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烟台市环境受体PM2.5四季污染特征与来源解析
引用本文:刘童,王晓军,陈倩,温杰,黄渤,朱红霞,田瑛泽,冯银厂.烟台市环境受体PM2.5四季污染特征与来源解析[J].环境科学,2019,40(3):1082-1090.
作者姓名:刘童  王晓军  陈倩  温杰  黄渤  朱红霞  田瑛泽  冯银厂
作者单位:南开大学环境科学与工程学院,国家环境保护城市空气颗粒物污染防治重点实验室,天津300071;烟台市环境监控中心,烟台,264003;广州禾信仪器股份有限公司,广州,510530;中国环境监测总站,北京,100012
基金项目:中央高校基本科研业务费专项
摘    要:于2016~2017年四季在烟台市3个点位采集了PM_(2.5)样品,分析了其质量浓度和化学组分特征.利用CMB模型对受体进行解析,并利用后向轨迹和PSCF对传输气流和潜在源区进行了分析.结果表明,烟台市监测点位冬季、春季、夏季和秋季的PM_(2.5)平均质量浓度分别为(89. 45±56. 80)、(76. 78±28. 44)、(32. 65±17. 92)和(57. 32±24. 60)μg·m~(-3). PM_(2.5)浓度表现出明显的季节变化特征(P 0. 01).全年PM_(2.5)各源类分担率大小依次为:二次硝酸盐源(20. 3%)城市扬尘源(15. 7%)机动车排放源(14. 9%)燃煤源(13. 8%)二次硫酸盐源(12. 8%) SOC(6. 1%)建筑水泥尘源(5. 5%)海盐源(2. 9%),可以看到烟台市以二次源、扬尘、机动车排放源和燃煤源为主要污染源.春季硝酸盐源和城市扬尘源是重要贡献源类,夏季硫酸盐源贡献突出,燃煤源在秋冬季占比突出.烟台市气流输送和潜在源区也呈现出明显的季节变化:冬季主要受烟台市短距离输送的影响;夏季主要受烟台东部沿海和本地的影响;春秋季主要受山东东北部和东部沿海地区的区域传输和烟台市本地源的影响.

关 键 词:季节差异  化学质量平衡模型(CMB)  潜在源贡献因子(PSCF)  PM2.5  烟台市
收稿时间:2018/7/29 0:00:00
修稿时间:2018/9/13 0:00:00

Pollution Characteristics and Source Apportionment of Ambient PM2.5 During Four Seasons in Yantai City
LIU Tong,WANG Xiao-jun,CHEN Qian,WEN Jie,HUANG Bo,ZHU Hong-xi,TIAN Ying-ze and FENG Yin-chang.Pollution Characteristics and Source Apportionment of Ambient PM2.5 During Four Seasons in Yantai City[J].Chinese Journal of Environmental Science,2019,40(3):1082-1090.
Authors:LIU Tong  WANG Xiao-jun  CHEN Qian  WEN Jie  HUANG Bo  ZHU Hong-xi  TIAN Ying-ze and FENG Yin-chang
Institution:State Environmental Protection Key Laboratory of Urban Ambient Air Particulate Matter Pollution Prevention and Control, College of Environmental Science and Engineering, Nankai University, Tianjin 300071, China,Yantai Environmental Monitoring Center, Yantai 264003, China,Yantai Environmental Monitoring Center, Yantai 264003, China,State Environmental Protection Key Laboratory of Urban Ambient Air Particulate Matter Pollution Prevention and Control, College of Environmental Science and Engineering, Nankai University, Tianjin 300071, China,Guangzhou Hexin Instrument Company Limited, Guangzhou 510530, China,China Environmental Monitoring Station, Beijing 100012, China,State Environmental Protection Key Laboratory of Urban Ambient Air Particulate Matter Pollution Prevention and Control, College of Environmental Science and Engineering, Nankai University, Tianjin 300071, China and State Environmental Protection Key Laboratory of Urban Ambient Air Particulate Matter Pollution Prevention and Control, College of Environmental Science and Engineering, Nankai University, Tianjin 300071, China
Abstract:
Keywords:seasonal variation  chemical mass balance (CMB) model  potential source contribution function (PSCF)  PM2  5  Yantai City
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