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WRF/Chem simulated springtime impact of rising Asian emissions on air quality over the U.S.
Authors:Yongxin Zhang  Seth C Olsen  Manvendra K Dubey
Institution:1. State Key Joint Laboratory of Environmental Simulation & Pollution Control, School of Environment, Beijing Normal University, Beijing 100875, China;2. Center for Atmospheric Environmental Studies, Beijing Normal University, Beijing 100875, China;3. State Key Laboratory of Operation and Control of Renewable Energy & Storage Systems, China Electric Power Research Institute, Beijing 100192, China;4. Department of Air Pollution Control, Beijing Municipal Institute of Labour Protection, Beijing 100054, China;5. Wuhan Municipal Institute of Environmental Protection Science, Wuhan 430015, China;6. National Engineering Research Center of Urban Environmental Pollution Control, Beijing Municipal Research Institute of Environmental Protection, Beijing 100037, China
Abstract:This paper examines the impact of tripled anthropogenic emissions from China and India over the base level (gaseous species and carbonaceous aerosols for 2000) on air quality over the U.S. using the WRF/Chem (Weather Research and Forecasting – Chemistry) model at 1° resolution. WRF/Chem is a state-of-the-science, fully coupled chemistry and meteorology system suitable for simulating the transport and dispersion of pollutants and their impacts. The analyses in this work were focused on MAM (March, April and May). The simulations indicate an extensive area of elevated pollutant concentrations spanning from the Arabian Sea to the Northern Pacific and to the Northern Atlantic. MAM mean contributions from the tripled Asian emissions over the U.S. are found to be: 6–12 ppbv for CO, 1.0–2.5 ppbv for O3, and 0.6–1.6 μg m?3 for PM2.5 on a daily basis.
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