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北京城区大气干沉降的水溶性离子特征
引用本文:蔡阳阳,杨复沫,贺克斌,马永亮,奥田知明,田中茂.北京城区大气干沉降的水溶性离子特征[J].中国环境科学,2011,31(7):1071-1076.
作者姓名:蔡阳阳  杨复沫  贺克斌  马永亮  奥田知明  田中茂
作者单位:1. 中国科学院研究生院地球科学学院,计算地球动力学重点实验室,北京 100049
2. 清华大学环境学院,北京,100084
3. 庆应大学科学与技术学院,日本横滨 223-8522
基金项目:清华大学-日本庆应大学3E研究国际合作项目
摘    要:为了解北京城区大气干沉降中水溶性离子的化学组成与时间变化特征,连续进行了4年多的干沉降采样与分析.结果表明,在222个有效干沉降样品中,存在不同程度的阴离子缺失. SO42-与Ca2+分别是含量最丰富的阴、阳离子组分,其次是NO3-和NH4+. SO42-、NO3-和NH4+呈现相似的季节变化特征,即其浓度在夏季最高,冬季最低. 干沉降基本呈中性,其pH值月变化幅度小,但季节变化明显,夏季低而春季高.

关 键 词:干沉降  水溶性离子  化学组成  季节变化  北京城区  
收稿时间:2010-12-29;

Characteristics of water-soluble ions in dry deposition in urban Beijing
CAI Yang-yang,YANG Fu-mo,HE Ke-bin,MA Yong-liang,Tomoaki Okuda,Shigeru Tanaka.Characteristics of water-soluble ions in dry deposition in urban Beijing[J].China Environmental Science,2011,31(7):1071-1076.
Authors:CAI Yang-yang  YANG Fu-mo  HE Ke-bin  MA Yong-liang  Tomoaki Okuda  Shigeru Tanaka
Institution:CAI Yang-yang1,YANG Fu-mo1,HE Ke-bin2,MA Yong-liang2,Tomoaki Okuda3,Shigeru Tanaka3(1.Key Laboratory of Computational Geodynamics,College of Earth Science,Graduate University of Chinese Academy of Sciences,Beijing 100049,China,2.School of Environment,Tsinghua University,Beijing 100084,3.Faculty of Science and Technology,Keio University,Yokohama 223-8522,Japan)
Abstract:To understand the chemical composition and temporal variations of precipitation in Beijing, one-week integrated dry deposition samples were collected for more than four years. Among 222 dry deposition samples, there existed more or less anion deficits. SO42- and Ca2+ were the most abundant anion and cation, followed by NO3- and NH4+, respectively. SO42-、NO3- and NH4+ exhibited similar seasonal pattern, with higher and lower concentrations occurring in summer and winter, respectively. Dry deposition samples usually appeared neutral, with narrow variations in their monthly averages but an evident seasonal pattern, i.e., lower level in summer and higher level in spring.
Keywords:dry deposition  water-soluble ions  chemical composition  seasonal trend  urban Beijing  
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