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Enhanced photocatalytic activity of quantum-dot-sensitized one-dimensionally-ordered ZnO nanorod photocatalyst
Authors:Jinzhao Huang  Song Liu  Lei Kuang  Yongdan Zhao  Tao Jiang  Shiyou Liu and Xijin Xu
Institution:School of Physics and Technology, University of Jinan, Jinan 250022, China;School of Physics and Technology, University of Jinan, Jinan 250022, China;School of Physics and Technology, University of Jinan, Jinan 250022, China;School of Physics and Technology, University of Jinan, Jinan 250022, China;School of Physics and Technology, University of Jinan, Jinan 250022, China;School of Physics and Technology, University of Jinan, Jinan 250022, China;School of Physics and Technology, University of Jinan, Jinan 250022, China
Abstract:An efficient photocatalyst was fabricated by assembling quantum dots (QDs) onto one-dimensionally-ordered ZnO nanorods, and the photocatalytic properties for Methyl Orange degradation were investigated by scanning electron microscopy, transmission electron microscopy, X-ray diffraction, UV-Vis-NIR absorption spectroscopy and photoluminescence. The results indicate that the catalyst with assembled QDs is more favorable for the degradation than the pristine ZnO nanorods. The QDs with core-shell structure lower the photocatalytic ability due to the higher carrier transport barrier of the ZnS shell layer. Besides its degradation efficiency, the photocatalyst has several advantages given that the one-dimensionally-ordered ZnO nanorods have been grown directly on indium tin oxide substrates. The article provides a new method to design an effective and easily recyclable photocatalyst.
Keywords:quantum dots  one-dimensionally-ordered ZnO nanorods  photocatalyst
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