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Spatial variations of aluminum species in drinking water supplies in Xi’anstudied applying geographic information system
引用本文:Wendong Wang,Hua Li,Xiaochang Wang,Yongjun Liu. Spatial variations of aluminum species in drinking water supplies in Xi’anstudied applying geographic information system[J]. 环境科学学报(英文版), 2010, 22(4): 519-525. DOI: 10.1016/S1001-0742(09)60136-4
作者姓名:Wendong Wang  Hua Li  Xiaochang Wang  Yongjun Liu
作者单位:School of Environmental and Municipal Engineering, Xi’an University of Architecture and Technology, Xi’an 710055, China.E-mail: wwd@xauat.edu.cn,School of Environmental and Municipal Engineering, Xi’an University of Architecture and Technology, Xi’an 710055, China.,School of Environmental and Municipal Engineering, Xi’an University of Architecture and Technology, Xi’an 710055, China. and School of Environmental and Municipal Engineering, Xi’an University of Architecture and Technology, Xi’an 710055, China.
基金项目:This work was supported by the National Natural ScienceFoundation of China (No. 50838005), the ChangjiangScholars and Innovative Research Team in University (No.IRT0853) and the Nature Science Fundation of Shaanxi(No. 2009JQ7001). Authors express their thanks to DejunKang, Li Luo, Zaiji Yu, Zhao Yang, Xiaopeng Qiu, and XinJin for their help in sampling process.
摘    要:This article aimed to investigate the variation of aluminum species and the effects of coagulant type and water quality on aluminum speciation in drinking water.Statistical analysis showed that the concentration of total aluminum(AlT) of drinking water in Xi'an ranged from 0.051 to 0.417 mg/L and the concentration of AlT in about 24.7% studied samples was higher than the currently recommended value(0.2 mg/L).The areas fed by surface water plants had a larger portion(39.4%) of samples over the recommended value.In drinking water treated by alum coagulant,the average concentration of monomeric aluminum(Ala) was higher than that in water treated by poly aluminum chlorine(PACl) and poly aluminum ferric chloride(PAFC).The average concentrations of polynuclear aluminum(Alb) and colloidal/suspended aluminum(Alc) in the drinking water treated by alum were lower than those in water treated by PACl and PAFC.There was a notable decrease in AlT along with the delivery pipeline away from the plants,with an average decline of about 36 μg/(L·km).Besides coagulant type,water quality also could afflect aluminum speciation.In drinking water without orthophosphate,the concentrations of Ala and AlT were positively correlated with pH;while,in drinking water with orthophosphate,the concentrations of Ala and AlT were negatively correlated with pH.The addition of orthophosphate salts in the drinking water treatment process would be an effective method for aluminum control in pH range 6.5-8.2.

关 键 词:聚合氯化铝铁  饮用水  地理信息系统  水运  空间变化  西安  平均浓度  物种
收稿时间:2009-06-07
修稿时间:2009-08-18

Spatial variations of aluminum species in drinking water supplies in Xi'an studied applying geographic information system
Wendong Wang,Hua Li,Xiaochang Wang and Yongjun Liu. Spatial variations of aluminum species in drinking water supplies in Xi'an studied applying geographic information system[J]. Journal of environmental sciences (China), 2010, 22(4): 519-525. DOI: 10.1016/S1001-0742(09)60136-4
Authors:Wendong Wang  Hua Li  Xiaochang Wang  Yongjun Liu
Affiliation:School of Environmental and Municipal Engineering, Xi''an University of Architecture and Technology, Xi''an 710055, China
Abstract:This article aimed to investigate the variation of aluminum species and the effects of coagulant type and water quality on aluminum speciation in drinking water. Statistical analysis showed that the concentration of total aluminum (Al_T) of drinking water in Xi'an ranged from 0.051 to 0.417 mg/L and the concentration of Al_T in about 24.7% studied samples was higher than the currently recommended value (0.2 mg/L). The areas fed by surface water plants had a larger portion (39.4%) of samples over the recommended value. In drinking water treated by alum coagulant, the average concentration of monomeric aluminum (Al_a) was higher than that in water treated by poly aluminum chlorine (PACl) and poly aluminum ferric chloride (PAFC). The average concentrations of polynuclear aluminum (Al_b) and colloidal/suspended aluminum (Al_c) in the drinking water treated by alum were lower than those in water treated by PACl and PAFC. There was a notable decrease in Al_T along with the delivery pipeline away from the plants, with an average decline of about 36 (μg/(L·km). Besides coagulant type, water quality also could affect aluminum speciation. In drinking water without orthophosphate, the concentrations of Al_a and Al_T were positively correlated with pH; while, in drinking water with orthophosphate, the concentrations of Al_a and Al_T were negatively correlated with pH. The addition of orthophosphate salts in the drinking water treatment process would be an effective method for aluminum control in pH range 6.5-8.2.
Keywords:aluminum species   geographic information system   orthophosphate   water quality
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