Variations in Environmental Tritium Dose Estimates Due to Meteorological Data Averaging and Uncertainties in Pathway Model Parameters

The large amounts of tritium produced at the Savannah River Site (SRS) coupled with the current dose reconstruction study at the facility emphasize the importance of ensuring accurate and efficient prediction of tritium doses to the public. Presently, dose estimates to the general population in the site vicinity are calculated annually using a five year meteorological database. Determining whether detailed monthly dose estimates are necessary or whether annual averaged data is sufficient offers the potential for more efficient dose prediction. In this study, off site collective committed doses and maximum individual doses due to atmospheric tritium releases were calculated according to the methods outlined in the U.S. Nuclear Regulatory Commission's Regulatory Guide 1.109 and compared using monthly versus five-year meteorological data and source terms. Site-specific variables not currently utilized at SRS for annual dose estimates also have been included. In addition, the range of predicted doses, based on the distribution in model parameters given in the literature, were estimated. Finally, a sensitivity analysis was performed in order to determine the influence of model inputs on dose estimates. Results corroborate previous studies by indicating that the primary contributor to infant tritium dose is the ingestion of milk, while for all other age groups, the most important pathway is the ingestion of vegetation. These relative pathway contributions remain constant throughout the year for infants; for children, teenagers, and adults, however, inhalation and absorption of tritium through the skin increases in relative importance in the months of June to September. It was found that the model utilized was most sensitive to dose factors, the ratio of the specific activity of tritium oxide in vegetation to the specific activity of atmospheric tritium oxide, and breathing rates. Most importantly, it was found that over a five-year period, the use of averaged meteorological data results in total individual doses that are only 2 to 6% higher than doses determined monthly, depending on the pathway of interest.