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生物脱氮好氧阶段不同反应过程N2O产量
引用本文:巩有奎, 苗志加, 彭永臻. 生物脱氮好氧阶段不同反应过程N2O产量[J]. 环境工程学报, 2016, 10(12): 6963-6968. doi: 10.12030/j.cjee.201505067
作者姓名:巩有奎  苗志加  彭永臻
作者单位:1. 石家庄铁路职业技术学院, 石家庄 050041; 2. 北京工业大学环境与能源工程学院, 北京 100022; 3. 河北地质大学水资源与环境学院, 石家庄 050031
基金项目:国家自然科学基金资助项目(51008005) 河北省高等学校科学技术研究青年基金项目(QN2013172)
摘    要:在成功实现生活污水短程生物脱氮的基础上,采用体积为3 L的小试反应器,利用在线DO监测手段控制DO=1.0 mg·L-1,通过投加NaNO2的方式控制系统初始NO2--N=40 mg·L-1,以丙烯基硫脲(ATU)抑制NH4+-N的氧化过程,考察了生物脱氮好氧阶段不同反应过程中N2O的产生量。结果表明,除缺氧反硝化细菌的反硝化过程外,好氧条件下,氨氧化菌(AOB)能够以NH4+-N作为电子供体,NO2--N作为电子受体,进行反硝化脱氮过程,其反硝化产物为N2O。生物脱氮好氧阶段AOB的好氧反硝化和异养菌的缺氧反硝化反应中,N2O的产量分别占分别占进水总氮(NH4+-N+NO2--N)的7.23%和7.80%。好氧阶段NH4+-N和NO2-的氧化过程中,几乎没有N2O的产生。

关 键 词:N2O   硝化菌反硝化   缺氧反硝化   亚硝态氮
收稿时间:2015-06-30

Nitrous oxide production from sequencing batch reactor sludge under nitrifying conditions of different process
GONG Youkui, MIAO Zhijia, PENG Yongzhen. Nitrous oxide production from sequencing batch reactor sludge under nitrifying conditions of different process[J]. Chinese Journal of Environmental Engineering, 2016, 10(12): 6963-6968. doi: 10.12030/j.cjee.201505067
Authors:GONG Youkui  MIAO Zhijia  PENG Yongzhen
Affiliation:1. Shijiazhuang Institute of Railway Technology, Shijiazhuang 050041, China; 2. College of Environmental and Energy Engineering, Beijing University of Technology, Beijing 100022, China; 3. School of Water Resources and Environment, Hebei Geological University, Shijiazhuang 050031, China
Abstract:Contributions of NH4+ oxidation,NO2- oxidation,and heterotrophic and nitrifier denitrification during the N-removal process were investigated in a lab-scale nitrifying reactor.Allylthiourea (ATU) was used to inhibit NH4+ oxidation and investigate processes under nitrifying conditions.The results confirmed that besides heterotrophic bacteria,ammonium-oxidizing bacteria (AOB) could undertake denitrification processes,with NH4+ as the electron donor,NO2- as the electron acceptor,and N2O as one of the final products.The relative contribution of the heterotrophic and nitrifier denitrification to total N2O emission was 51% and 47%,respectively.Little N2O was emitted during the NH4+ and NO2- oxidation processes.
Keywords:N2O  denitrification of nitrification bacteria  anoxic denitrification  nitrite nitrogen
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