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盘锦市秋冬季节PM2.5中碳组分特征及来源解析
引用本文:张蕾,姬亚芹,张军,王士宝,李越洋,赵静琦,张伟.盘锦市秋冬季节PM2.5中碳组分特征及来源解析[J].环境科学,2018,39(7):3051-3056.
作者姓名:张蕾  姬亚芹  张军  王士宝  李越洋  赵静琦  张伟
作者单位:南开大学环境科学与工程学院国家环境保护城市空气颗粒物污染防治重点实验室;盘锦市环境保护监测站
摘    要:为研究盘锦市秋冬季节大气PM_(2.5)中碳组分的污染特征和来源,于2016年10月和2017年1月采集盘锦市3个点位PM_(2.5)样品,通过OC/EC比值法,EC示踪法以及主成分分析法对PM_(2.5)中碳组分进行污染特征分析及来源解析.结果表明,盘锦市秋冬季节PM_(2.5)浓度均超过环境空气质量标准(GB 3095-2012)二级标准,秋季OC和EC的平均浓度为10.02μg·m~(-3)和3.91μg·m~(-3),冬季为16.04μg·m~(-3)和5.62μg·m~(-3);采样期间秋冬季节OC/EC均大于2.0,说明各采样点位在秋冬季均可能存在二次污染,Spearman相关分析及线性拟合可知开发区OC与EC来源复杂,第二中学及文化公园OC和EC可能具有同源性;通过EC示踪法对SOC进行定量估算,得出秋季SOC浓度为7.21μg·m~(-3),冬季为23.07μg·m~(-3),对结果进行不确定性分析,可知秋冬季节SOC不确定性的绝对误差和相对误差均在可接受范围内;通过主成分分析得出盘锦市秋冬季节PM_(2.5)中碳组分主要来源于煤烟尘,生物质燃烧以及机动车尾气.

关 键 词:盘锦市  有机碳(OC)  元素碳(EC)  二次有机碳(SOC)  来源解析
收稿时间:2017/12/16 0:00:00
修稿时间:2018/1/8 0:00:00

Characteristics and Sources of Carbon Components in PM2.5 During Autumn and Winter in Panjin City
ZHANG Lei,JI Ya-qin,ZHANG Jun,WANG Shi-bao,LI Yue-yang,ZHAO Jing-qi and ZHANG Wei.Characteristics and Sources of Carbon Components in PM2.5 During Autumn and Winter in Panjin City[J].Chinese Journal of Environmental Science,2018,39(7):3051-3056.
Authors:ZHANG Lei  JI Ya-qin  ZHANG Jun  WANG Shi-bao  LI Yue-yang  ZHAO Jing-qi and ZHANG Wei
Institution:State Environmental Protection Key Laboratory of Urban Ambient Air Particulate Matter Pollution Prevention and Control, College of Environmental Science and Engineering, Nankai University, Tianjin 300350, China,State Environmental Protection Key Laboratory of Urban Ambient Air Particulate Matter Pollution Prevention and Control, College of Environmental Science and Engineering, Nankai University, Tianjin 300350, China,Panjin Environmental Monitoring Center, Panjin 124010, China,State Environmental Protection Key Laboratory of Urban Ambient Air Particulate Matter Pollution Prevention and Control, College of Environmental Science and Engineering, Nankai University, Tianjin 300350, China,State Environmental Protection Key Laboratory of Urban Ambient Air Particulate Matter Pollution Prevention and Control, College of Environmental Science and Engineering, Nankai University, Tianjin 300350, China,State Environmental Protection Key Laboratory of Urban Ambient Air Particulate Matter Pollution Prevention and Control, College of Environmental Science and Engineering, Nankai University, Tianjin 300350, China and State Environmental Protection Key Laboratory of Urban Ambient Air Particulate Matter Pollution Prevention and Control, College of Environmental Science and Engineering, Nankai University, Tianjin 300350, China
Abstract:
Keywords:Panjin City  organic carbon(OC)  elemental carbon(EC)  secondary organic carbon(SOC)  source apportionment
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