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Modeling of air quality with a modified two-dimensional Eulerian model: A case study in the Pearl River Delta (PRD) region of China
作者姓名:CHENG Yan-li  BAI Yu-hu  LI Jin-long  LIU Zhao-rong
作者单位:College of Environmental Sciences, Peking University, Beijing 100871, China
基金项目:国家自然科学基金 , 国家重点基础研究发展计划(973计划)
摘    要:A modified two-dimensional Eulerian air quality model was used to simulate both the gaseous and particulate pollutant concentrations during October 21-24, 2004 in the Pearl River Delta (PRD) region, China. The most significant improvement to the model is the added capability to predict the secondary organic aerosols (SOA) concentrations because of the inclusion of the SOA formation chemistry. The meteorological input data were prepared using the CALMET meteorological model. The concentrations of aerosol-bound species such as NO3^-, NH4^+, SO4^2-, and SOA were calculated in the fine particle size range (〈2.5 μm). The results of the two-dimensional model were compared to the measurements at the ground level during the PRD Intensive Monitoring Campaign (IMC). Overall, there were good agreements between the measured and modeled concentrations of inorganic aerosol components and O3. Both the measured and the modeled results indicated that the maximum hourly O3 concentrations exceeded the China National Air Quality Standard. The predicted 24-h average SOA concentrations were in reasonable agreement with those predicted by the method of minimum OC/EC ratio.

关 键 词:珠江三角洲地区  空气质量  改良欧拉二维模型  建模  气溶胶
收稿时间:2006-05-29
修稿时间:2006-08-14

Modeling of air quality with a modified two-dimensional Eulerian model: A case study in the Pearl River Delta (PRD) region of China
CHENG Yan-li,BAI Yu-hu,LI Jin-long,LIU Zhao-rong.Modeling of air quality with a modified two-dimensional Eulerian model: A case study in the Pearl River Delta (PRD) region of China[J].Journal of Environmental Sciences,2007,19(5):572-577.
Authors:CHENG Yan-li  BAI Yu-hu  LI Jin-long and LIU Zhao-rong
Institution:College of Environmental Sciences, Peking University, Beijing 100871, China
Abstract:A modified two-dimensional Eulerian air quality model was used to simulate both the gaseous and particulate pollutant concentrations during October 21-24, 2004 in the Pearl River Delta (PRD) region, China. The most significant improvement to the model is the added capability to predict the secondary organic aerosols (SOA) concentrations because of the inclusion of the SOA formation chemistry. The meteorological input data were prepared using the CALMET meteorological model. The concentrations of aerosol-bound species such as NO3-, NH4 , SO42-, and SOA were calculated in the fine particle size range (<2.5 μm). The results of the two-dimensional model were compared to the measurements at the ground level during the PRD Intensive Monitoring Campaign (IMC). Overall, there were good agreements between the measured and modeled concentrations of inorganic aerosol components and O3. Both the measured and the modeled results indicated that the maximum hourly O3 concentrations exceeded the China National Air Quality Standard. The predicted 24-h average SOA concentrations were in reasonable agreement with those predicted by the method of minimum OC/EC ratio.
Keywords:air quality model  numerical simulation  secondary organic aerosol  inorganic aerosol  model  modified  air quality  Modeling  the Pearl River Delta  case study  ratio  average  reasonable  method of  minimum  maximum  National  Standard  good  inorganic  aerosol  components  results  measurements
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