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Boy Jens Strey Simone Schönenberg Regine Strey Robert Weber-Santos Oscarlina Nendel Claas Klingler Michael Schumann Charlotte Hartberger Korbinian Guggenberger Georg 《Regional Environmental Change》2018,18(1):63-75
Regional Environmental Change - Soil carbon stocks of 29 plots along a transect through tropical Brazil showed only minor soil carbon losses after land use shift, although replacement of... 相似文献
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Korbinian P. Freier Rainer Brüggemann Gunnar Nützmann 《Environmental Sciences Europe》2007,19(3):189-196
Background
Current hydrological research is increasingly focusing on pharmaceutically active compounds (PhACs). Concerning the issue of quality of drinking water, this problem has also become the focus of public interest. However, in spire of the fact that the fate of chemicals in surface waters has been assessed in great detail, the influence of groundwater-exchange is yet only little known.Goal
This study gives emphasis to the question of how transport and degradation of PhACs interact with the exchange of surface water with groundwater. Special interest is given to alternating groundwater regimes.Methods
Based on a small stream system in the north of Berlin, Germany, a one-dimensional compartment-model was established using differential mass-balance. The stream which, at its mouth, discharges 0.3 m3 s?1 is already well investigated and thus provides a good empirical data basis. The processes taken into account by the model were ‘exchange of surface-water with groundwater’, ‘decomposition’ as well as ‘transport’ of PhACs. Calculations were performed using the commonly used analgesic Diclofenac as an example and defining 81 scenarios by different groundwater regimes. Hasse Diagramm Technique was used to compare the scenarios.Results
All scenarios show a big influence of groundwater-exchange to the fate and concentration of PhACs in surface waters. In the case of the modelled stream system, dilution by groundwater was more responsible for a decrease in concentration than degradation was. Furthermore, on the background of a standard scenario, the loss due to groundwater by 5.4 percent was in the same magnitude as the loss due to decomposition (9.7 percent). A crucial difference between punctual versus linear afflux of groundwater has not been observed.Discussion
The alteration of discharge resulted in a big influence of the case differentiation between ‘constant velocity’ and ‘constant cross-section’. Furthermore, the model was based on the assumption that groundwater was unloaded with PhACs or diluted very well in comparison to the stream. In contrast, regarding measurements in the catchment, groundwater could even be a diffuse source of the contamination of the stream.Conclusions
The fate of PhACs in our model is crucially driven by interactions with groundwater. Therefore, assessing the risk emanating from substances like Diclofenac, it is very important to regard their accessibility to decomposition as well as the morphology of the stream-system and its interactions with the groundwater.Perspectives
In this model, the process of transport from the surface to groundwater back to the surface was dealt with insufficiently; in order to be able to observe fully developed interaction in a further step of modelling, a groundwater-transportmodel should be coupled completely with a surface-water-model. 相似文献
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