| 2011年春季沙尘天气影响下上海大气颗粒物及其化学组分的变化特征 |
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| 引用本文： | 李贵玲,周敏,陈长虹,王红丽,王倩,楼晟荣,乔利平,唐喜斌,李莉,黄海英,陈明华,黄成,张钢锋.2011年春季沙尘天气影响下上海大气颗粒物及其化学组分的变化特征[J].环境科学,2014,35(5):1644-1653. |
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| 作者姓名： | 李贵玲 周敏 陈长虹 王红丽 王倩 楼晟荣 乔利平 唐喜斌 李莉 黄海英 陈明华 黄成 张钢锋 |
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| 作者单位： | 华东理工大学资源与环境工程学院,上海 200237;上海市环境科学研究院国家环境保护城市大气复合污染成因与防治重点实验室（筹）,上海 200233;上海市环境科学研究院国家环境保护城市大气复合污染成因与防治重点实验室（筹）,上海 200233;上海市大气颗粒物污染防治重点实验室,上海 200433;上海市环境科学研究院国家环境保护城市大气复合污染成因与防治重点实验室（筹）,上海 200233;上海市大气颗粒物污染防治重点实验室,上海 200433;上海市环境科学研究院国家环境保护城市大气复合污染成因与防治重点实验室（筹）,上海 200233;上海市大气颗粒物污染防治重点实验室,上海 200433;上海市环境科学研究院国家环境保护城市大气复合污染成因与防治重点实验室（筹）,上海 200233;上海市大气颗粒物污染防治重点实验室,上海 200433;上海市环境科学研究院国家环境保护城市大气复合污染成因与防治重点实验室（筹）,上海 200233;上海市大气颗粒物污染防治重点实验室,上海 200433;上海市环境科学研究院国家环境保护城市大气复合污染成因与防治重点实验室（筹）,上海 200233;上海市大气颗粒物污染防治重点实验室,上海 200433;华东理工大学资源与环境工程学院,上海 200237;上海市环境科学研究院国家环境保护城市大气复合污染成因与防治重点实验室（筹）,上海 200233;上海市环境科学研究院国家环境保护城市大气复合污染成因与防治重点实验室（筹）,上海 200233;上海市大气颗粒物污染防治重点实验室,上海 200433;上海市环境科学研究院国家环境保护城市大气复合污染成因与防治重点实验室（筹）,上海 200233;上海市环境科学研究院国家环境保护城市大气复合污染成因与防治重点实验室（筹）,上海 200233;上海市环境科学研究院国家环境保护城市大气复合污染成因与防治重点实验室（筹）,上海 200233;上海市大气颗粒物污染防治重点实验室,上海 200433;上海市环境科学研究院国家环境保护城市大气复合污染成因与防治重点实验室（筹）,上海 200233 |
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| 基金项目： | 环境保护公益性行业科研专项（201409008，201209007，201209001）；中国科学院战略性先导科技专项（XDB020300）；上海市科委项目（11231200500）；上海市重大科技专项 （沪环科2013-03） |
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| 摘 要： | 于2011年4月28日~5月18日对上海大气中颗粒物的质量浓度及细粒子中的化学组分进行了连续观测,获得了上海受春季沙尘天气影响下大气颗粒物质量浓度和主要化学组分特征.结果表明,沙尘天气中PM10和PM2.5的质量浓度显著高于非沙尘天,最高日均浓度分别达到787.2μg·m-3和139.5μg·m-3,PM2.5/PM10的均值为(32.9±14.6)%(15.6%~85.1%);总水溶性无机离子(TWSⅡ)占PM2.5的质量分数为(27.2±19.2)%(4.8%~80.8%),二次组分SNA(SO2-4、NO-3、NH+4)占TWSⅡ的(76.9±13.9)%(41.9%~94.2%),TWSⅡ和SNA对PM2.5的贡献均小于非沙尘天,而Ca2+的含量比却有明显上升.非沙尘天测得的OC/EC值高于强沙尘天,但低于弱沙尘天.此外分析还得到,沙尘中的高矿尘粒子具有酸性缓冲作用,使得沙尘天颗粒的碱性强于沙尘发生前.非沙尘天SO2-4、NO-3主要以NH4HSO4、(NH4)2SO4和NH4NO3的形式存在,沙尘天还会与其他矿物离子结合.
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| 关 键 词： | 沙尘 颗粒物 化学组分 水溶性离子 离子形态 |
| 收稿时间： | 7/8/2013 12:00:00 AM |
| 修稿时间： | 2013/9/16 0:00:00 |
Characteristics of Particulate Matters and Its Chemical Compositions During the Dust Episodes in Shanghai in Spring, 2011 |
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| LI Gui-ling,ZHOU Min,CHEN Chang-hong,WANG Hong-li,WANG Qian,LOU Sheng-rong,QIAO Li-ping,TANG Xi-bin,LI Li,HUANG Hai-ying,CHEN Ming-hu,HUANG Cheng and ZHANG Gang-feng.Characteristics of Particulate Matters and Its Chemical Compositions During the Dust Episodes in Shanghai in Spring, 2011[J].Chinese Journal of Environmental Science,2014,35(5):1644-1653. |
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| Authors: | LI Gui-ling ZHOU Min CHEN Chang-hong WANG Hong-li WANG Qian LOU Sheng-rong QIAO Li-ping TANG Xi-bin LI Li HUANG Hai-ying CHEN Ming-hu HUANG Cheng and ZHANG Gang-feng |
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| Institution: | School of Resources and Environmental Engineering, East China University of Science and Technology, Shanghai 200237, China;State Environmental Protection Key Laboratory of the Cause and Prevention of Urban Air Pollution Complex, Shanghai Academy of Environmental Sciences, Shanghai 200233, China;State Environmental Protection Key Laboratory of the Cause and Prevention of Urban Air Pollution Complex, Shanghai Academy of Environmental Sciences, Shanghai 200233, China;Shanghai Key Laboratory of Atmospheric Particle Pollution Prevention, Shanghai 200433, China;State Environmental Protection Key Laboratory of the Cause and Prevention of Urban Air Pollution Complex, Shanghai Academy of Environmental Sciences, Shanghai 200233, China;Shanghai Key Laboratory of Atmospheric Particle Pollution Prevention, Shanghai 200433, China;State Environmental Protection Key Laboratory of the Cause and Prevention of Urban Air Pollution Complex, Shanghai Academy of Environmental Sciences, Shanghai 200233, China;Shanghai Key Laboratory of Atmospheric Particle Pollution Prevention, Shanghai 200433, China;State Environmental Protection Key Laboratory of the Cause and Prevention of Urban Air Pollution Complex, Shanghai Academy of Environmental Sciences, Shanghai 200233, China;Shanghai Key Laboratory of Atmospheric Particle Pollution Prevention, Shanghai 200433, China;State Environmental Protection Key Laboratory of the Cause and Prevention of Urban Air Pollution Complex, Shanghai Academy of Environmental Sciences, Shanghai 200233, China;Shanghai Key Laboratory of Atmospheric Particle Pollution Prevention, Shanghai 200433, China;State Environmental Protection Key Laboratory of the Cause and Prevention of Urban Air Pollution Complex, Shanghai Academy of Environmental Sciences, Shanghai 200233, China;Shanghai Key Laboratory of Atmospheric Particle Pollution Prevention, Shanghai 200433, China;School of Resources and Environmental Engineering, East China University of Science and Technology, Shanghai 200237, China;State Environmental Protection Key Laboratory of the Cause and Prevention of Urban Air Pollution Complex, Shanghai Academy of Environmental Sciences, Shanghai 200233, China;State Environmental Protection Key Laboratory of the Cause and Prevention of Urban Air Pollution Complex, Shanghai Academy of Environmental Sciences, Shanghai 200233, China;Shanghai Key Laboratory of Atmospheric Particle Pollution Prevention, Shanghai 200433, China;State Environmental Protection Key Laboratory of the Cause and Prevention of Urban Air Pollution Complex, Shanghai Academy of Environmental Sciences, Shanghai 200233, China;State Environmental Protection Key Laboratory of the Cause and Prevention of Urban Air Pollution Complex, Shanghai Academy of Environmental Sciences, Shanghai 200233, China;State Environmental Protection Key Laboratory of the Cause and Prevention of Urban Air Pollution Complex, Shanghai Academy of Environmental Sciences, Shanghai 200233, China;Shanghai Key Laboratory of Atmospheric Particle Pollution Prevention, Shanghai 200433, China;State Environmental Protection Key Laboratory of the Cause and Prevention of Urban Air Pollution Complex, Shanghai Academy of Environmental Sciences, Shanghai 200233, China |
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| Abstract: | |
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| Keywords: | dust particulate matter chemical composition water-soluble ions ionic form |
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