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珠三角地区利用PM2.5反演气溶胶数浓度谱方法
引用本文:李菲,谭浩波,邓雪娇,邹宇,刘礼,蔡明甫,张芷言,周声圳.珠三角地区利用PM2.5反演气溶胶数浓度谱方法[J].环境科学,2019,40(2):525-531.
作者姓名:李菲  谭浩波  邓雪娇  邹宇  刘礼  蔡明甫  张芷言  周声圳
作者单位:中山大学大气科学学院, 广州 510275;中国气象局广州热带海洋气象研究所, 广州 510640;广东省生态气象中心,广州,510640;中国气象局广州热带海洋气象研究所,广州,510640;中山大学大气科学学院,广州,510275
基金项目:国家重点研发计划项目(2016YFC0202000);广东省自然科学基金项目(2014A030313788);国家自然科学基金青年科学基金项目(41405133);广东省科技计划重点项目(2010A030200012);广东省气象局科技创新团队计划项目(201103)
摘    要:大气气溶胶数浓度谱分布(PNSD)对于大气辐射和光学计算至关重要,利用目前普遍观测的气溶胶质量浓度(PM_(2.5))来反演计算PNSD,能有效补充PNSD观测的不足,对于需要PNSD信息的研究工作如大气能见度计算等有重要的实用价值.本文利用2014年11月~2015年1月在广州城市站进行同期连续观测的干气溶胶粒子的PM_(2.5)、PNSD数据进行客观分析,建立了一种使用PM_(2.5)反演PNSD的方法,并评估了该方法的适用性.结果表明该反演算法具有较好地适用性和稳定性,对于积聚模态的PNSD反演效果较好,但对于PM_(2.5)高浓度的反演结果差异较大.该反演方法将为珠三角地区的大气能见度计算和应用提供有利的依据和支撑.

关 键 词:气溶胶质量浓度  气溶胶数浓度谱分布  气溶胶体积分数谱分布  能见度  珠三角
收稿时间:2018/7/4 0:00:00
修稿时间:2018/9/12 0:00:00

A Method of Aerosol Particle Number Size Distribution Inversed by PM2.5 Mass Concentration in PRD
LI Fei,TAN Hao-bo,DENG Xue-jiao,ZOU Yu,LIU Li,CAI Ming-fu,ZHANG Zhi-yan and ZHOU Sheng-zhen.A Method of Aerosol Particle Number Size Distribution Inversed by PM2.5 Mass Concentration in PRD[J].Chinese Journal of Environmental Science,2019,40(2):525-531.
Authors:LI Fei  TAN Hao-bo  DENG Xue-jiao  ZOU Yu  LIU Li  CAI Ming-fu  ZHANG Zhi-yan and ZHOU Sheng-zhen
Institution:School of Atmospheric Science, Sun Yat-sen University, Guangzhou 510275, China;Institute of Tropical and Marine Meteorology, China Meteorological Administration, Guangzhou 510640, China,Guangdong Ecological Meteorological Center, Guangzhou 510640, China,Institute of Tropical and Marine Meteorology, China Meteorological Administration, Guangzhou 510640, China,Institute of Tropical and Marine Meteorology, China Meteorological Administration, Guangzhou 510640, China,School of Atmospheric Science, Sun Yat-sen University, Guangzhou 510275, China;Institute of Tropical and Marine Meteorology, China Meteorological Administration, Guangzhou 510640, China,School of Atmospheric Science, Sun Yat-sen University, Guangzhou 510275, China,Institute of Tropical and Marine Meteorology, China Meteorological Administration, Guangzhou 510640, China and School of Atmospheric Science, Sun Yat-sen University, Guangzhou 510275, China
Abstract:The aerosol particle number size distribution(PNSD) is of great importance in calculating atmospheric radiation and optics. It can effectively supplement the inadequate observation of PNSD using the widely known aerosol mass concentration (PM2.5) measurement to invert PNSD. It would be valuable for research that needs PNSD data, like atmospheric visibility calculation. This paper created a PNSD inversed method based on the statistics and parameterization of the dry aerosol PM2.5 and PNSD dataset from the Guangzhou urban site''s simultaneous measurements from November 2014 to January 2015. The inversed results appeared good in the accumulation mode, whereas more differences showed with higher PM2.5 loading. The applicability and stability of this method makes it preferable. It would provide advanced technical support for the visibility calculation and application in PRD.
Keywords:aerosol mass concentration  aerosol particle number size distribution  aerosol particle volume size distribution  visibility  Pearl River Delta
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