Radon and thoron monitoring in the environment of Kumaun Himalayas: survey and outcomes

Monitoring of radon, thoron and their daughter products was carried out in houses of Kumaun Himalaya, India using LR-115 plastic track detectors. The measurements were made in residential houses from June 1999 to May 2000 at a height of 2.5 m from ground level using a twin chamber radon dosimeter. The twin chamber radon dosimeter can record the values of radon, thoron and their decay products separately. Maximum and minimum indoor radon and thoron concentrations were evaluated and activity concentrations of radon and thoron daughters were estimated. The resulting dose rates due to radon, thoron and their decay products varied from 0.04 to 1.89 microSv/h. A detailed analysis of the distribution of radon, thoron and their decay products inside the house is also reported. The observed dose rates inside the houses of Kumaun Himalaya were found to be lower than the ICRP recommended value of 200 Bq/m3 and thus are within safe limits.     

Indoor air quality: Radon—Report on a WHO working group

The WHO Regional Office for Europe organized a working group in Dubrovnik, Yugoslavia, on 26–30 August 1985, which discussed radon as a pollutant affecting indoor air quality. Much of the natural background radiation to which the general public is exposed comes from the decay of ²²⁶Ra which produces radon gas and other products. Because radium is a trace element in most rock and soil, indoor concentrations of radon can come from a wide variety of substances, such as building materials and the soil under building foundations. Tap water taken from wells or underground springs may be an additional source. Radon daughter concentrations are considerably higher indoors than outdoors and are of the order of 2–5 Bq m⁻³ equilibrium equivalent radon (EER) concentration. It has been estimated that current exposure to radon gas could account for as much as 5–15% of all lung cancer deaths. It was recommended that, in general, buildings with concentrations of more than 100 Bq m⁻³ EER, as an annual average, should be considered for remedial action to lower such concentrations if simple measures are possible.     

Radon gas distribution in natural gas processing facilities and workplace air environment

Evaluation was made of the distribution of radon gas and radiation exposure rates in the four main natural gas treatment facilities in Syria. The results showed that radiation exposure rates at contact of all equipment were within the natural levels (0.09-0.1 microSvh(-1)) except for the reflex pumps where a dose rate value of 3 microSvh(-1) was recorded. Radon concentrations in Syrian natural gas varied between 15.4 Bq m(-3) and 1141 Bq m(-3); natural gas associated with oil production was found to contain higher concentrations than the non-associated natural gas. In addition, radon concentrations were higher in the central processing facilities than the wellheads; these high levels are due to pressurizing and concentrating processes that enhance radon gas and its decay products. Moreover, the lowest 222Rn concentration was in the natural gas fraction used for producing sulfur; a value of 80 Bq m(-3) was observed. On the other hand, maximum radon gas and its decay product concentrations in workplace air environments were found to be relatively high in the gas analysis laboratories; a value of 458 Bq m(-3) was observed. However, all reported levels in the workplaces in the four main stations were below the action level set by IAEA for chronic exposure situations involving radon, which is 1000 Bq m(-3).     

The influence of the cigarette smoke pollution and ventilation rate on alpha-activities per unit volume due to radon and its progeny

Alpha and beta activities per unit volume air due to radon, thoron and their decay products were evaluated in the air of various cafe rooms polluted by cigarette smoke. Both CR-39 and LR-115 type II solid state nuclear track detectors (SSNTD) were used. Equilibrium factors between radon and its progeny and thoron and its daughters have been evaluated in the air of the studied cafe rooms. The committed equivalent doses due to short-lived radon decay products were determined in different regions of the respiratory tract of non-smoker members of the public. The influence of cigarette smoke pollution, ventilation rate and exposure time on committed equivalent dose in the respiratory systems of non-smokers was investigated. Committed equivalent doses ranged from 1.15 x 10(-11)-2.7 x 10(-7) Sv.y(-1)/h of exposure in the extrathoracic region and from 0.8 x 10(-12)-1.7 x 10(-8) Sv.y(-1)/h of exposure in the thoracic region of the respiratory tract of non-smokers.     

Long period study of outdoor radon concentration in Milan and correlation between its temporal variations and dispersion properties of atmosphere

The results of a survey of outdoor radon concentrations in Milan are reported. Measurements were performed hourly over a continuous four year period from January 1997 to December 2000. Radon concentration was obtained by two means: both direct measurement of radon; and measurement of its decay products. The average daily pattern of radon concentration featured a minimum in the late afternoon and a maximum in the early hours of the morning. A seasonal pattern with higher concentrations in winter than in summer (from around 15 Bq m(-3) in winter to around 5 Bq m(-3) in summer) was also observed. Similar average annual values of around 10 Bq m(-3) were obtained. The annual effective outdoor radon dose was found to be 0.12 mSv. The variation from minimum in the afternoon to maximum the following morning was found to be a good indicator of the height of the nocturnal mixing layer. The variation between maximum and minimum levels on the same day is an index of the maximum height of the mixing layer. Furthermore, our long term measurements of radon have permitted us to examine the dispersion characteristics of the atmosphere over Milan, and to establish the frequency of conditions unfavourable to the dispersion of atmospheric pollutants.     

Radon variations during treatment in thermal spas of Lesvos Island (Greece)

The aim of this paper was to study the variations of radon and daughter nuclei during treatment in the thermal spas of Lesvos Island (Greece). For this purpose, in the thermal spas of Lesvos we have measured the radon concentrations of thermal waters, as well as indoor radon, daughter and coarse particle (>500 nm) concentrations. Various instruments and procedures were employed for measurements. Radon concentrations of thermal waters were found to lie in the range 10 Bq l(-1) and 304 Bq l(-1). Concentration peaks both for radon, radon daughter and coarse particle, were found to appear during filling of baths in the treatment process. The doses delivered to the bathers during treatment were in the range of 0.00670-0.1279 mSv per year, while the doses delivered to personnel were below 20 mSv per year.     

Radon variations during treatment in thermal spas of Lesvos Island (Greece)

The aim of this paper was to study the variations of radon and daughter nuclei during treatment in the thermal spas of Lesvos Island (Greece). For this purpose, in the thermal spas of Lesvos we have measured the radon concentrations of thermal waters, as well as indoor radon, daughter and coarse particle (>500 nm) concentration. Various instruments and procedures were employed for measurements. Radon concentrations of thermal waters were found to lie in the range 10 and 304 Bq l(-1). Concentration peaks both for radon, radon daughter and coarse particle, were found to appear during filling of baths in the treatment process. The doses delivered to the bathers during treatment were in the range of 0.00670 mSv per year to 0.1279 mSv per year, while the doses delivered to personnel were below 20 mSv per year.     

Spatial and time variations of radon-222 concentration in the atmosphere of a dead-end horizontal tunnel

The concentration of radon-222 has been monitored since 1995 in the atmosphere of a 2 m transverse dimension, 128 m long, dead-end horizontal tunnel located in the French Alps, at an altitude of 1600 m. Most of the time, the radon concentration is stable, with an average value ranging from 200 Bq m(-3) near the entrance to about 1000 Bq m(-3) in the most confined section, with an equilibrium factor between radon and its short-lived decay products varying from 0.61 to 0.78. However, radon bursts are repeatedly observed, with amplitudes reaching up to 36 x 10(3) Bq m(-3) and durations varying from one to several weeks, with similar spatial variations along the tunnel as the background concentration. These spatial variations are qualitatively interpreted in terms of natural ventilation. Comparing the radon background concentration with the measured radon exhalation flux at the wall yields an estimate of 8+/-2 x 10(-6) s(-1) (0.03+/-0.007 h(-1)) for the ventilation rate. The hypothesis that the bursts could be due to transient changes in ventilation can be ruled out. Thus, the bursts are the results of transient increased radon exhalation at the walls, that could be due to meteorological effects or possibly combined hydrological and mechanical forcing associated with the water level variations of the nearby Roselend reservoir lake. Such studies are of interest for radiation protection in poorly ventilated underground settings, and, ultimately, for a better understanding of radon exhalation associated with tectonic or volcanic processes.     

Soil radium, soil gas radon and indoor radon empirical relationships to assist in post-closure impact assessment related to near-surface radioactive waste disposal

Least squares (LS), Theil’s (TS) and weighted total least squares (WTLS) regression analysis methods are used to develop empirical relationships between radium in the ground, radon in soil and radon in dwellings to assist in the post-closure assessment of indoor radon related to near-surface radioactive waste disposal at the Low Level Waste Repository in England. The data sets used are (i) estimated ²²⁶Ra in the <2 mm fraction of topsoils (eRa226) derived from equivalent uranium (eU) from airborne gamma spectrometry data, (ii) eRa226 derived from measurements of uranium in soil geochemical samples, (iii) soil gas radon and (iv) indoor radon data. For models comparing indoor radon and (i) eRa226 derived from airborne eU data and (ii) soil gas radon data, some of the geological groupings have significant slopes. For these groupings there is reasonable agreement in slope and intercept between the three regression analysis methods (LS, TS and WTLS). Relationships between radon in dwellings and radium in the ground or radon in soil differ depending on the characteristics of the underlying geological units, with more permeable units having steeper slopes and higher indoor radon concentrations for a given radium or soil gas radon concentration in the ground. The regression models comparing indoor radon with soil gas radon have intercepts close to 5 Bq m⁻³ whilst the intercepts for those comparing indoor radon with eRa226 from airborne eU vary from about 20 Bq m⁻³ for a moderately permeable geological unit to about 40 Bq m⁻³ for highly permeable limestone, implying unrealistically high contributions to indoor radon from sources other than the ground. An intercept value of 5 Bq m⁻³ is assumed as an appropriate mean value for the UK for sources of indoor radon other than radon from the ground, based on examination of UK data. Comparison with published data used to derive an average indoor radon: soil ²²⁶Ra ratio shows that whereas the published data are generally clustered with no obvious correlation, the data from this study have substantially different relationships depending largely on the permeability of the underlying geology. Models for the relatively impermeable geological units plot parallel to the average indoor radon: soil ²²⁶Ra model but with lower indoor radon: soil ²²⁶Ra ratios, whilst the models for the permeable geological units plot parallel to the average indoor radon: soil ²²⁶Ra model but with higher than average indoor radon: soil ²²⁶Ra ratios.     

Occupational exposure of phosphate mine workers: airborne radioactivity measurements and dose assessment

Under the Egyptian program for radiation safety and control, airborne radioactivity measurements and radiological dose assessment were conducted in some phosphate and uranium mines. Abu-Tartor mine is one of the biggest underground phosphate mines in Egypt. Airborne radioactivity, radon ((222)Rn) and its short-lived decay products (progenies) and thoron ((220)Rn), were measured in selected locations along the mine. The environmental gamma and workers dose equivalent rate (mSv/y) were measured inside and outside the mine using thermo-luminescence dosimeters (TLD). The results were presented and discussed. The calculated annual effective dose due to airborne radioactivity is the main source of occupational exposure and exceeding the maximum recommended level by ICRP-60 inside the mine tunnels. A number of recommendations are suggested to control the occupational exposures.     

The practical use of electrets in a public health radon remediation campaign

As part of a long-term assessment of domestic radon in Northamptonshire, England, a batch of 50 commercially available electrets was deployed for nearly 1,000 exposures, individual exposure periods ranging from one to eight weeks. Responsivity was comparable with that of recently-calibrated Durridge RAD-7 continuously-monitoring equipment. Voltage history analysis indicated mean voltage decay during manufacturers' QA assessment of 0.059+/-0.026 Vday(-1), increasing to 0.114+/-0.073 Vday(-1) during storage to first use and to 0.204+/-0.49 Vday(-1) during inter-deployment storage. At a representative elevated radon concentration of 500 Bqm(-3), the resulting perturbation is 3% over a 7-day deployment; at the typical mean Northamptonshire level of 80 Bqm(-3) it approaches 22%. Each electret can be used for up to 25 measurements, which makes the technology attractive for organisational use. It is not suited for deployment by individual householders.     

Time-integrating radon gas measurements in domestic premises: comparison of short-, medium- and long-term exposures

To identify the most applicable technology for the short-term assessment of domestic radon levels, comparative assessments of a number of integrating detector types, including track-etch, electret and activated charcoal were undertaken. Thirty-four unremediated dwellings in a high-radon area were monitored using track-etch detectors exposed for one-month and three-month periods. In parallel, one-week measurements were made in the same homes at one-month intervals, using co-located track-etch, charcoal and electret detectors exposed simultaneously, while three of the homes were also monitored by continuous-sampling detectors at hourly intervals over extended periods. Calibration of dose-integrating devices against each other and against continuous-monitoring systems confirmed good responsivity and linearity. Although track-etch, charcoal and electret devices are suitable in principle for one-week measurements, zero-exposure offset and natural radon variability cause many one-week results to be equivocal, necessitating repetition of the measurement. One-week exposures can be reliable indicators in low-radon areas or for new properties, but in high-radon areas, the use of three-month exposures is indicated. This analysis also established confidence limits for short-term measurements.     

Indoor radon in a Spanish region with different gamma exposure levels

In the beginning of 1990s within the framework of a national radon survey of more than 1500 points, radon measurements were performed in more than 100 houses located in Galicia region, in the Northwest area of Spain. The houses were randomly selected only bearing in mind general geological aspects of the region. Subsequently, a nationwide project called MARNA dealt with external gamma radiation measurements in order to draw a Spanish natural radiation map. The comparison in Galicia between these estimations and the indoor radon levels previously obtained showed good agreement. With the purpose of getting a confirmation of this relationship and also of creating a radon map of the zone, a new set of measurements were carried out in 2005. A total of 300 external gamma radiation measurements were carried out as well as 300 measurements of (226)Ra, (232)Th and (40)K content in soil. Concerning radon, 300 1-m-depth radon measurements in soil were performed, and indoor radon concentration was determined in a total of 600 dwellings. Radon content in soil gave more accurate indoor radon predictions than external gamma radiation or (226)Ra concentration in soil.     

Two error components model for measurement error: application to radon in homes

In this paper, a simple model for analysing variability in radon concentrations in homes is tested. The approach used here involves two error components, representing additive and multiplicative errors, together with variation between-houses. We use a Bayesian approach for our analysis and apply this model to two datasets of repeat radon measurements in homes; one based on 3-month long measurements for which the original measurements were close to the current UK Radon Action Level (200 Bq m⁻³), and the other based on 6-month measurement data (from regional and national surveys), for which the original measurements cover a wide range of radon concentrations, down to very low levels. The model with two error components provides a better fit to these datasets than does a model based on solely multiplicative errors.     

Experimental methods of determining the activity depth distribution of implanted 210Pb in glass

Glass is often used in radon surveys to estimate retrospective radon concentrations, as radon progenies are embedded in the upper surface layer. Experimental methods based on etching to determine the depth distribution of recoil-implanted 210Po in glass from radon decay in air is presented. By carefully controlling chemical concentrations and exposure time during which the glass is etched, stepwise removal of the surface material was possible. Two different etching agents, diluted HF/HNO3 and NaOH were utilised, with very similar results. Experimental recoil depths of 210Po agree with theoretical calculations from the literature. The maximum implantation depth obtained using this procedure was 100 +/- 20nm.     

Radon-222 in Brazil: an outline of indoor and outdoor measurements

This study discusses the methodology for measuring and assessing the radon concentration in indoor and outdoor environments. A research study was developed to investigate the long-term behavior of the diurnal and seasonal fluctuations of radon (222)Rn EEC (Equilibrium-Equivalent Concentration) and the influence of temperature and other climatic aspects on this behavior. The study was performed by means of both integrated and instantaneous measurements of radon and its short-lived daughter products for a period of 1 year in an indoor environment in Rio de Janeiro city, Brazil (reference environment), with continuous measurement, using a radon monitor with an alpha spectrometry detector.For a single day, a variability of about 50% could be observed in the (222)Rn EEC values measured on a hourly basis, with a maximum occurring early in the morning and a minimum in the afternoon. For the long-term period, seasonality is responsible for a two order of magnitude variability, with a maximum of 50 Bq.m(-3) in winter (dry season) and a minimum of 0.5 Bq.m(-3) in the summer months (wet season), outdoors. A negative correlation with temperature was observed. The conclusions of this experiment led to a survey of radon gas concentration in dwellings in Rio de Janeiro city, Brazil, in urban area with nearly 7 million inhabitants, through integrated sampling methods, using a Solid State Nuclear Track Detectors Technique (SSNTD). The study was conducted in different geomorphological locations in town. The radon gas concentration in Rio de Janeiro dwellings ranged from 5 Bq.m(-3) to 200 Bq.m(-3). A good correlation between indoor radon gas concentration and location of dwellings was observed. The seashore areas presented the lowest levels of indoor radon concentration, whereas the highest levels were found close to the mountains.     

Radon (222Rn) level variations on a regional scale: influence of the basement trace element (U, Th) geochemistry on radon exhalation rates

The approach proposed in this study provides insight into the influence of the basement geochemistry on the spatial distribution of radon (222Rn) levels both at the soil/atmosphere interface and in the atmosphere. We combine different types of in situ radon measurements and a geochemical classification of the lithologies, based on 1/50,000 geological maps, and on their trace element (U, Th) contents. The advantages of this approach are validated by a survey of a stable basement area of Hercynian age, located in South Brittany (western France) and characterized by metamorphic rocks and granitoids displaying a wide range of uranium contents. The radon source-term of the lithologies, their uranium content, is most likely to be the primary parameter which controls the radon concentrations in the outdoor environment. Indeed, the highest radon levels (> or = 100 Bq m-3 in the atmosphere, > or = 100 mBq m-2 s-1 at the surface of the soil) are mostly observed on lithologies whose mean uranium content can exceed 8 ppm and which correspond to peraluminous leucogranites or metagranitoids derived from uraniferous granitoids.     

In-field radon measurement in water: a novel approach

This paper presents a novel approach of measuring radon in-water in the field by inserting a MEDUSA gamma-ray detector into a 210 L or 1000 L container. The experimental measurements include investigating the effect of ambient background gamma-rays on in-field radon measurement, calibrating the detector efficiency using several amounts of KCl salt dissolved in tap water, and measuring radon in borehole water. The results showed that there is fairly good agreement between the field and laboratory measurements of radon in water, based on measurements with Marinelli beakers on a HPGe detector. The MDA of the method is 0.5 Bq L⁻¹ radon in-water.     

Radon mapping by retrospective measurements - an approach based on CDs/DVDs

This article points out the ability to map retrospective ²²²Rn concentrations by home stored CDs/DVDs. The method employs the high radon absorption ability of the polycarbonate material of CDs and DVDs and their track-etch properties. The principle steps for the application of the method are addressed. The possibility for individual a posteriori calibration is studied, demonstrating that better than 10% accuracy in retrospective measurements is potentially achievable. Results from retrospective measurements in three different regions are shown, demonstrating the potential of the method for large-scale radon mapping. Comparison with independently evaluated retrospective ²²²Rn concentrations in places with known radon history was made and very good correspondence was observed. The experience indicates that the method can be used for large scale retrospective radon mapping and its applications can be expanded towards mapping of radon concentrations in water and soil gas.     

Radon and its daughter products behaviour in the air of an underground tourist route in the former arsenic and gold mine in Z?oty Stok (Sudety Mountains, SW Poland).

This paper describes the occurrence of radon and its daughter products in the accessible workings, partially open to the public, in the former arsenic and gold mine in Zloty Stok. The geology of the area and the characteristics of the workings provide the background for explanation of the genesis of radon and its daughter products and of the spatial and temporal variations in their concentrations. The results demonstrate that well-ventilated areas along the tourist route have the lowest values of all the measured parameters and that temporal variations of these parameters are irregular. The highest concentration values for radon (up to 18.50kBq/m3) and its daughter products (up to 14.49kBq/m3) have been recorded in the workings with obstructed natural ventilation. These are the areas where seasonal oscillations in the concentrations of these isotopes have been registered, with the maxima in summer and the minima in winter. These sections of the workings are inaccessible to the casual visitor. Radon is supplied to the workings from the side walls and its concentration is influenced, most of all, by ventilation and the degree of rock fissuring. The reason is the uniform and not very high content of 226Ra in the rocks where the galleries were excavated. Only locally, in the workings of the Gertruda adit lying outside the tourist route, do open fault zones have significant influence on enhanced concentrations of radon and its daughter products. These fault zones constitute effective routes of radon migration to the workings. In spite of this, it must be stated that neither guides nor tourists are exposed to excessive concentrations of radon or its daughter products in the tourist route area. However, the extension of the route to other workings will require the introduction of forced ventilation in order to lower theconcentration of radon and its daughter products. reserved.