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基于样方法的天津市春季道路扬尘PM2.5中水溶性离子特征及来源解析
引用本文:赵静琦,姬亚芹,张蕾,王士宝,李越洋.基于样方法的天津市春季道路扬尘PM2.5中水溶性离子特征及来源解析[J].环境科学,2018,39(5):1994-1999.
作者姓名:赵静琦  姬亚芹  张蕾  王士宝  李越洋
作者单位:南开大学环境科学与工程学院
基金项目:环境保护公益性行业科研专项(201409004);大气重污染成因与治理攻关项目(DQGG0201)
摘    要:为研究天津市道路扬尘PM_(2.5)中水溶性无机离子组分特征及其来源,于2015年4月采集天津市道路扬尘样品,利用再悬浮采样器将采集的样品悬浮到滤膜上,用离子色谱仪分析其水溶性无机离子组分,利用相关分析和比值分析及主成分法对其污染特征和来源进行探讨.结果表明,天津市8种水溶性无机离子占道路扬尘PM_(2.5)的6.13%±2.32%;不同道路类型道路扬尘PM_(2.5)中水溶性无机离子总量差异较大.相关性分析表明Na~+、K~+、Mg~(2+)和Ca~(2+)这4种离子同源性较高.NO_3~-/SO_4~(2-)比值显示固定源对天津市春季道路扬尘PM_(2.5)的影响更为显著.通过主成分分析法可知,天津市春季道路扬尘PM_(2.5)主要来源于燃煤源、移动源、生物质燃烧源和建筑施工扬尘.

关 键 词:天津市  道路扬尘  PM2.5  水溶性无机离子  来源解析
收稿时间:2017/10/13 0:00:00
修稿时间:2017/11/7 0:00:00

Characteristics and Source Apportionment of Water-soluble Inorganic Ions in Road Dust PM2.5 During Spring in Tianjin Using the Quadrat Sampling Method
ZHAO Jing-qi,JI Ya-qin,ZHANG Lei,WANG Shi-bao and LI Yue-yang.Characteristics and Source Apportionment of Water-soluble Inorganic Ions in Road Dust PM2.5 During Spring in Tianjin Using the Quadrat Sampling Method[J].Chinese Journal of Environmental Science,2018,39(5):1994-1999.
Authors:ZHAO Jing-qi  JI Ya-qin  ZHANG Lei  WANG Shi-bao and LI Yue-yang
Institution:College of Environmental Science and Engineering, Nankai University, Tianjin 300350, China,College of Environmental Science and Engineering, Nankai University, Tianjin 300350, China,College of Environmental Science and Engineering, Nankai University, Tianjin 300350, China,College of Environmental Science and Engineering, Nankai University, Tianjin 300350, China and College of Environmental Science and Engineering, Nankai University, Tianjin 300350, China
Abstract:In order to collect comprehensive information regarding the characteristics and sources of the water-soluble inorganic ions in road dust (RD) PM2.5 in Tianjin, samples of road dust were collected in April 2015 in Tianjin, and then re-suspended on filters using a NK-ZXF sampler. The concentrations of the major water-soluble inorganic ions were analyzed by ion chromatography. A correlation analysis, ratio method, and principal component analysis were used to analyze the sources of RD PM2.5. The results showed that the total water-soluble inorganic ion concentration in Tianjin accounted for 6.13%±2.32%, varying with different road types. Na+, K+, Mg2+, and Ca2+ showed high homology. NO3-/SO42- revealed that the main source of PM2.5 was mostly attributed to fixed sources. The principal component analysis showed that the main sources of RD PM2.5 in Tianjin were coal combustion, mobile sources, biomass burning, and construction dust.
Keywords:Tianjin  road dust  PM2  5  water-soluble inorganic ions  source apportionment
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