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1.
Background, Aim and Scope Air quality is an field of major concern in large cities. This problem has led administrations to introduce plans and regulations
to reduce pollutant emissions. The analysis of variations in the concentration of pollutants is useful when evaluating the
effectiveness of these plans. However, such an analysis cannot be undertaken using standard statistical techniques, due to
the fact that concentrations of atmospheric pollutants often exhibit a lack of normality and are autocorrelated. On the other
hand, if long-term trends of any pollutant’s emissions are to be detected, meteorological effects must be removed from the
time series analysed, due to their strong masking effects.
Materials and Methods The application of statistical methods to analyse temporal variations is illustrated using monthly carbon monoxide (CO) concentrations
observed at an urban site. The sampling site is located at a street intersection in central Valencia (Spain) with a high traffic
density. Valencia is the third largest city in Spain. It is a typical Mediterranean city in terms of its urban structure and
climatology. The sampling site started operation in January 1994 and monitored CO ground level concentrations until February
2002. Its geographic coordinates are W0°22′52″ N39°28′05″ and its altitude is 11 m. Two nonparametric trend tests are applied.
One of these is robust against serial correlation with regards to the false rejection rate, when observations have a strong
persistence or when the sample size per month is small. A nonparametric analysis of the homogeneity of trends between seasons
is also discussed. A multiple linear regression model is used with the transformed data, including the effect of meteorological
variables. The method of generalized least squares is applied to estimate the model parameters to take into account the serial
dependence of the residuals of this model. This study also assesses temporal changes using the Kolmogorov-Zurbenko (KZ) filter.
The KZ filter has been shown to be an effective way to remove the influence of meteorological conditions on O3 and PM to examine underlying trends.
Results The nonparametric tests indicate a decreasing, significant trend in the sampled site. The application of the linear model
yields a significant decrease every twelve months of 15.8% for the average monthly CO concentration. The 95% confidence interval
for the trend ranges from 13.9% to 17.7%. The seasonal cycle also provides significant results. There are no differences in
trends throughout the months. The percentage of CO variance explained by the linear model is 90.3%. The KZ filter separates
out long, short-term and seasonal variations in the CO series. The estimated, significant, long-term trend every year results
in 10.3% with this method. The 95% confidence interval ranges from 8.8% to 11.9%. This approach explains 89.9% of the CO temporal
variations.
Discussion The differences between the linear model and KZ filter trend estimations are due to the fact that the KZ filter performs the
analysis on the smoothed data rather than the original data. In the KZ filter trend estimation, the effect of meteorological
conditions has been removed. The CO short-term componentis attributable to weather and short-term fluctuations in emissions.
There is a significant seasonal cycle. This component is a result of changes in the traffic, the yearly meteorological cycle
and the interactions between these two factors. There are peaks during the autumn and winter months, which have more traffic
density in the sampled site. There is a minimum during the month of August, reflecting the very low level of vehicle emissions
which is a direct consequence of the holiday period.
Conclusions The significant, decreasing trend implies to a certain extent that the urban environment in the area is improving. This trend
results from changes in overall emissions, pollutant transport, climate, policy and economics. It is also due to the effect
of introducing reformulated gasoline. The additives enable vehicles to burn fuel with a higher air/fuel ratio, thereby lowering
the emission of CO. The KZ filter has been the most effective method to separate the CO series components and to obtain an
estimate of the long-term trend due to changes in emissions, removing the effect of meteorological conditions.
Recommendations and Perspectives Air quality managers and policy-makers must understand the link between climate and pollutants to select optimal pollutant
reduction strategies and avoid exceeding emission directives. This paper analyses eight years of ambient CO data at a site
with a high traffic density, and provides results that are useful for decision-making. The assessment of long-term changes
in air pollutants to evaluate reduction strategies has to be done while taking into account meteorological variability 相似文献
2.
研制了一种测定水中Mg2 + 的测试管 ,测定范围为 0 .5mg/L~ 2 .0mg/L。该测试管适用于现场应急监测 ,具有快速、简便、抗干扰能力强和价格低廉等特点 相似文献
3.
4.
关于我国一氧化碳室内空气质量评价标准的建议 总被引:1,自引:0,他引:1
人们大部分时间处于室内,室内空气质量直接影响人们的身体健康。当前,室内空气污染己成为社会关注的热点问题,一氧化碳(CO)含量高低是室内空气质量(IAQ)好坏的重要指示指标。本文通过分析一氧化碳(CO)的理化特性,来源,毒理学研究和流行病学研究结果,在参考世界卫生组织(WHO)或国外相关标准的基础上,结合我国的实际情况和目前污染水平,首次提出了我国一氧化碳(CO)室内空气质量三级标准建议值。 相似文献
5.
IntroductionEightypercentoforganicsubstancesinthesourcewaterisfromcrudehumicacidthatisacrudeorganiccompoundcreatedbyrottinganddecomposinginnaturalcycle ,thehighercontentofhumicacidis ,theworsequalityofthewateris,notonlycanitcausechrominance,offensiveodor,… 相似文献
6.
对含柠檬酸盐电镀废水的几种处理方法的比较表明,氯化钡添加法能较好地使柠檬酸盐沉淀,操作简便,处理效果理想,其柠檬酸根离子的去除率达98%以上。 相似文献
7.
SO2 和氟化物对农作物的危害可通过症状、镜检和受害叶片的化学分析来鉴别 ,并从风向、与污染源距离、障碍物和叶片成熟程度几方面与作物病虫等影响因素相区别。排放浓度、接触时和作物本身抗性是影响危害程度的主要因素。应从治理污染、选种抗性强树木、避开作物敏感生育期、合理种植、加强施肥等方面采取措施加以防治 相似文献
8.
窑尾监测SO_2时,有时会出现其浓度低于仪器最低检出限的情况,应根据窖尾类型、煤中硫含量大小,有无脱硫工艺等情况,认真对比、计算分析,以保证监测数据真实可靠。 相似文献
9.
Gong Peiyu Wu Kunjun Li XiuzhenInstitute of Zoology Chinese Academy of Sciences Beijing China. 《环境科学学报(英文版)》1993,(2)
SO2 Pollution; rape plant (Brassica chinensis); turnip moth (Agrotis segetum); growth and developmental parameters. 相似文献
10.
Stickler syndrome is an autosomal dominant disorder of the connective tissue which includes ocular and systemic manifestations. We report on a large kindred in which we were able to demonstrate very tight linkage between the disease and the type II collagen gene (COL2A1) (LOD score 3·91 at θ=0). In a family in which the father and one of his daughters were severely affected, DNA analysis from a chorionic villus sample demonstrated that the fetus possessed the normal allele of COL2A1. Thereafter a normal child was born. 相似文献