三峡库区消落带农用坡地磷素径流流失特征

消落带是三峡库区重要的生态交错带，但自发农用和无序开发可能会造成更多的氮磷流失，进而加剧三峡库区水体富营养化。通过对库区连续3 a的定位监测（2011~2013年），研究了三峡库区消落带农用坡地的磷素流失特征。结果表明：次降雨事件中常规施肥处理的地表径流、壤中流总磷平均浓度分别为0.848±0.153、0.140±0.006 mg/L，其中地表径流中磷的形态以颗粒态为主，壤中流以溶解态的生物可利用磷为主。常规施肥下，地表径流、壤中流磷素年均流失通量分别为0.236±0.004、0.100±0.003 kg·hm 2，地表径流、壤中流磷素流失通量分别占总流失通量的70.2%、29.8%，地表径流是坡地磷素流失的主要途径，但壤中流也是不可忽视的重要途径。与常规施肥处理相比，减量施肥处理地表径流、壤中流磷素流失量分别降低了45.3%、40.0%。建议采取减量施肥的方式，以降低营养盐负荷，保护水环境。     

The regulatory role of endogenous iron on greenhouse gas emissions under intensive nitrogen fertilization in subtropical soils of China

Environmental Science and Pollution Research - Anaerobic batch experiments were conducted to study the regulatory role of endogenous iron in greenhouse gas emissions under intensive nitrogen...     

Study of the adsorption of endocrine disruptor compounds on typical filter materials using a quartz crystal microbalance

Environmental Science and Pollution Research - Drinking water containing environmental endocrine disruptor compounds (EDCs) endangers human health, and researching the purification process of...     

天津市地表水体与沉积物中7种高关注酚类化合物的污染特征与生态风险分析

为探究地表水体与沉积物中酚类化合物的污染分布特征和生态风险,选择天津市3个水源地与6条主要河流,采集了26个地表水样与6个沉积物样品,利用固相萃取与超声萃取、高效液相色谱-串联质谱法(HPLC-MS/MS)测定了水样及沉积物中1-萘酚(1-naphthol)、壬基酚(nonylphenol, NP)、双酚A(bisphenol A, BPA)、2-苯基苯酚(biphenyl-2-ol)、3,4-二氯酚(3,4-dichlorophenol)、四溴双酚A(tetrabromobisphenol A, TBBPA)和对叔丁基苯酚(p-tert-butylphenol, PTBP)等7种高关注酚类化合物的浓度水平,并应用物种敏感性分布(species sensitivity distribution, SSD)法和熵值法(ecological risk quotient, RQ)评估7种酚类化合物水环境和沉积物的生态风险。结果表明,地表水样中7种酚类化合物均全部检出;其中壬基酚的检出浓度最高,其次为四溴双酚A、对叔丁基苯酚、1-萘酚、2-苯基苯酚、3,4-二氯酚和双酚A。沉积物中酚类化合物的污染分布规律与水样相似,除双酚A外的目标物全部检出。其中,壬基酚浓度比其他物质浓度高2个数量级。风险评估结果显示,壬基酚对水环境与沉积物存在不可接受的风险;而四溴双酚A、对叔丁基苯酚、1-萘酚、2-苯基苯酚、3,4-二氯酚和双酚A则对环境具有较低风险或者存在一定的风险。     

玛纳斯河流域荒漠草地沙化遥感监测研究

以1989—2016年玛纳斯河流域TM/OLI遥感影像为数据源,利用混合像元分解技术,计算玛纳斯河流域草地总覆盖度和裸沙面积。在此基础上通过监测年与基期年的比较,计算草地覆盖度相对基期年的减少率和裸沙面积相对基期年的增加率两个监测指标,依据《天然草地退化、沙化、盐渍化的分级指标》(GB 19377—2003),对计算出的两个指标分别进行沙化等级评定和赋值,将两种评定结果相综合来监测草地沙化。结果表明,玛纳斯河流域近30年来荒漠草地沙漠化总体呈现先增加后降低的趋势。分析表明,玛纳斯河流域草地沙化是人为和自然因素双重作用的结果。     

Quantification of nitrogen in the liquid fraction and in vitro assessment of lysine bioavailability in the solid fraction of soybean meal hydrolysates

Soybean meal (SBM) is a product generated from the manufacture of soybean oil and has the potential for use as a source of fermentable sugars for ethanol production or as a protein source for animal feeds. Knowing the levels of nitrogen available from ammonium is a necessary element of the ethanolic fermentation process while identifying the levels of essential amino acids such as lysine is important in determining usage as a feed source. As such the purpose of this study was to quantify total nitrogen and ammonium in the liquid fraction of hydrolyzed SBM and to evaluate total and bioavailable lysine in the solid fraction of the hydrolyzed SBM. The effects of acid concentration, cellulase and β-glucosidase on total and ammonium nitrogen were studied with analysis indicating that higher acid concentrations increased nitrogen compounds with ammonium concentrations ranging from 0.20 to 1.24 g L^?1 while enzymatic treatments did not significantly increase nitrogen levels. Total and bioavailable lysine was quantified by use of an auxotrophic gfpmut3 E.coli whole-cell bioassay organism incapable of lysine biosynthesis. Acid and enzymatic treatments were applied with lysine bioavailability increasing from a base of 82% for untreated SBM to up to 97%. Our results demonstrated that SBM has the potential to serve in ethanolic fermentation and as an optimal source essential amino acid lysine.     

Structural and technological determinants of carbon intensity reduction of China’s electricity generation

Environmental Science and Pollution Research - Electricity generation is the largest sector with decarbonization potential for China and the world. Based on the new emission factors, this paper...     

试论生态文明制度体系的构建

建立健全生态文明制度体系是推进我国生态文明建设的重点。党的十八届三中全会通过的《中共中央关于全面深化改革若干重大问题的决定》指出,生态文明制度体系应当包括决策制度、评价制度、管理制度与考核制度等内容。立足社会主义制度建设的中国特色,针对我国生态文明建设的具体需求,本文将生态文明制度体系解构为四大板块:绿色高效决策制度、生态有价评估制度、生态环境监管制度与生态优先考核制度,并进一步明确了各项制度构建工作的具体内容。生态文明制度体系的构建和不断完善,将为全面建成人与自然和谐的美丽中国提供系统保障。     

Background biomonitoring of residue levels of 137 pesticides in the blood plasma of the general population in Beijing

Due to the widespread use of pesticides, human exposure to pesticides is possible and can potentially cause adverse impacts on public health. We measured 137 pesticides including organophosphorus, organochlorine, pyrethroid and carbamate pesticides together with various herbicides in 100 human blood samples collected from the general population in Beijing. The samples were analysed by triple quadrupole tandem gas chromatography-mass spectrometry. In total, 24 organochlorine pesticides, 5 pyrethroid pesticides and 6 organophosphorus pesticides were detected. The detection rates of HCB, α-HCH, β-HCH, γ-HCH, p,p′-DDE and quintozene were 99, 96, 74, 72, 96 and 95%, respectively. No statistically significant gender difference in the blood concentrations of the pesticides was found. Consistent with the trend of the increasing β-HCH, p,p′-DDE and quintozene concentrations with age, a strong positive correlation between the age and concentrations of β-BHC, p,p′-DDE and quintozene was observed.     

NOx attenuation in flue gas by •OH/SO4•--based advanced oxidation processes

Environmental Science and Pollution Research - The combustion of fossil fuels has resulted in rapidly increasing emissions of nitrogen oxide (NOx), which has caused serious human health and...