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典型热带林地土壤团聚体颗粒中重金属的分布特征及其环境意义
引用本文:龚仓,徐殿斗,成杭新,任雅阁,刘志明,刘应汉,刘飞,聂海峰,郑祥,马玲玲.典型热带林地土壤团聚体颗粒中重金属的分布特征及其环境意义[J].环境科学,2013,34(3):1094-1100.
作者姓名:龚仓  徐殿斗  成杭新  任雅阁  刘志明  刘应汉  刘飞  聂海峰  郑祥  马玲玲
作者单位:1. 中国科学院高能物理研究所核分析技术重点实验室,北京 100049;成都理工大学材料与化学化工学院,成都610059
2. 中国科学院高能物理研究所核分析技术重点实验室,北京,100049
3. 中国地质科学院地球物理与地球化学勘查研究所地球表层碳-汞地球化学循环重点实验室,廊坊,065000
4. 中国科学院高能物理研究所核分析技术重点实验室,北京 100049;北京化工大学化学工程学院,北京 100029
5. 北京化工大学化学工程学院,北京,100029
6. 中国人民大学环境学院,北京,100872
基金项目:中国地质调查局专项(1212011087123);国土资源部行业基金项目(200911020);国家自然科学基金项目(11075171,10905061)
摘    要:以海口、琼海和屯昌的典型热带林地土壤为研究对象,采用干筛法获得6个粒级的土壤团聚体颗粒组.用ICP-MS测定了本土和不同团聚体颗粒中重金属Cr、Ni、Cu、Zn、Cd、As和Pb的含量,并对其分布特征及对有机碳和铁的响应进行了解析.研究表明,重金属在土壤各粒径团聚体颗粒组中差异性分布,随着团聚体粒径的减小而呈现富集增大的趋势,其中Cr、Ni、Cu、Zn、Cd和Cd主要富集在粉-黏团聚体(<53μm)颗粒中;As主要赋存在53~1 000μm的颗粒组中.总体来讲,微团聚体(<250μm)对土壤重金属含量贡献为14.38%~65.04%,其中粉粒级团聚体(<53μm)的贡献为2.61%~32.01%.有机碳和铁氧化物含量随着团聚体粒径减小而升高,并与除了As及海口的Cd和Pb以外的其他重金属分布具有显著相关性.

关 键 词:重金属  团聚体颗粒组  有机碳  林地  分布特征
收稿时间:6/6/2012 12:00:00 AM
修稿时间:9/4/2012 12:00:00 AM

Distribution Characteristics and Environmental Significance of Heavy Metals in Soil Particle Size Fractions from Tropical Forests in China
GONG Cang,XU Dian-dou,CHENG Hang-xin,REN Ya-ge,LIU Zhi-ming,LIU Ying-han,LIU Fei,NIE Hai-feng,ZHENG Xiang and MA Ling-ling.Distribution Characteristics and Environmental Significance of Heavy Metals in Soil Particle Size Fractions from Tropical Forests in China[J].Chinese Journal of Environmental Science,2013,34(3):1094-1100.
Authors:GONG Cang  XU Dian-dou  CHENG Hang-xin  REN Ya-ge  LIU Zhi-ming  LIU Ying-han  LIU Fei  NIE Hai-feng  ZHENG Xiang and MA Ling-ling
Institution:Key Laboratory of Nuclear Analytical Techniques,Institute of High Energy Physics,Chinese Academy of Sciences,Beijing 100049,China;College of Materials and Chemistry and Chemical Engineering, Chengdu University of Technology,Chengdu 610059,China;Key Laboratory of Nuclear Analytical Techniques,Institute of High Energy Physics,Chinese Academy of Sciences,Beijing 100049,China;Key Laboratory of Geochemical Cycling of Carbon and Mercury in the Earth's Critical Zone, Institute of Geophysical & Geochemical Exploration,Chinese Academy of Geological Sciences,Langfang 065000,China;Key Laboratory of Nuclear Analytical Techniques,Institute of High Energy Physics,Chinese Academy of Sciences,Beijing 100049,China;College of Chemical Engineering, Beijing University of Chemical Technology,Beijing 100029,China;College of Chemical Engineering, Beijing University of Chemical Technology,Beijing 100029,China;Key Laboratory of Geochemical Cycling of Carbon and Mercury in the Earth's Critical Zone, Institute of Geophysical & Geochemical Exploration,Chinese Academy of Geological Sciences,Langfang 065000,China;Key Laboratory of Geochemical Cycling of Carbon and Mercury in the Earth's Critical Zone, Institute of Geophysical & Geochemical Exploration,Chinese Academy of Geological Sciences,Langfang 065000,China;Key Laboratory of Geochemical Cycling of Carbon and Mercury in the Earth's Critical Zone, Institute of Geophysical & Geochemical Exploration,Chinese Academy of Geological Sciences,Langfang 065000,China;School of Environment and Natural Resources,Renmin University of China,Beijing 100872,China;Key Laboratory of Nuclear Analytical Techniques,Institute of High Energy Physics,Chinese Academy of Sciences,Beijing 100049,China
Abstract:
Keywords:heavy metal  particle size fractions  organic carbon  forest soil  distribution characteristics
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