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黑碳仪测量气溶胶吸收系数的校正算法和影响因素研究进展
引用本文:蔡园青,徐学哲,周家成,刘芊芊,赵卫雄,方波,王朔,张为俊.黑碳仪测量气溶胶吸收系数的校正算法和影响因素研究进展[J].中国环境科学,2021,41(9):4026-4035.
作者姓名:蔡园青  徐学哲  周家成  刘芊芊  赵卫雄  方波  王朔  张为俊
作者单位:1. 安徽大学物质科学与信息技术研究院, 安徽 合肥 230601;2. 中国科学院合肥物质科学研究院, 安徽光学精密机械研究所, 安徽 合肥 230031;3. 中国科学技术大学, 安徽 合肥 230026
基金项目:国家自然科学基金(41905118,42022051);中国科学院科研仪器设备研制项目(YJKYYQ20180049);合肥研究院院长基金(BJPY2019B02,YZJJ2019QN3);安徽省自然科学基金(1908085QD157)
摘    要:黑碳仪作为常用的吸收系数测量方法之一,广泛应用于气溶胶光吸收特性的实验室和外场观测研究.然而,受测量方法的限制,吸收系数测量的准确性受到颗粒物负载效应,以及滤膜和颗粒物的多重散射效应的影响.本文综述了黑碳仪的测量原理及现有校正算法,探究了其吸收系数测量的影响因素,分析了黑碳气溶胶的混合状态对其吸收系数测量偏差(Cref’)的影响,探讨了Cref’与气溶胶单次散射反照率(SSA)的关系以及Cref’的波长依赖关系,并提出了今后相关研究的建议.

关 键 词:黑碳仪  吸收系数  校正算法  测量偏差  
收稿时间:2021-02-22

Research progress of correction algorithm and influence factors for aerosol absorption coefficient from aethalometer measurement
CAI Yuan-qing,XU Xue-zhe,ZHOU Jia-cheng,LIU Qian-qian,ZHAO Wei-xiong,FANG Bo,WANG Shuo,ZHANG Wei-jun.Research progress of correction algorithm and influence factors for aerosol absorption coefficient from aethalometer measurement[J].China Environmental Science,2021,41(9):4026-4035.
Authors:CAI Yuan-qing  XU Xue-zhe  ZHOU Jia-cheng  LIU Qian-qian  ZHAO Wei-xiong  FANG Bo  WANG Shuo  ZHANG Wei-jun
Institution:1. Institute of Physical Science and Information Technology, Anhui University, Hefei 230601, China;2. Anhui Institute of Optics and Fine Mechanics, Hefei Institute of Physical Science, Chinese Academy of Sciences, Hefei 230031, China;3. University of Science and Technology of China, Hefei 230026, China
Abstract:As one of the commonly used techniques for aerosol absorption coefficient measurement, Aethalometer is widely used to investigate aerosol light absorption properties in laboratory and field experiments. However, owing to the constraint of filter-based method, the accuracy of the absorption coefficient measurement is affected by the filter-loading effect, and by the multiple-scattering effects caused by the filter fibers and aerosol particles. The instrument methodology and the developed correction algorithms of Aethalometer were reviewed. The influence factors for absorption coefficient measurement were explored. The influence of mixing state of black carbon (BC) on Aethalometer measurement deviation (Cref') of absorption coefficient were analyzed. The relationship between Cref' and aerosol single scattering albedo (SSA), and the wavelength-dependent relationship of Cref' were discussed. Furthermore, some suggestions for the future research were proposed.
Keywords:aethalometer  absorption coefficient  correction algorithm  measurement deviation  
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