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氧化石墨烯强化厌氧氨氧化菌的脱氮性能
引用本文:黄硕,于德爽,陈光辉,王晓霞,吕廷廷,唐鹏,刘诚诚.氧化石墨烯强化厌氧氨氧化菌的脱氮性能[J].中国环境科学,2019,39(5):1945-1953.
作者姓名:黄硕  于德爽  陈光辉  王晓霞  吕廷廷  唐鹏  刘诚诚
作者单位:1. 青岛大学环境科学与工程学院, 山东 青岛 266071; 2. 北京工业大学国家工程实验室, 北京市污水脱氮除磷处理与过程控制工程技术研究中心, 北京 100124
基金项目:中国博士后科学基金资助项目(2018M630053);北京市博士后科学基金资助项目(2018-ZZ-012);朝阳区博士后资助项目(2018ZZ-01-24);山东省自然科学基金资助项目(ZR2017BEE076);国家自然科学基金资助项目(51478229)
摘    要:采用氧化石墨烯(GO)增强厌氧氨氧化菌的脱氮性能.通过批次试验观察GO对厌氧氨氧化菌的影响,结果表明:当GO浓度为0.15g/L时,厌氧氨氧化菌脱氮性能最好,总氮去除率比无GO的空白组提高18.6%;当GO剂量达到0.2g/L时,厌氧氨氧化菌活性受到抑制,总氮去除率比空白组降低了26.0%.通过对照实验研究GO对厌氧氨氧化菌脱氮性能的长期影响,结果表明:添加GO的R2反应器在每个基质浓度阶段的平均总氮去除率分别为85.3%,83.2%,81.1%,80.8%,均高于未添加GO的R1反应器.对R2反应器周期内脱氮性能进行动力学分析发现,修正的Boltzmann模型和修正的Gompertz模型比修正的Logistic模型更适合描述GO作用下周期内基质去除特性,并且通过模型得到了周期内任意t时刻下的出水总氮浓度和总氮去除率预测公式.

关 键 词:厌氧氨氧化  氧化石墨烯  脱氮效能  总氮去除率  动力学  
收稿时间:2018-09-30

Improvement of the activity of anammox bacteria using graphene oxide
HUANG Shuo,YU De-shuang,CHEN Guang-hui,WANG Xiao-xia,LU Ting-ting,TANG Peng,LIU Cheng-cheng.Improvement of the activity of anammox bacteria using graphene oxide[J].China Environmental Science,2019,39(5):1945-1953.
Authors:HUANG Shuo  YU De-shuang  CHEN Guang-hui  WANG Xiao-xia  LU Ting-ting  TANG Peng  LIU Cheng-cheng
Institution:1. School of Environmental Science and Engineering, Qingdao University, Qingdao 266071, China; 2. National Engineering Laboratory for Advanced Municipal Wastewater Treatment and Reuse Technology, Engineering Research Center of Beijing, Beijing University of Technology, Beijing 100124, China
Abstract:Graphene oxide (GO) was used to enhance denitrification performance of anammox bacteria. Batch experiments were executed to explore effect of GO on anammox bacteria. The results showed anammox bacteria had the best nitrogen removal performance when the concentration of GO was 0.15g/L, and the total nitrogen removal rate was 18.6% higher than blank group. When GO concentration reached 0.2g/L, anammox bacteria activity was inhibited, and the total nitrogen removal rate was reduced by 26.0% compare with the blank group. A long-term experiment was operated to ident the effect of GO on anammox bacteria by set control group. The results showed the average total nitrogen removal rate of the R2 reactor with GO was 85.3%, 83.2% and 81.1% and 80.8%, respectively, which was higher than the R1reactor without GO. The kinetics characteristics of nitrogen removal in a single cycle of the R2 reactor were evaluated. The modified Boltzmann and Gompertz model were found to be the appropriate models to describe the denitrification performance of the R2 reactor in a single cycle. Moreover, the formula to predict the total nitrogen effluent concentration and removal rate at any time in the cycle was obtained.
Keywords:anammox  graphene oxide  nitrogen removal efficiency  total nitrogen removal efficiency  kinetic  
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