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51.
J. L. Hanisch B. R. Hart W. S. Turetsky H. T. Garabedian G. H. Pain 《Environmental management》1978,2(2):127-133
The body of information presented in this paper is directed to air pollution engineers who are concerned with the effect of indirect sources on ambient concentrations of carbon monoxide (CO). Data taken under controlled conditions are used to empirically derive and calibrate a model for predicting CO concentrations in the vicinity of roadway intersections and other points of possible vehicular congestion. Since the predicted free flow CO contribution of vehicles traveling at normal road speeds is relatively low, it is concluded that idling vehicles at points of congestion are the major cause of CO violations, and that state and federal programs should place more emphasis on relieving congestion and reducing idling emission rates in new vehicles. 相似文献
52.
The concentrations, distribution and sources of PAHs in agricultural soils and vegetables from Shunde, Guangdong, China 总被引:4,自引:0,他引:4
Li YT Li FB Chen JJ Yang GY Wan HF Zhang TB Zeng XD Liu JM 《Environmental monitoring and assessment》2008,139(1-3):61-76
The concentrations, distribution and sources of 16 polycyclic aromatic hydrocarbons (PAHs) were determined in 30 agricultural
soil and 16 vegetable samples collected from subtropical Shunde area, an important manufacturing center in China. The total
PAHs ranged from 33.7 to 350 μg/kg in soils, and 82 to 1,258 μg/kg in vegetables. The most abundant individual PAHs are phenanthrene,
fluoranthene, chrysene, pyrene and benzo(b)fluoranthene for soil samples, and anthracene, naphthalene, phenanthrene, pyrene
and chrysene for vegetable samples. Average vegetable–soil ratios of total PAHs were 2.20 for leafy vegetables and 1.27 for
fruity vegetables. Total PAHs in vegetable samples are not significantly correlated to those in corresponding soil samples.
Principal component analyses were conducted to distinguish samples on basis of their distribution in each town, soil type
and vegetable specie. Relatively abundant soil PAHs were found in town Jun’an, Beijiao, Chencun, Lecong and Ronggui, while
abundant vegetable PAHs were observed in town Jun’an, Lecong, Xingtan, Daliang and Chenchun. The highest level of total PAHs
were found in vegetable soil, followed by pond sediment and “stacked soil” on pond banks. The PAHs contents in leafy vegetables
are higher than those in fruity vegetables. Some PAH compound ratios suggest the PAHs derived from incomplete combustion of
petroleum, coal and refuse from power generation and ceramic manufacturing, and paint spraying on furniture, as well as sewage
irrigation from textile industries. Soil PAHs contents have significant logarithmic correlation with total organic carbon,
which demonstrates the importance of soil organic matter as sorbent to prevent losses of PAHs. 相似文献
53.
徐州城市表层土壤中重金属的富积、分布特征与环境风险 总被引:3,自引:0,他引:3
研究了徐州城市表层土壤的21个样品中30种元素的富集与分布特征。结果表明,与我国土壤元素的背景值(算术平均值)相比,表层土壤中Zn、Cd、As、Hg、Sb、Sn、Ag等元素富集大;Fe、Se、Sc、Ba、Bi、Pb、Cu、Ni、Cr、Mn、Mo、Be、Ti、Al、Ga、Li、Co等元素的富集较小。污染元素的空间分布特征显示了Zn、Cu、Pb、Cd等元素主要与交通运输等扩散污染源相关,而元素As、Sb的空间分布主要与工业污染源(点源)有关。环境风险指数的计算结果表明,表层土壤中重金属污染具有较大的环境风险,其中属于中等环境风险级别以上的样品占近40%,而且高风险区域主要集中在钢铁厂和化机厂等工业区范围内。 相似文献
54.
Kelsey RH Scott GI Porter DE Thompson B Webster L 《Environmental monitoring and assessment》2003,81(1-3):337-348
Multiple Antibiotic Resistance (MAR) analysis and regression modeling techniques were used to identify surface water areas impacted by fecal pollution from human sources, and to determine the effects of land use on fecal pollution in Murrells Inlet, a small, urbanized, high-salinity estuary located between Myrtle Beach and Georgetown, South Carolina. MAR analysis was performed to identify areas in the estuary that are impacted by human-source fecal pollution. Additionally, regression analysis was performed to determine if an association exists between land use and fecal coliform densities over the ten-year period from 1989 to 1998. Land-use variables were derived using Geographic Information System (GIS) techniques and were used in the regression analysis.MAR analyses were conducted by comparing the frequency and patterns of antibiotic resistance found in Escherichia coli isolates derived from surface water samples and from sewage sources in the Murrells Inlet sewage collection system. The MAR results suggest that the majority of the fecal pollution detected in the Murrells Inlet estuary may be from non-human sources, including fecal coliforms isolated from areas in close proximity to high densities of active septic tanks.A MAR Index, which measures the frequency of antibiotic resistance, was calculated for each of twenty-three water samples and nine sewage samples. The antibiotic resistance pattern comparisons were performed using cluster analysis. Although the MAR indices indicated that several surface water sites had potential human-source contamination, the cluster analysis suggests that only one sampling site had MAR patterns that were similar to those found in the sewage samples. This site was in close proximity to several large pleasure boats as well as a sewage collection system lift station, but was not near areas with active septic tanks. The results of the regression analysis also suggest that sewage sources and rainfall runoff from urbanized areas may contribute to fecal pollution in the estuary. 相似文献
55.
《环境科学学报(英文版)》2023,35(4):708-721
Nowadays, the fine particle pollution is still severe in some megacities of China, especially in the Sichuan Basin, southwestern China. In order to understand the causes, sources, and impacts of fine particles, we collected PM2.5 samples and analyzed their chemical composition in typical months from July 2018 to May 2019 at an urban and a suburban (background) site of Chengdu, a megacity in this region. The daily average concentrations of PM2.5 ranged from 5.6-102.3 µg/m3 and 4.3-110.4 µg/m3 at each site. Secondary inorganics and organic matters were the major components in PM2.5 at both sites. The proportion of nitrate in PM2.5 has exceeded sulfate and become the primary inorganic component. SO2 was easier to transform into sulfate in urban areas because of Mn-catalytic heterogeneous reactions. In contrast, NO2 was easily converted in suburbs with high aerosol water content. Furthermore, organic carbon in urban was much greater than that in rural, other than elemental carbon. Element Cr and As were the key cancer risk drivers. The main sources of PM2.5 in urban and suburban areas were all secondary aerosols (42.9%, 32.1%), combustion (16.0%, 25.2%) and vehicle emission (15.2%, 19.2%). From clean period to pollution period, the contributions from combustion and secondary aerosols increased markedly. In addition to tightening vehicle controls, urban areas need to restrict emissions from steel smelters, and suburbs need to minimize coal and biomass combustion in autumn and winter. 相似文献
56.
57.
Racha Dejchanchaiwong Napawan Mahasakpan Phatsarakorn Chaisongkaew Muanfun Iner Nobchonnee Nim Worradorn Phairuang Surajit Tekasakul Masami Furuuchi Mitsuhiko Hat Thaniya Kaosol Perapong Tekasakul 《环境科学学报(英文版)》2023,35(2):253-267
Distribution of PM0.1,PM1and PM2.5particle-and gas-polycyclic aromatic hydrocarbons(PAHs) during the 2019 normal,partial and strong haze periods at a background location in southern Thailand were investigated to understand the behaviors and carcinogenic risks PM1was the predominant component,during partial and strong haze periods,accounting for 45.1%and 52.9%of total suspended particulate matter,respectively,while during nor mal period the contribution... 相似文献
58.
59.
对2005年7月至2006年2月采集到的南京市气溶胶Pm2.5 进行季节性初步分析,并对其中的15种优控多环芳烃(PAHs)进行分析研究,通过比值法判断南京市PAHs夏季主要来源于柴油型燃烧,冬季主要来源于柴油和煤型相结合的燃烧.对15种优控PAHs两两之间的相关性分析,发现各化合物之间显著相关,表明各化合物的来源有相似之处. 相似文献
60.
Tracing the sources of refractory dissolved organic matter in a large artificial lake using multiple analytical tools 总被引:2,自引:0,他引:2
Structural and chemical characteristics of refractory dissolved organic matter (RDOM) from seven different sources (algae, leaf litter, reed, compost, field soil, paddy water, treated sewage) were examined using multiple analytical tools, and they were compared with those of RDOM in a large artificial lake (Lake Paldang, Korea). Treated sewage, paddy water, and field soil were distinguished from the other sources investigated by their relatively low specific UV absorbance (SUVA) values and more pronounced fulvic-like versus humic-like fluorescence of the RDOM samples. Microbial derived RDOM from algae and treated sewage showed relatively low apparent molecular weight and a higher fraction of hydrophilic bases relative to the total hydrophilic fraction. For the biopolymer types, the presence of polyhydroxy aromatics with the high abundance of proteins was observed only for vascular plant-based RDOM (i.e., leaf litter and reed). Molecular weight values exhibited positive correlations with the SUVA and the hydrophobic content among the different RDOM, suggesting that hydrophobic and condensed aromatic structures may be the main components of high molecular weight RDOM. Principal component analysis revealed that approximately 77% of the variance in the RDOM characteristics might be explained by the source difference (i.e., terrestrial and microbial derived) and a tendency of further microbial transformation. Combined results demonstrated that the properties of the lake RDOM were largely affected by the upstream sources of field soil, paddy water, and treated sewage, which are characterized by low molecular weight UV-absorbing and non-aromatic structures with relatively high resistance to further degradation. 相似文献