| 三峡库首秭归地区大气降水硫同位素组成及示踪研究 |
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| 引用本文： | 吴起鑫,韩贵琳.三峡库首秭归地区大气降水硫同位素组成及示踪研究[J].环境科学,2012,33(7):2145-2150. |
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| 作者姓名： | 吴起鑫 韩贵琳 |
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| 作者单位： | 中国科学院地球化学研究所环境地球化学国家重点实验室,贵阳 550002;中国科学院研究生院地球科学学院,北京 100049;中国科学院地球化学研究所环境地球化学国家重点实验室,贵阳 550002 |
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| 基金项目： | 中国科学院知识创新工程重要方向项目(KZCX2-YW-QN109);国家自然科学基金项目(40973088,41021062) |
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| 摘 要： | 2009年6月～2010年7月对三峡库首秭归地区大气降水SO24-含量和硫同位素组成特征进行了连续1 a的研究.结果表明,秭归地区降水SO24-浓度在31.4～668.1μmol.L-1之间,加权平均浓度为161.9μmol.L-1;降水SO24-硫同位素值δ34S在-2.14‰～6.07‰之间,平均值为2.06‰±1.97‰.SO24-含量季节变化特征明显,夏秋季节低,冬春季节高;而δ34S值则冬季偏正,而其他3个季节都相对偏负.对硫同位素值分析表明,生物来源硫可能对当地大气降水酸度有一定的贡献,且在夏秋季节尤为明显.
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| 关 键 词： | 三峡水库 大气降水 硫同位素 生物来源硫 秭归 |
| 收稿时间： | 9/1/2011 12:00:00 AM |
| 修稿时间： | 2011/10/28 0:00:00 |
Isotopic Composition and Isotope Tracing of Sulfur in Atmospheric Precipitation at the Head Area of the Three Gorges Reservoir, China |
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| WU Qi-xin and HAN Gui-lin.Isotopic Composition and Isotope Tracing of Sulfur in Atmospheric Precipitation at the Head Area of the Three Gorges Reservoir, China[J].Chinese Journal of Environmental Science,2012,33(7):2145-2150. |
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| Authors: | WU Qi-xin and HAN Gui-lin |
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| Institution: | State Key Laboratory of Environmental Geochemistry, Institute of Geochemistry, Chinese Academy of Sciences, Guiyang 550002, China;College of Earth Science, Graduate University of Chinese Academy of Sciences, Beijing 100049, China;State Key Laboratory of Environmental Geochemistry, Institute of Geochemistry, Chinese Academy of Sciences, Guiyang 550002, China |
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| Abstract: | Rainwater samples were collected in the head area of the Three Gorges Reservoir from June 2009 to July 2010.The SO2-4 content and the characteristics of sulfur isotopic composition were determined.The results showed that the concentrations of SO2-4 ranged from 31.4-668.1 μmol·L-1 with a weighted average of 161.9 μmol·L-1,whereas the variation of δ34S values for SO2-4 ranged from-2.14‰ to 6.07‰ with an annual average of 2.06‰±1.97‰.Significant seasonal variations were found in the SO2-4 content,which were higher in winter and spring and lower in summer and autumn.The δ34S values for SO2-4 measured in winter were much higher than those in the other seasons.Analysis of the δ34S values showed that the biogenic sulfur might have significant contribution to the acidity of rainwater,especially in summer and autumn. |
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| Keywords: | the Three Gorges Reservoir rainwater sulfur isotope biogenic sulfur Zigui |
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