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Fowler D. Sutton M. A. Flechard C. Cape J. N. Storeton-West R. Coyle M. Smith R. I. 《Water, Air, & Soil Pollution: Focus》2001,1(5-6):39-48
Two years of continuous measurements of SO2deposition fluxes to moorland vegetation are reported. The mean flux of 2.8 ng SO2 m-2 s-1 is regulated predominantly by surface resistance (r
c) which, even for wet surfaces, was seldom smaller than 100 s m-1. The control of surface resistance is shown to be regulated by the ratio of NH3SO2 concentrations with an excess of NH3 generating the small surface resistances for SO2. A dynamic surface chemistry model is used to simulate the effects of NH3 on SO2 deposition flux and is able to capture responses to short-term changes in ambient concentrations of SO2, NH3 and meteorological conditions. The coupling between surface resistance and NH3/SO2 concentration ratios shows that the deposition velocity for SO2 is regulated by the regional pollution climate. Recent long-term SO2 flux measurements in a transect over Europe demonstrate the close link between NH3/SO2 concentrations and rc (SO2). The deposition velocity for SO2 is predicted to have increased with time since the 1970s and imply a 40% increase in v
d at a site at which the annual mean ambient SO2 concentrations declined from 47 to 3 g m-3 between 1973 and 1998. 相似文献
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Hargreaves KJ Fowler D Storeton-West RL Duyzer JH 《Environmental pollution (Barking, Essex : 1987)》1992,75(1):53-59
Fluxes of NO, NO2 and O3 were determined over a drained marshland pasture in south-east England by using flux-gradient techniques. Nitric oxide was found to be emitted at rates of up to 40 ng m(-2) s(-1), the rate of emission being related to the magnitude of the eddy diffusivity. Nitrogen dioxide deposited at rates of up to 90 ng m(-2) s(-1) under the control of stomatal resistance, a clear diurnal cycle being observed. Minimum canopy resistance was of the order of 80 s m(-1). Ozone deposition was also controlled by stomatal resistance, the minimum canopy resistance being around 100 s m(-1) and fluxes reaching a maximum of 220 ng m(-2) s(-1). Corrections made to NO and NO2 fluxes to compensate for chemical reactions showed flux divergences of the order of 30% for NO and NO2, but these were not statistically significantly different from the measured fluxes. The pasture was found to be a net sink for nitrogen in the form of NOx. 相似文献
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