2,6-D which is a structure isomer of the herbicide 2,4-D. This substance has not been described in literature or chemical substance databases known to us yet. Structure isomers have been found in other samples too. We suppose that the chlorinated phenoxyalkanoic acids chlorinated in the 6-position of the phenyl ring are formed as a technical by-product and show a higher persistance than the commonly known agents. 相似文献
82.
Evaluation of factors influencing soluble microbial product in submerged MBR through hybrid ASM model 总被引:1,自引:0,他引:1
Fangyue Li Joachim Behrendt Knut Wichmann Ralf Otterpohl 《Frontiers of Environmental Science & Engineering in China》2009,3(2):226-235
In this study, a mathematical model was established to predict the formation of the soluble microbial product (SMP) in a submerged
membrane bioreactor. The developed model was calibrated under the reference condition. Simulation results were in good agreement
with the measured results under the reference condition. The calibrated model was then used in the scenario studies to evaluate
the effect of three chosen operating parameters: hydraulic retention time (HRT), dissolved oxygen concentration, and sludge
retention time (SRT). Simulation results revealed that the SMP dominated the soluble organic substances in the supernatant.
The scenario studies also revealed that the HRT can be decreased to 1 h without deteriorating the effluent quality; dissolved
oxygen concentration in the reactor can be kept at 2–3 mg/L to maintain the effluent quality, reduce the content of SMP, and
minimize operating costs; the optimal SRT can be controlled to 10–15 d to achieve complete nitrification process, less membrane
fouling potential, and acceptable organic removal efficiency. 相似文献
83.
Daria Schurmann Jana Collatz Steffen Hagenbucher Joachim Ruther Johannes L. M. Steidle 《Die Naturwissenschaften》2009,96(3):383-391
Associative learning of host-associated chemical cues was studied in Nasonia vitripennis, a parasitoid of fly pupae in nests of hole-nesting birds. When females encountered a fly pupa and performed one sequence
of host recognition behaviour including drilling the ovipositor into the host in the presence of the artificial odour furfurylheptanoate
(FFH), they were afterwards arrested by FFH in olfactometer experiments. The response vanished after 4 days and could be blocked
after 3 days by feeding wasps with ethacrynic acid prior and after the training. This indicates the formation of an intermediate
form of memory by one host experience in N. vitripennis. Interestingly, the trained wasps avoided odours that were not present during the host encounter, although naive wasps did
not react to these odours. This unique behaviour probably causes wasps to focus during host searching on those chemical cues
they have experienced in the host environment. Studies in nests of hole-nesting birds revealed that about 30% of all nests
contained only one fly pupa, and laboratory studies showed that N. vitripennis females are able to parasitise around 100 fly pupae in their life. It is discussed that under these conditions, the formation
of a non-permanent intermediate memory for host-associated odours after one host encounter is adaptive to avoid costs involved
with formation and maintenance of memory for misleading cues. The demonstration of associative olfactory learning in N. vitripennis, the first parasitoid species with sequenced genome, opens the gate to study molecular mechanisms of memory formation and
its ecological adaptation in parasitoids. 相似文献
84.
Giovannangelo ME Gehring U Nordling E Oldenwening M van Rijswijk K de Wind S Hoek G Heinrich J Bellander T Brunekreef B 《Environment international》2007,33(1):9-16
BACKGROUND: Mold growth is believed to be one causative factor underlying the association between dampness in buildings and increased respiratory morbidity. Measurements of beta(1-->3)-glucans and fungal extracellular polysaccharides (EPS) are used as markers of mold exposure in field studies. Little is known about their levels and determinants in homes. OBJECTIVE: To study levels and determinants of beta(1-->3)-glucan and EPS levels in mattress and living room floor dust in three European countries. METHODS: Mattress and living room floor dust was collected in the homes of 1065 German, Dutch, and Swedish (pre-)school children. All samples were analyzed for beta(1-->3)-glucans and EPS in one central laboratory. Determinants were assessed by questionnaire. RESULTS: Amounts of dust, EPS and beta(1-->3)-glucan levels differed between countries. Amounts of dust, beta(1-->3)-glucan and EPS levels for mattresses were only weakly correlated with those for living room floors. Floor dust beta(1-->3)-glucan loads, EPS loads and EPS concentrations were strongly correlated with the amount of dust sampled, which is largely determined by the type of floor that was sampled (carpeted floors had 5-20 higher amounts of dust). None of the other determinants was consistently and statistically significantly associated with amounts of dust, beta(1-->3)-glucan and EPS concentrations on floors and mattresses. CONCLUSION: Mattress dust and floor dust are two different measures of exposure to the investigated mold components. Living room floor beta(1-->3)-glucan and EPS loads and EPS concentrations are largely determined by the type of floor sampled. Differences between countries can only partly be explained by the determinants studied. 相似文献
85.
Bishawjit Mallick Khan Rubayet Rahaman Joachim Vogt 《Mitigation and Adaptation Strategies for Global Change》2011,16(6):629-648
This paper aimed at to explore the consequences of cyclone victims due to unavailability of infrastructural supports and to
prop up the recognition that the infrastructure has a vital role to play in societies’ resilience during catastrophic situation.
The paper begins with a review of the science regarding climate change impact and cyclone disaster in Bangladesh. It emphasizes
the consequences of cyclone Aila in a selected coastal community in the remote coastal area. A field survey was conducted
by authors during March-August 2009. Eight available infrastructures were selected for this analysis. Uniformity of distribution
(R), demand index (Di) and degree of demand (DD) of the selected infrastructures were calculated by using nearest neighbourhood
methods of analysis. Results show that based on its specific planning standards none of the selected infrastructure can support
50% of the total population. Accordingly, it was observed that 76% respondent could not reach in safer place due to rush of
water intrusion and also because of the inundation of road-network. The nearness to the available cyclone shelter, and place
of taking shelter during cyclone is positively correlated (r = 0.38; p < 0.001). However, the poor people had less opportunity to take shelter in cyclone shelters, although none of the respondents
groups whose monthly income is above 75 USD stands without any infrastructural support. Such important observation may hint
the influence of local elites on the local disaster mitigation planning practice in Bangladesh. Almost 90% of the respondents
claimed that they had no access to enter the available cyclone shelter. Furthermore, the damaged infrastructures added more
hindrances during post disaster activities and also increased the sufferings of the victims. If there were adequate cyclone
shelters or rehabilitation centre, the affected people could take shelter and continue other works temporarily. Results drawn
from this research will be useful for local and national level planners, as well as international donors for future disaster
mitigation planning in the studied area and the methodology can be applied in similar countries and geographical territories. 相似文献
86.
Marco Munari Joachim Sturve Matthew B. Sanders Paul Christian Marco Nigro 《Chemistry and Ecology》2014,30(8):719-725
The use of functionalised metal sulphide nanoparticles (NPs) for nanoremediation and biomedical application is rapidly increasing, which could lead to significant inputs into the marine environment. The potential impact of some NPs on marine organisms is still poorly understood. In the present paper the genotoxic potential of Ag2S and CdS NPs on Mytilus edulis haemocytes was assessed. MPEG-SH (thiol-terminated methyl polyethylene glycol), was used as capping agent to avoid NPs agglomeration. TEM analysis showed that the Ag2S NPs size was 13±7 nm, whereas CdS quantum dots had an average diameter of 4±1 nm. DNA integrity was evaluated by Comet assay following exposure to increasing concentration series (0.01–10 mg/L). Both silver and cadmium NPs showed genotoxic effects at the highest dose. MPEG-SH was also found to exert a weak genotoxic activity, suggesting that at least part of the genotoxic potential of functionalised NPs on mussel cells might be attributable to the capping agent. These results confirm the genotoxic potential of Ag2S NPs for mussel cells and demonstrated, for the first time, that CdS NPs is genotoxic in a marine organism. 相似文献
87.
Antibiotics of inorganic and organic origin in pig manure can inhibit the anaerobic process in biogas plants. The influence of three frequently used antibiotics, copper dosed as CuSO4, sulfadiazine (SDZ), and difloxacin (DIF), on the anaerobic digestion process of pig manure was studied in semi-continuous experiments. Biogas production recovered after every Cu dosage up to a sum of 12.94 g Cu kg−1 organic dry matter (ODM), probably due to Cu precipitation following the formation of sulphide from sulphate. Complete inhibition was found at the very high Cu concentration of 19.40 g Cu kg−1 ODM. Inhibitory effect of SDZ and DIF was observed at concentrations as high as 2.70 g kg−1 ODM and 0.54 g kg−1 ODM, respectively. It seems very unlikely that the antibiotics tested would inhibit the anaerobic process in a full-scale biogas plant. 相似文献
88.
Joachim Maes Jo Vliegen Karen Van de Vel Stijn Janssen Felix Deutsch Koen De Ridder Clemens Mensink 《Atmospheric environment (Oxford, England : 1994)》2009,43(6):1246-1254
CORINAIR atmospheric emission inventories are frequently used input data for air quality models with a domain situated in Europe. In CORINAIR emission inventories, sources are broken down over 11 major source categories. This paper presents spatial surrogates for the disaggregation of CORINAIR atmospheric emission inventories for input of air pollutants and particulate matter to grid or polygon based air quality model domains inside Europe. The basis for the disaggregation model was the CLC2000 land cover data to which statistical weights were added. Weights were population census data for residential emissions, employment statistics for agricultural and industrial area emissions, livestock statistics for ammonia emissions and annual aircraft movements for emissions realized by air transport. Additional road and off-road network information was used to disaggregate emissions realized by traffic. A comparison of top down produced emission estimates with spatially resolved national emission data for The Netherlands and the United Kingdom gave confidence in the present spatial surrogates as a tool for the top down production of atmospheric emission maps. Explained variance at a spatial resolution of 5 km was >70% for CO, NMVOC and NOx, >60% for PM10 and almost 50% for SO2. 相似文献
89.
Wu Jiayu Chen Tianyue Ge Shengbo Fan Wei Wang Hui Zhang Zhongfeng Lichtfouse Eric Van Tran Thuan Liew Rock Keey Rezakazemi Mashallah Huang Runzhou 《Environmental Chemistry Letters》2023,21(6):3393-3424
Environmental Chemistry Letters - In the context of the circular economy and decreasing earth resources, waste should be converted into value-added materials such as carbon quantum dots, which are... 相似文献
90.
The use of heavy metal hyperaccumulating plants has the potential to become a promising new technique to remediate contaminated sites. We investigated the role of metal mobilization in the Cd hyperaccumulation of Thlaspi caerulescens (J. & C. Presl, 'Ganges'). In a micro-lysimeter experiment we investigated the dynamics of Cd concentration of leachate as well as Cd removal by plant uptake in four treatments: (i) Control (bare soil), (ii) T. caerulescens, (iii) nonhyperaccumulator Brassica juncea (L.) Czern. ('PI 426308'), and (iv) co-cropping of the hyperaccumulator and nonhyperaccumulator. The experimental findings were analyzed using one- and two-site rate-limited desorption models. Co-cropping of T. caerulescens and B. juncea did not enhance metal uptake by B. juncea. Although Cd uptake of T. caerulescens was 10 times higher than that of B. juncea, the Cd concentration of leachate of the T. caerulescens treatment did not decrease below that of the B. juncea treatment. The Cd depletion in leachate was well reproduced by the two-site rate-limited desorption model. The optimized desorption coefficient was three orders of magnitude higher in the rhizosphere than in the bulk soil. Our results indicate that T. caerulescens accelerates the resupply of Cd from soil pointing to an important role of kinetic desorption in the hyperaccumulation by T. caerulescens. 相似文献