全文获取类型
收费全文 | 939篇 |
免费 | 41篇 |
国内免费 | 107篇 |
专业分类
安全科学 | 43篇 |
废物处理 | 11篇 |
环保管理 | 110篇 |
综合类 | 444篇 |
基础理论 | 88篇 |
污染及防治 | 199篇 |
评价与监测 | 174篇 |
社会与环境 | 17篇 |
灾害及防治 | 1篇 |
出版年
2023年 | 13篇 |
2022年 | 24篇 |
2021年 | 14篇 |
2020年 | 35篇 |
2019年 | 17篇 |
2018年 | 20篇 |
2017年 | 16篇 |
2016年 | 33篇 |
2015年 | 51篇 |
2014年 | 51篇 |
2013年 | 46篇 |
2012年 | 49篇 |
2011年 | 74篇 |
2010年 | 53篇 |
2009年 | 70篇 |
2008年 | 87篇 |
2007年 | 72篇 |
2006年 | 53篇 |
2005年 | 27篇 |
2004年 | 23篇 |
2003年 | 26篇 |
2002年 | 32篇 |
2001年 | 24篇 |
2000年 | 42篇 |
1999年 | 31篇 |
1998年 | 19篇 |
1997年 | 20篇 |
1996年 | 14篇 |
1995年 | 11篇 |
1994年 | 4篇 |
1993年 | 10篇 |
1992年 | 5篇 |
1991年 | 3篇 |
1990年 | 3篇 |
1989年 | 2篇 |
1988年 | 2篇 |
1987年 | 1篇 |
1986年 | 1篇 |
1985年 | 1篇 |
1984年 | 3篇 |
1981年 | 1篇 |
1980年 | 1篇 |
1979年 | 2篇 |
1977年 | 1篇 |
排序方式: 共有1087条查询结果,搜索用时 31 毫秒
81.
Kros J Frumau KF Hensen A de Vries W 《Environmental pollution (Barking, Essex : 1987)》2011,159(11):3171-3182
The integrated modelling system INITIATOR was applied to a landscape in the northern part of the Netherlands to assess current nitrogen fluxes to air and water and the impact of various agricultural measures on these fluxes, using spatially explicit input data on animal numbers, land use, agricultural management, meteorology and soil. Average model results on NH3 deposition and N concentrations in surface water appear to be comparable to observations, but the deviation can be large at local scale, despite the use of high resolution data. Evaluated measures include: air scrubbers reducing NH3 emissions from poultry and pig housing systems, low protein feeding, reduced fertilizer amounts and low-emission stables for cattle. Low protein feeding and restrictive fertilizer application had the largest effect on both N inputs and N losses, resulting in N deposition reductions on Natura 2000 sites of 10% and 12%, respectively. 相似文献
82.
S.M. Eldridge C.R. Chen Z.H. Xu P.N. Nelson S.E. Boyd I. Meszaros K.Y. Chan 《Waste management (New York, N.Y.)》2013,33(11):2157-2169
Using solid state 13C NMR data and elemental composition in a molecular mixing model, we estimated the molecular components of the organic matter in 16 recycled organic (RO) wastes representative of the major materials generated in the Sydney basin area. Close correspondence was found between the measured NMR signal intensities and those predicted by the model for all RO wastes except for poultry manure char. Molecular nature of the organic matter differed widely between the RO wastes. As a proportion of organic C, carbohydrate C ranged from 0.07 to 0.63, protein C from <0.01 to 0.66, lignin C from <0.01 to 0.31, aliphatic C from 0.09 to 0.73, carbonyl C from 0.02 to 0.23, and char C from 0 to 0.45. This method is considered preferable to techniques involving imprecise extraction methods for RO wastes. Molecular composition data has great potential as a predictor of RO waste soil carbon and nutrient outcomes. 相似文献
83.
Primary production in the eutrophic Baltic Sea is limited by nitrogen availability; hence denitrification (natural transformation
of nitrate to gaseous N2) in the sediments is crucial in mitigating the effects of eutrophication. This study shows that dissimilatory nitrate reduction
to ammonium (DNRA) process, where nitrogen is not removed but instead recycled in the system, dominates nitrate reduction
in low oxygen conditions (O2 <110 μM), which have been persistent in the central Gulf of Finland during the past decade. The nitrogen removal rates measured
in this study show that nitrogen removal has decreased in the Gulf of Finland compared to rates measured in mid-1990s and
the decrease is most likely caused by the increased bottom water hypoxia. 相似文献
84.
Gert Jan Reinds Maximilian Posch 《Environmental pollution (Barking, Essex : 1987)》2009,157(4):1258-1269
The dynamic soil chemistry model SMART was applied to 121 intensive forest monitoring plots (mainly located in western and northern Europe) for which both element input (deposition) and element concentrations in the soil solution were available. After calibration of poorly known parameters, the model accurately simulated soil solution concentrations for most plots as indicated by goodness-of-fit measures, although some of the intra-annual variation especially in nitrate and aluminium concentrations could not be reproduced. Model evaluations of two emission-deposition scenarios (current legislation and maximum feasible reductions) for the period 1970-2030 show a strong reduction in sulphate concentrations between 1980 and 2000 in the soil due to the high reductions in sulphur emissions. However, current legislation hardly reduces future nitrogen concentrations, whereas maximum feasible reductions reduces them by more than half. Maximum feasible reductions are also more effective in increasing pH and reducing aluminium concentrations, mostly below ‘critical’ values. 相似文献
85.
Long-term depletion of calcium and other nutrients in eastern US forests 总被引:10,自引:0,他引:10
C. Anthony Federer James W. Hornbeck Louise M. Tritton C. Wayne Martin Robert S. Pierce C. Tattersall Smith 《Environmental management》1989,13(5):593-601
Both harvest removal and leaching losses can deplete nutrient capital in forests, but their combined long-term effects have not been assessed previously. We estimated changes in total soil and biomass N, Ca, K, Mg, and P over 120 years from published data for a spruce-fir site in Maine, two northern hardwood sites in New Hampshire, central hardwood sites in Connecticut and Tennessee, and a loblolly pine site in Tennessee. For N, atmospheric inputs counterbalance the outputs, and there is little long-term change on most sites. For K, Mg, and P, the total pool may decrease by 2%–10% in 120 years depending on site and harvest intensity. For Ca, net leaching loss is 4–16 kg/ha/yr in mature forests, and whole-tree harvest removes 200–1100 kg/ha. Such leaching loss and harvest removal could reduce total soil and biomass Ca by 20%–60% in only 120 years. We estimated unmeasured Ca inputs from rock breakdown, root-zone deepening, and dry deposition; these should not be expected to make up the Ca deficit. Acid precipitation may be the cause of current high leaching of Ca. Although Ca deficiency does not generally occur now in acid forest soils, it seems likely if anthropogenic leaching and intensive harvest removal continue. 相似文献
86.
The amount of struvite (MgNH4PO4·6H2O) produced by Myxococcus xanthus as well as the culture parameter values (pH, total phosphorus, total Kjeldahl nitrogen) were dependent on the culture medium used. Struvite formation started during the exponential phase and the maximum concentration was observed at the beginning of stationary growth phase. The addition of each medium component to the liquid culture influenced the amount of crystal produced. This amount did not depend on the pH increase during the culture period. The moment of the bacterial growth phase, at which each medium component was added, influenced the struvite formation. 相似文献
87.
A nonstationary time-series model is used to examine the changes occurring at sampling stations on the Chicago Sanitary and Ship Canal. Using data from upstream sampling sites, downstream levels of dissolved oxygen, total dissolved solids, nitrates and nitrites, and ammonia are accurately predicted. The method is simple, insensitive to extreme values, and responsive to changes in the system. 相似文献
88.
Brian P. Leaderer Rebecca T. Zagraniski Jan A. J. Stolwijk 《Environmental management》1977,1(1):31-37
A method is presented here by which the actual numbers of individuals in the U.S. population who would be expected to suffer respiratory illness as a result of exposure to ambient nitrogen dioxide (NO2) concentrations in excess of the Federally-designated ambient air quality standard can be estimated. At the same time we have attempted to quantify how these adverse health effects would be alleviated by various degrees of reductions in current ambient concentrations. In addition, the health benefit expected to be derived by various NOx emission control strategies will be examined utilizing the health benefit estimation method presented.It is estimated that there were approximately 33.2×106 excess cases of respiratory illnesses in the U.S. in 1973 associated with ambient NO2 concentrations in excess of the national ambient standard. A reduction of approximately 50 to 60 percent below 1973 NO2 levels is needed to essentially eliminate excess respiratory illness associated with ambient NO2 concentration. 相似文献
89.
《Journal of environmental science and health. Part. B》2013,48(6):865-881
The potential risk of groundwater contamination by the excessive leaching of N, P and heavy metals from soils amended at heavy loading rates of biosolids, coal ash, N‐viro soil (1:1 mixture of coal ash and biosolids), yard waste compost and co‐compost (3:7 mixture of biosolids to yard wastes), and by soil incorporation of green manures of sunn hemp (Crotalaria juncea) and sorghum sudangrass (Sorghum bicolor × S. bicolor var. sudanense) was studied by collecting and analyzing leachates from pots of Krome very gravelly loam soil subjected to these treatments. The control consisted of Krome soil without any amendment. The loading rate was 205 g pot? 1 for each amendment (equivalent to 50 t ha? 1 of the dry weight), and the amounts of the cover crops incorporated into the soil in the pot were those that had been grown in it. A subtropical vegetable crop, okra (Abelmoschus esculentus L.), was grown after the soil amendments or cover crops had been incorporated into the soil. The results showed that the concentration of NO3‐N in leachate from biosolids was significantly higher than in leachate from other treatments. The levels of heavy metals found in the leachates from all amended soils were so low, as to suggest these amendments may be used without risk of leaching dangerous amounts of these toxic elements. Nevertheless the level of heavy metals in leachate from coal ash amended soil was substantially greater than in leachates from the other treatments. The leguminous cover crop, sunn hemp, returned into the soil, increased the leachate NO3‐N and inorganic P concentration significantly compared with the non‐legume, sorghum sudangrass. The results suggest that at heavy loading rates of soil amendments, leaching of NO3 ? could be a significant concern by application of biosolids. Leaching of inorganic P can be increased significantly by both co‐compost and biosolids, but decreased by coal ash and N‐viro soil by virtue of improved adsorption. The leguminous cover crop, sunn hemp, when incorporated into the soil, can cause the concentration of NO3‐N to increase by about 7 fold, and that of inorganic P by about 23% over the non‐legume. Regarding the metals, biosolids, N‐viro soil and coal ash significantly increased Ca and Mg concentrations in leachates. Copper concentration in leachate was increased by application of biosolids, while Fe concentration in leachates was increased by biosolids, coal ash and co‐compost. The concentrations of Zn, Mo and Co in leachate were increased by application of coal ash. The concentrations of heavy metals in leachates were very low and unlikely to be harmful, although they were increased significantly by coal ash application. 相似文献
90.
Sally R. Gadsdon Sally A. Power 《Environmental pollution (Barking, Essex : 1987)》2009,157(10):2845-2852
NO2 and NH3 concentrations were measured across a Special Area for Conservation in southern England, at varying distances from the local road network. Exceedances of the critical levels for these pollutants were recorded at nearly all roadside locations, extending up to 20 m away from roads at some sites. Further, paired measurements of NH3 and NO2 concentrations revealed differences between ground and tree canopy levels. At “background” sites, away from the direct influence of roads, concentrations were higher within tree canopies than at ground level; the reverse pattern was, however, seen at roadside locations. Calculations of pollutant deposition rates showed that nitrogen inputs are dominated by NH3 at roadside sites. This study demonstrates that local traffic emissions contribute substantially to the exceedance of critical levels and critical loads, and suggests that on-site monitoring is needed for sites of nature conservation value which are in close proximity to local transport routes. 相似文献