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On the horizontal homogeneity of mass-related aerosol properties
Authors:Lammel G  Brüggemann E  Müller K  Röhrl A
Institution:(1) Max Planck Institute for Meteorology, Hamburg, Germany;(2) Institute for Tropospheric Research, Leipzig, Germany;(3) Institute for Inorganic and Applied Chemistry, University of Hamburg, Hamburg, Germany
Abstract:We studied the mass-related aerosol properties, simultaneously attwo sites at the urban roof top level in the same city. Nosystematic influence of the wind vector on the difference in theaerosol concentrations between the two locations could be found.These results are compared with results from a second, similarexperiment over a larger distance including one urban and onerural site. Surprisingly, we could not detect a tendency whichwould indicate that sampling air at distance in the order of 1 kmwould be less affected by the heterogeneity than samplingdistanced in the order of 10 km apart. On the contrary, theresults suggest that mass-related properties at two sites in thesame city are not necessarily more similar than at an urban and arural site outside the city. These results stress the limitedhorizontal homogeneity of urban atmospheric aerosol. As aconclusion it is suggested that single-site measurements of mass-related aerosol properties should be considered to berepresentative for an area smaller than 1 km2 on size.
Keywords:atmospheric aerosols  horizontal homogeneity  urbanaerosol  PM10
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