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生物滴滤塔净化甲基叔丁基醚废气的研究
引用本文:褚其英,姚露露,吕雄标,叶杰旭,叶虹霓,潘梁柱,陈建孟,陈东之.生物滴滤塔净化甲基叔丁基醚废气的研究[J].环境科学,2018,39(2):633-639.
作者姓名:褚其英  姚露露  吕雄标  叶杰旭  叶虹霓  潘梁柱  陈建孟  陈东之
作者单位:浙江工业大学环境学院, 杭州 310032,浙江工业大学环境学院, 杭州 310032,浙江菲尔特环保工程有限公司, 杭州 310014,浙江工业大学环境学院, 杭州 310032,浙江工业大学环境学院, 杭州 310032,浙江工业大学环境学院, 杭州 310032,浙江工业大学环境学院, 杭州 310032,浙江工业大学环境学院, 杭州 310032
基金项目:国家自然科学基金项目(21477116);浙江省自然科学基金项目(LY17E080019)
摘    要:应用生物滴滤塔处理甲基叔丁基醚废气,研究其挂膜启动及稳定运行阶段的降解性能,并考察了稳定期该系统的生物群落结构.结果表明,生物滴滤塔在停留时间为60 s,进气质量浓度为100 mg·m~(-3)的条件下,运行23 d后完成挂膜,填料上的生物量明显增加,去除率可维持在70%以上.反应器稳定运行时,去除负荷可达13.47 g·(m3·h)~(-1),矿化率可达68%;用Haldane模型拟合生物滴滤塔中去除负荷的变化趋势,获得理论ECmax为21.03 g·(m3·h)~(-1),KS为0.16 g·m~(-3),KI为0.99g·m~(-3).运用高通量测序技术分析生物膜中的微生物群落结构,发现其中优势菌属为Methylibium sp.和Blastocatella sp.,分别占11.33%和9.95%.

关 键 词:生物滴滤塔  甲基叔丁基醚  去除负荷  动力学
收稿时间:2017/3/8 0:00:00
修稿时间:2017/6/3 0:00:00

Treatment of the Waste Gas Containing Methyl tert-Butyl Ether via a Biotrickling Filter
CHU Qi-ying,YAO Lu-lu,L&#; Xiong-biao,YE Jie-xu,YE Hong-ni,PAN Liang-zhu,CHEN Jian-meng and CHEN Dong-zhi.Treatment of the Waste Gas Containing Methyl tert-Butyl Ether via a Biotrickling Filter[J].Chinese Journal of Environmental Science,2018,39(2):633-639.
Authors:CHU Qi-ying  YAO Lu-lu  L&#; Xiong-biao  YE Jie-xu  YE Hong-ni  PAN Liang-zhu  CHEN Jian-meng and CHEN Dong-zhi
Institution:College of Environment, Zhejiang University of Technology, Hangzhou 310032, China,College of Environment, Zhejiang University of Technology, Hangzhou 310032, China,Feierte Environmental Engineering Company Limited of Zhejiang Province, Hangzhou 310014, China,College of Environment, Zhejiang University of Technology, Hangzhou 310032, China,College of Environment, Zhejiang University of Technology, Hangzhou 310032, China,College of Environment, Zhejiang University of Technology, Hangzhou 310032, China,College of Environment, Zhejiang University of Technology, Hangzhou 310032, China and College of Environment, Zhejiang University of Technology, Hangzhou 310032, China
Abstract:The performance and microbial communities of methyl tert-butyl ether (MTBE) treatment using a biotrickling filter (BTF) that was inoculated with activated sewage sludge were investigated. The BTF successfully started up within 23 days when the inlet concentration of MTBE was 100 mg·m-3 and empty bed retention time was 60 s, with 70% removal efficiency (RE). Under steady-state conditions, an elimination capacity (EC) and a mineralization ratio of 13.47 g·(m3·h)-1 and 68% were achieved, respectively. The ECmax was 21.03 g·(m3·h)-1 according to the Haldane model, and a KS of 0.16 g·m-3 and KI of 0.99 g·m-3 were obtained. High-throughput sequencing was used to identify the community structure of the mixed microbial consortium in the BTF. The results indicated that Methylibium sp. (11.33%) and Blastocatella sp. (9.95%) were the dominant bacteria.
Keywords:biotrickling filter  methyl tert-butyl ether(MTBE)  elimination capacity  kinetic
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