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Characteristics of atmospheric particles and heavy metals in winter in Chang-Zhu-Tan city clusters, China
作者姓名:Kai Zhang  Fahe Chai  Zilong Zheng  Qing Yang  Juansheng Li  Jing Wang  Yujie Zhang
作者单位:State Key Laboratory of Environmental Criteria and Risk Assessment, Chinese Research Academy of Environmental Sciences, Beijing 100012, China;;State Key Laboratory of Environmental Criteria and Risk Assessment, Chinese Research Academy of Environmental Sciences, Beijing 100012, China;;State Key Laboratory of Environmental Criteria and Risk Assessment, Chinese Research Academy of Environmental Sciences, Beijing 100012, China;Shandong University of Science and Technology, Qingdao 266510, China;;State Key Laboratory of Environmental Criteria and Risk Assessment, Chinese Research Academy of Environmental Sciences, Beijing 100012, China;Shandong University of Science and Technology, Qingdao 266510, China;;Changsha Environmental Protection College, Changsha 410004, China;State Key Laboratory of Environmental Criteria and Risk Assessment, Chinese Research Academy of Environmental Sciences, Beijing 100012, China;;State Key Laboratory of Environmental Criteria and Risk Assessment, Chinese Research Academy of Environmental Sciences, Beijing 100012, China;
基金项目:This work was supported by the National Department Public Benefit Research Foundation (No. 201109005) and the National Natural Science Foundation of China (No. 41205093).
摘    要:To understand the pollution characteristics of atmospheric particles and heavy metals in winter in Chang-Zhu-Tan city clusters, China, total suspended particulate(TSP) and PM10samples were collected in cities of Changsha, Zhuzhou and Xiangtan from December 2011 to January 2012, and heavy metals of Cd, Pb, Cr, and As were analyzed. It shows that the average TSP concentration in Changsha, Zhuzhou and Xiangtan were(183 ± 73),(201 ± 84) and(190 ± 66) μg/m3respectively, and the average PM10 were(171 ± 82),(178 ± 65) and(179 ± 55) μg/m3respectively. The lowest TSP and PM10concentrations occurred at the background Shaping site of Changsha. The average ratio of ρ(PM10)/ρ(TSP) was 91.9%, ranging from 81.3% to 98.9%. Concerning heavy metals, in TSP samples, the concentration of Cr, As, Cd and Pb were 28.8–56.5, 18.1–76.3, 3.9–26.1 and 148.0–460.9 ng/m3, respectively, while in PM10samples, were 16.4–42.1, 15.5–67.9, 3.3–22.2 and 127.9–389.3 ng/m3, respectively. The enrichment factor of Cd was the highest, followed by Pb and As, while that of Cr was the lowest.

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Characteristics of atmospheric particles and heavy metals in winter in Chang-Zhu-Tan city clusters, China
Kai Zhang,Fahe Chai,Zilong Zheng,Qing Yang,Juansheng Li,Jing Wang,Yujie Zhang.Characteristics of atmospheric particles and heavy metals in winter in Chang-Zhu-Tan city clusters, China[J].Journal of Environmental Sciences,2014,26(1):147-153.
Authors:Kai Zhang  Fahe Chai  Zilong Zheng  Qing Yang  Juansheng Li  Jing Wang and Yujie Zhang
Institution:State Key Laboratory of Environmental Criteria and Risk Assessment, Chinese Research Academy of Environmental Sciences, Beijing 100012, China;;State Key Laboratory of Environmental Criteria and Risk Assessment, Chinese Research Academy of Environmental Sciences, Beijing 100012, China;;State Key Laboratory of Environmental Criteria and Risk Assessment, Chinese Research Academy of Environmental Sciences, Beijing 100012, China;Shandong University of Science and Technology, Qingdao 266510, China;;State Key Laboratory of Environmental Criteria and Risk Assessment, Chinese Research Academy of Environmental Sciences, Beijing 100012, China;Shandong University of Science and Technology, Qingdao 266510, China;;Changsha Environmental Protection College, Changsha 410004, China;State Key Laboratory of Environmental Criteria and Risk Assessment, Chinese Research Academy of Environmental Sciences, Beijing 100012, China;;State Key Laboratory of Environmental Criteria and Risk Assessment, Chinese Research Academy of Environmental Sciences, Beijing 100012, China;
Abstract:To understand the pollution characteristics of atmospheric particles and heavy metals in winter in Chang-Zhu-Tan city clusters, China, total suspended particulate (TSP) and PM10 samples were collected in cities of Changsha, Zhuzhou and Xiangtan from December 2011 to January 2012, and heavy metals of Cd, Pb, Cr, and As were analyzed. It shows that the average TSP concentration in Changsha, Zhuzhou and Xiangtan were (183±73), (201±84) and (190±66) g/m3 respectively, and the average PM10 were (171±82), (178±65) and (179±55) g/m3 respectively. The lowest TSP and PM10 concentrations occurred at the background Shaping site of Changsha. The average ratio of (PM10)/ (TSP) was 91.9%, ranging from 81.3% to 98.9%. Concerning heavy metals, in TSP samples, the concentration of Cr, As, Cd and Pb were 28.8-56.5, 18.1-76.3, 3.9-26.1 and 148.0-460.9 ng/m3, respectively, while in PM10 samples, were 16.4-42.1, 15.5-67.9, 3.3-22.2 and 127.9-389.3 ng/m3, respectively. The enrichment factor of Cd was the highest, followed by Pb and As, while that of Cr was the lowest.
Keywords:atmospheric particles  pollution characteristics  enrichment factors  Chang-Zhu-Tan city clusters
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