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生态净化系统中DOM光学特性及影响因素分析:以盐龙湖春季为例
引用本文:马睿,李璇,王莲,王家新,马卫星,丁成,吴向阳.生态净化系统中DOM光学特性及影响因素分析:以盐龙湖春季为例[J].环境科学,2019,40(4):1742-1750.
作者姓名:马睿  李璇  王莲  王家新  马卫星  丁成  吴向阳
作者单位:盐城工学院环境科学与工程学院,盐城224000;江苏大学环境与安全工程学院,镇江212013;盐城工学院环境科学与工程学院,盐城,224000;江苏大学环境与安全工程学院,镇江,212013
基金项目:国家自然科学基金项目(51608466);江苏省自然科学基金青年基金项目(BK20160438,BK20160439)
摘    要:为了探究生态净化系统中溶解性有机物(DOM)的光学特性、空间分布特征及主要影响因子.以盐龙湖生态净化系统为例,取2017、2018年春季数据进行研究.结果表明,盐龙湖春季总磷、总氮、高锰酸盐指数浓度变化范围分别为0.05~0.25、1.25~2.75、3.99~7.17 mg·L-1,出水溶解氧升高至(11.93±1.31)mg·L-1、浊度降低至(13.23±2.24)NTU,而高锰酸盐指数变化不显著.主成分分析(PCA)表明盐龙湖原水、预处理区水质与外源汇入有关;而沉水植物区和深度净化区水质依赖于内源影响.荧光指数、腐殖化指数及生物源指数分析综合发现水体中DOM主要是源于陆生植物与土壤输入,腐殖化程度较低且新生的自生源DOM较多.PARAFAC模型将DOM可分为紫外光区类富里酸(239 nm,304 nm/407 nm),可见光区类富里酸(256 nm,352 nm/439 nm),色氨酸类蛋白质(276 nm/327 nm)和胡敏酸(292 nm,395 nm/491 nm).紫外吸收指数表明盐龙湖原水、预处理单元、挺水植物区DOM光谱强度波动较大,沉水植物区、深度净化区DOM光谱强度较稳定.水质参数中对DOM光学特性有影响的因素主要是透明度、溶解氧、电导率、总氮和藻细胞数.

关 键 词:春季  溶解性有机物(DOM)  生态净化系统  光学特性  影响因素
收稿时间:2018/8/16 0:00:00
修稿时间:2018/11/5 0:00:00

Analysis of the Optical Properties and Factors Influencing DOM in an Ecological Purification System: A Case Study of Yanlong Lake in Spring
MA Rui,LI Xuan,WANG Lian,WANG Jia-xin,MA Wei-xing,DING Cheng and WU Xiang-yang.Analysis of the Optical Properties and Factors Influencing DOM in an Ecological Purification System: A Case Study of Yanlong Lake in Spring[J].Chinese Journal of Environmental Science,2019,40(4):1742-1750.
Authors:MA Rui  LI Xuan  WANG Lian  WANG Jia-xin  MA Wei-xing  DING Cheng and WU Xiang-yang
Institution:College of Environmental Science and Engineering, Yancheng Institute of Technology, Yancheng 224000, China;School of Environment and Safety Engineering, Jiangsu University, Zhenjiang 212013, China,College of Environmental Science and Engineering, Yancheng Institute of Technology, Yancheng 224000, China,College of Environmental Science and Engineering, Yancheng Institute of Technology, Yancheng 224000, China;School of Environment and Safety Engineering, Jiangsu University, Zhenjiang 212013, China,College of Environmental Science and Engineering, Yancheng Institute of Technology, Yancheng 224000, China,College of Environmental Science and Engineering, Yancheng Institute of Technology, Yancheng 224000, China,College of Environmental Science and Engineering, Yancheng Institute of Technology, Yancheng 224000, China and School of Environment and Safety Engineering, Jiangsu University, Zhenjiang 212013, China
Abstract:An investigation the optical properties and spatial distribution of dissolved organic matter (DOM) in an ecological purification system and the primary factors that affect the optical properties of the DOM was conducted. Taking the Yanlong Lake ecological purification system as an example, data from spring 2017 and 2018 were compared. The results show that the concentrations of total phosphorus and total nitrogen and the permanganate index in Yanlong Lake were 0.05-0.25, 1.25-2.75, and 3.99-7.17 mg·L-1, respectively. In addition, the dissolved oxygen in the effluent of Yanlong Lake increased to (11.93±1.31) mg·L-1, and the turbidity decreased to (13.23±2.24) NTU, while the change in the permanganate index was not significant. Principal component analysis (PCA) showed that the water quality of the Yanlong Lake raw water and water in the pre-treatment area was closely related to the inflow of exogenous sources, while the water quality in submerged plant areas and deep purification areas was dependent on endogenous effects. According to the fluorescence index, humification index, and biological source index analysis, it was found that there are new spontaneous sources of DOM in this body of water, the degree of humification is lower, and endogenous biological DOM is dominant. The PARAFAC model can be used to classify DOM into UV-fulvic acid-like components (239 nm, 304 nm/407 nm), visible light fulvic acid-like components (256 nm, 352 nm/439 nm), tryptophan-like protein (276 nm/327 nm) and humic acid (292 nm, 395 nm/491 nm). The UV absorption index indicates that the spectral intensity of DOM in the raw water, pretreatment unit, and emergent water plant area of Yanlong Lake fluctuates greatly, and the DOM spectral intensity of the submerged plant area and deep purification area is relatively stable. The factors affecting the optical properties of the DOM in terms of water quality parameters are mainly transparency, dissolved oxygen, conductivity, total nitrogen, and algae cell number.
Keywords:spring  dissolved organic matter (DOM)  ecological purification system  optical properties  influencing factor
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