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电晕氧化结合化学吸收脱除烟气中NO2实验研究
引用本文:魏恩宗.电晕氧化结合化学吸收脱除烟气中NO2实验研究[J].环境科学学报,2004,24(6):1074-1078.
作者姓名:魏恩宗
作者单位:浙江大学能源洁净利用与环境工程教育部重点实验室,杭州,310027
基金项目:国家"863"计划资助项目(2002AA529180);博士点基金资助项目(20020335061);浙江省科技计划项目(2003201509)
摘    要:实验研究了直流电晕湿空气自由基簇射结合25%的NaOH溶液吸收的NOx脱除过程.结果表明:通过调节流过喷嘴电极中的空气流量,可以得到稳定的流光电晕;空气中水蒸汽对NOx脱除效率有影响;在反应器内同时有HNO2和HNO3生成;实验工况下,反应器NOx转化率45%以上,经吸收液吸收后系统总脱氮效率可达70%.

关 键 词:电晕放电  自由基簇射  NOx脱除过程  化学吸收
文章编号:0253-2468(2004)06-1074-05
收稿时间:2003/12/12 0:00:00
修稿时间:2003年12月12

Experimental study on the removal of NOx from flue gases by corona oxidation in conjunction with chemical absorption
WEI Enzong.Experimental study on the removal of NOx from flue gases by corona oxidation in conjunction with chemical absorption[J].Acta Scientiae Circumstantiae,2004,24(6):1074-1078.
Authors:WEI Enzong
Institution:Clean Energy and Environmental Engineering Key Laboratory of Education Ministry, Zhejiang University, Hangzhou310027
Abstract:With moist air as the radical source, an experimental study was carried out for the removal of NO_x from flue gases by a DC corona discharge activated radical shower in conjunction with alkali solution (25% by weight of NaOH in water) scrubbing. The results of the study showed that a steady streamer corona could be obtained by adjusting the flow rate of the moist air fed into the nozzle electrode; the vapor in the moist air exerted an influence on the efficiency of NO_x removal; both HNO_2 and HNO_3 were simultaneously generated in the reactor with NO_x conversion rate being higher than 45%, and the overall efficiency of NO_x removal in the system can reach 70% after alkali solution scrubbing under the experimental conditions.
Keywords:corona discharge  radical shower  NO_x removal process  chemical absorption
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