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1.
药品和个人护理用品(PPCPs)对环境的污染现状与研究进展 总被引:24,自引:0,他引:24
在过去的30多年中,有关有毒污染物的研究主要集中在工业化学物质和农药上。近5年多来,国外已经开始关注药品和个人护理用品(PPCPs)对环境的污染,但在我国还没有引起重视。国外的研究表明,合成麝香物质、显影剂、抗生素、雌激素、消炎止痛药、杀菌消毒剂等与人类生活密切相关的药品和个人护理用品在环境中普遍存在,但是其质量浓度通常非常低,多数情况下在ng/L~μg/L水平。粪便施肥和污水排放是PPCPs进入环境的主要途径。在常见的PPCPs中,抗生素和消炎止痛药在环境中检测出的频率最高,在地表水、地下水、饮用水、污泥、土壤等环境介质中,PPCPs在地表水中检测出的频率最高。目前关于PPCPs的研究主要集中在分析方法以及环境污染水平的调查,有关PPCPs在环境中的迁移转化规律,生态与健康风险以及PPCPs污染控制技术等方面的研究有待加强。 相似文献
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Xueqi Fan Jie Gao Wenchao Li Jun Huang Gang Yu 《Frontiers of Environmental Science & Engineering》2020,14(1):8
3.
Endocrine disrupting compounds (EDCs), pharmaceuticals and personal care products (PPCPs) have attracted much attention due to widespread contamination in aquatic environment. In this study, we determined 13 EDCs and PPCPs in fish blood, bile and muscle by using gas chromatography-mass spectrometry (GC-MS). The limits of quantitation (LOQ) were in the ranges of 0.23–2.54, 0.22–2.36 ng·mL−1, and 0.24–2.57 ng·g−1 dry weight (dw) for fish blood, bile and muscle, respectively. Recoveries of target compounds spiked into sample matrices and passed through the entire analytical procedure ranged from 65% to 95%, from 60% to 92% and from 62% to 91% for blood, bile and muscle, respectively. The methods were applied to the analysis of fish from a lake in California. Target compounds were relatively low in bile, and only bisphenol A (BPA) and diclofenac were measurable near the LOQ. Seven of 13 compounds were detected in blood, with total concentrations up to 39 ng·mL−1. Only BPA was frequently found in muscle, with mean concentration of 7.26 ng·g−1 dw. The estimated daily intake of BPA through fish consumption for U.S. resident was significantly lower than the tolerable daily intake recommended by the European Food Safety Authority. This study showed that the exposure to the bisphenol A from fish diet is unlikely to pose a health risk. 相似文献
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Jie GAO Jun HUANG Weiwei CHEN Bin WANG Yujue WANG Shubo DENG Gang YU 《Frontiers of Environmental Science & Engineering》2016,10(3):491-501
The fate and removal of pharmaceuticals and personal care products (PPCPs) in wastewater treatment plants (WWTPs) has received great attention during the last decade. Numerous data concerning concentrations in the water phase can be found in the literature, however corresponding data from sludge as well as associated mass balance calculations are very limited. In the present study, the adsorbed and dissolved concentrations of 9 PPCPs were investigated in each unit of a WWTP in Beijing, China. Based on the calculation of mass balance, the relative mass distribution and removal efficiency of each target compound was obtained at each process. The amount of PPCPs entering into the WWTP ranged from 12 g·d–1 to 3848 g·d–1. Five target compounds (caffeine, chloramphenicol, bezafibrate, clofibric acid, and N,N-diethyl-meta-toluamide) were effectively removed, with rates of 57%–100%. Negative removal efficiencies were obtained for sulpiride, metoprolol, nalidixic acid, and carbamazepine, ranging from -19% to -79%. PPCPs mainly existed in dissolved form (≥92%) in both the raw influent and the final effluent. The sludge cake carried a much lower amount of PPCPs (17 g·d–1) compared with the discharged effluent (402 g·d–1). In A2/O treatment tanks, the anaerobic and anoxic tanks showed good performance for PPCPs removal, and the amount of adsorbed PPCPs was increased. The results reveal that both the dissolved and the adsorbed phases should be considered when assessing the removal capacity of each A2/O tank. 相似文献
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Wentao Zhao Ying Guo Shuguang Lu Pingping Yan Qian Sui 《Frontiers of Environmental Science & Engineering》2016,10(6):2
Pharmaceuticals and personal care products (PPCPs) have been regarded as an emerging problem in the surface water environment in the past few decades. In China, although related studies were initiated several years ago, an increasing number of studies on this topic have been conducted in recent years. These studies have expanded knowledge of their occurrence, behavior and associated risk in the surface water environment in China. This review compiles the most recent literature related to the studies of PPCPs in the surface water environment in China. It includes PPCP occurrence in surface water and sediments, their geographical distribution, and outcomes of the associated risk assessment. It shows that antibiotics have received much more attention in both surface water and sediments than other PPCPs. Compared to other countries; most antibiotics in the collected sediments in China showed higher contamination levels. Many more study areas have been covered in recent years; however, attention has been given to only specific areas. Environmental risk assessment based on risk quotients indicated that sulfamethoxazole presents the most significant environmental risk to relevant aquatic organisms; followed by ofloxacin, ciprofloxacin, enrofloxacin, 17α-ethynylestradiol, ibuprofen and diclofenac. Despite limited research on the environmental risk assessment of PPCPs in sediments, higher risks posed by PPCPs in the sediments rather than surface water were identified highlighting the need for further risk assessment of PPCPs in sediment samples.
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7.
Qian SUI Jun HUANG Shuguang LU Shubo DENG Bin WANG Wentao ZHAO Zhaofu QIU Gang YU 《Frontiers of Environmental Science & Engineering》2014,8(1):62-68
The application of appropriate advanced treat- ment process in the municipal wastewater treatment plants (WWTPs) has become an important issue considering the elimination of emerging contaminants, such as pharma- ceutical and personal care products (PPCPs). In the present study, the removal of 13 PPCPs belonging to different therapeutic classes by the sequential ultraviolet (UV) and ozonation process in a full-scale WWTP in Beijing was investigated over the course of ten months. Most of the target PPCPs were effectively removed, and the median removal efficiencies of individual PPCPs, ranging from -13% to 89%, were dependent on their reaction rate constants with molecular ozone. Noticeable fluctuation in the removal efficiencies of the same PPCPs was observed in different sampling campaigns. Nevertheless, the sequential UV and ozonation process still made a significant contribution to the total elimination of most PPCPs in the full-scale WWTP, by compensating for the poor or fluctuant removal performance of PPCPs by biologic treatment process. 相似文献
8.
Landfill gas (LFG) utilization which means a synergy between environmental protection and bioenergy recovery was investigated in this study. Pressure swing adsorption technology was used in LFG purification, and laboratory experiment, pilot-scale test, and on-site demonstration were carried out in Shenzhen, China. In the laboratory experiment, A-type carbon molecular sieve was selected as the adsorbent by comparison of several other adsorbents. The optimal adsorption pressure and adsorption time were 0.25 MPa and 2 min, respectively, under which the product generation rate was 4.5 m3/h and the methane concentration was above 90%. The process and optimization of the pilot-scale test were also reported in the paper. The product gas was of high quality compared with the National Standard of Compressed Natural Gas as Vehicle Fuel (GB18047-2000), when the air concentration in feed gas was under 10.96%. The demonstration project was composed of a collection system, production system, and utilization system. The drive performance, environmental protection performance, and economic feasibility of the product gas — as alternative fuel in passenger car, truck, and bulldozer—were tested, showing the feasibility technology for LFG utilization. 相似文献
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Jimoh O. Tijani Ojo O. Fatoba Omotola O. Babajide Leslie F. Petrik 《Environmental Chemistry Letters》2016,14(1):27-49
The presence of emerging micropollutants such as pharmaceuticals, endocrine disruptors, personal care products, nanomaterials and perfluorinated substances in the environment remains a great threat to the health and safety of humans and aquatic species. These micropollutants enter the environment via anthropogenic activities and have been detected in surface water, groundwater and even drinking water at nanogram per litre to microgram per litre concentration. To date, limited information exists on the fate, behaviours, and pathways of these micropollutants in the environment. The potential ecotoxicological effects on the receptors due to exposure to individual or mixture of these chemicals still remain unknown. This review provides an overview on pharmaceuticals, endocrine disrupting compounds, personal care products, nanomaterials and perfluorinated pollutants, with emphasis on their occurrences, effects, environmental fates, and potential risk of exposure in water, soil or sediment. Based on the literature survey, it was found that in spite of an extensive research and different developmental efforts on the challenges of emerging micropollutants, the solution to the problem of emerging micropollutants in the environment is far from being solved. The needs for behavioural change among citizens, strong political will and policy formulation on the part of government are identified as possible panacea for combating the growing influence of these potential damaging substances. Suggestions on proactive and precautionary measures that must be taken to protect the environment as well as guarantee the health and safety of humans and aquatic species are provided. Future research should concentrate on the development of a risk based screening models and framework that can predict the sources, fate and behaviours of emerging contaminants in the environment is recommended. 相似文献
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Anand Uttpal Adelodun Bashir Cabreros Carlo Kumar Pankaj Suresh S. Dey Abhijit Ballesteros Florencio Bontempi Elza 《Environmental Chemistry Letters》2022,20(6):3883-3904
Almost all aspects of society from food security to disease control and prevention have benefited from pharmaceutical and personal care products, yet these products are a major source of contamination that ends up in wastewater and ecosystems. This issue has been sharply accentuated during the coronavirus disease pandemic 2019 (COVID-19) due to the higher use of disinfectants and other products. Here we review pharmaceutical and personal care products with focus on their occurrence in the environment, detection, risk, and removal.
相似文献12.
Xinshu Jiang Yingxi Qu Liquan Liu Yuan He Wenchao Li Jun Huang Hongwei Yang Gang Yu 《Frontiers of Environmental Science & Engineering》2019,13(2):27
13.
Assessment of the contribution of land use pattern and intensity to landscape quality: use of a landscape indicator 总被引:4,自引:0,他引:4
The objective of this research work is the evaluation of the impact of landuse pattern and intensity on landscape by means of an indicator. The method used to calculate a ‘landscape indicator’ (Iland) allows to take into account the objective as well as the subjective approach of landscape. Iland corresponds to the degree of agreement between landscape supply by farmers and landscape demand by the social groups. The supply and the demand are evaluated through four criteria: ‘diversity’, ‘upkeep’, ‘openness’ and ‘heritage’. The landscape supply is calculated from data of landscape objects (punctual, linear and spatial) for each criterion recorded at the field level. The values of the four criteria for the landscape demand are allocated by the user(s) of the indicator (decision makers, regional council, social groups…) into five classes (0–4). The value of the landscape indicator is the least favourable difference between supply and demand for the four criteria. An example of calculation of the ‘landscape indicator’ for an arable farm is given. The collection of data needs 2 h with the farmer and 2 h for a survey of the farm land. 相似文献
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In this research, the data envelopment analysis (DEA) model of measuring the eco-efficiency of urban material metabolism has been constructed based on the urban material input and output indicators. According to the data of Xiamen from 1985 to 2007, an empirical study was conducted to measure the eco-efficiency of urban material metabolism using DEA program. The results showed a general downtrend of Xiamen's eco-efficiency of material metabolism from 1985 to 2007, in which there were 15 efficient years and eight inefficient years. The eco-efficiency and urbanization rate of Xiamen was remarkably negatively correlated. Moreover, the results revealed at 4 years (1995, 2001, 2002 and 2003) there had been undesirable output slack (environmental pollution), and at 2 years (1991 and 1999) there had been desirable output slack (GDP), and at 8 years there had been input slack (water, land, food and energy), especially for water and energy. Finally, some suggestions on promoting the eco-efficiency of urban material metabolism were put forward. 相似文献
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我国地表水中药物与个人护理品污染现状及其繁殖毒性筛查 总被引:2,自引:0,他引:2
根据文献报道,我国地表水中已检出至少144种药物及个人护理用品(pharmaceuticals and personal care products,PPCPs),包括抗生素、激素、其他药物、个人护理品(personal care products,PCPs)4大类,其中检出浓度最高的达到了μg·L~(-1)量级,在长期的污染下有可能对水生生物产生内分泌干扰效应或繁殖毒性,进而影响到整个水生生物种群的繁衍变化。因此,有必要根据我国地表水中PPCPs的污染水平,筛查出具有潜在生态风险的PPCPs。由于目前缺乏针对PPCPs类污染物的筛选体系,以国内外优先控制污染物筛选体系为基础,借鉴基于风险的欧洲兽药分级方法,利用风险指数(risk index,RI),筛选得出目前我国的地表水中有16种具有繁殖毒性的PPCPs的RI1,包括1种抗生素,5种激素类药物,3种其他药物和7种PCPs,其中乙炔雌二醇(ethinylestradiol,EE2)的RI最高(115 730),其次是壬基酚(nonylphenol,NP)(1 796)、邻苯二甲酸二丁酯(dibutyl phthalate,DBP)(255.31),对水生态环境有较高的风险的PPCPs需进一步进行较高层次的风险评价。 相似文献
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Changbo ZHANG Qishi LUO Chunnu GENG Zhongyuan LI 《Frontiers of Environmental Science & Engineering》2010,4(4):395-404
Stabilization is one of the best demonstrated available technologies for treating toxic pollutants in soils and has been used worldwide but is rarely used for treatment of contaminated sites in China despite many bench-scale studies. Here, a field-scale application of stabilization treatment in Shanghai, China was summarized to demonstrate the whole engineering process and the key technical issues regarding stabilization of contaminated soil. A site contaminated with arsenic (As) and polycyclic aromatic hydrocarbons (PAHs), formerly used as a lighting plant in Shanghai, was chosen as the demonstration site. Stabilizing measures were taken to treat the contaminated soil to reuse the site for residential purposes. The whole engineering remediation process consisted of phase I environmental site assessment (ESA) and phase II ESA, quantitative human health risk assessment, remediation alternatives evaluation, bench-scale testing, remedial design, engineering implementation, and post-remediation assessment. A third party conducted evaluation monitoring indicated desirable results were achieved via the stabilization treatment. In addition, some technical obstacles related to soil stabilization treatment were discussed, including soil quality evaluation, stabilization effectiveness validation, and soil reuse assessment. 相似文献
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Binbin Sheng Depeng Wang Xianrong Liu Guangxing Yang Wu Zeng Yiqing Yang Fangang Meng 《Frontiers of Environmental Science & Engineering》2020,14(6):93
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Energy consumption is a major cause of air pollution in Beijing, and the adjustment of the energy structure is of strategic importance to the reduction of carbon intensity and the improvement of air quality. In this paper, we explored the future trend of energy structure adjustment in Beijing till 2020, designed five energy scenarios focusing on the fuel substitution in power plants and heating sectors, established emission inventories, and utilized the Mesoscale Modeling System Generation 5 (MM5) and the Models-3/Community Multiscale Air Quality Model (CMAQ) to evaluate the impact of these measures on air quality. By implementing this systematic energy structure adjustment, the emissions of PM10, PM2.5, SO2, NO x , and non-methane volatile organic compounds (NMVOCs) will decrease distinctly by 34.0%, 53.2%, 78.3%, 47.0%, and 30.6% respectively in the most coalintensive scenario of 2020 compared with 2005. Correspondingly, MM5-Models-3/CMAQ simulations indicate significant reduction in the concentrations of major pollutants, implying that energy structure adjustment can play an important role in improving Beijing??s air quality. By fuel substitution for power plants and heating boilers, PM10, PM2.5, SO2, NO x , and NMVOCs will be reduced further, but slightly by 1.7%, 4.5%, 11.4%, 13.5%, and 8.8% respectively in the least coal-intensive scenario. The air quality impacts of different scenarios in 2020 resemble each other, indicating that the potential of air quality improvement due to structure adjustment in power plants and heating sectors is limited. However, the CO2 emission is 10.0% lower in the least coal-intensive scenario than in the most coal-intensive one, contributing to Beijing??s ambition to build a low carbon city. Except for energy structure adjustment, it is necessary to take further measures to ensure the attainment of air quality standards. 相似文献
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Yiyi Jiang 《国际发展与全球生态学杂志》2013,20(2):117-126
Studying eco-sustainability of tourism areas is part of sustainable development research. In tourism areas, the ecosystem comprises both the environment and the human system. The environmental system is basically physical, whereas the human system, consisting of both tourists and residents, is the dominant factor driving ecosystem change. If the combined influence of tourists and residents exceeds the carrying capacity of the environment, which is the ecological threshold of eco-sustainability in the tourism area, then the structure, function and stability of the environment will degenerate. Hence, eco-sustainability assessment of tourism areas should be based on analyses of the relationship between the influence of tourists and residents on the environment and the environmental carrying capacity. Using ecological footprint and tourism ecological footprint models, we developed and applied a synthetic assessment index system for eco-sustainability of tourism areas in Lijiang County, Yunnan Province, China, to conduct a quantitative spatial assessment for 2001. The eco-sustainability of Lijiang was high, with a harmonious relationship between regional socioeconomic development and the ecological environment. There were significant spatial differences in eco-sustainability among 24 towns in the region because of spatial heterogeneity in socioeconomic status, tourism development and environmental elements. 相似文献